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Physica A Statistical Mechanics and its Applications

Master equation for a quantum system driven by a strong periodic field in the quasienergy representation

Ioannis E. Antoniou, Yu. Melnikov, Bi Qiao

Published Nov 1, 1997• 25 citations
Publisher
DOI
10.1016/s0378-4371(97)00343-9

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We study the dynamics of open quantum systems driven by an external time-periodic force. Combining Floquet theory and the time-convolutionless projection operator technique we derive a time-local quantum master equation which exactly takes into account the periodic driving, while treating the system-environment interaction within second order in the coupling strength without performing the Markov approximation. The resulting equation of motion for the reduced density matrix is called Floquet time-convolutionless master equation. Employing the example of the driven spin-boson system, we demonstrate that this master equation is capable of describing strong non-Markovian effects, while yielding the Floquet-Lindblad master equation in the Markovian limit. A characteristic feature of memory effects in such driven dissipative systems is the emergence of sharp peaks of the trace-distance based non-Markovianity measure as a function of the driving amplitude, which can be traced back to quasienergy crossings leading to almost decoherence-protected subspaces through a quasienergy-induced dissipative decoupling mechanism.
Periodically driven quantum systems are commonly modeled using master equations constructed in the eigenbasis of an undriven Hamiltonian, implicitly assuming that environmental dissipation couples to static energy transitions even under strong time-periodic driving. The validity of this approximation beyond weak or near-resonant driving remains poorly understood. To address the need for a more self-consistent quantum theory approach, we formulate a nonsecular Floquet--Markov generalized master equation (F-GME) in the quasienergy basis, treating interaction-induced (internal) and drive-induced (external) nonperturbative dressing on an equal footing. We subsequently investigate dissipation in two minimal driven open quantum systems---a harmonically driven two-level system and a harmonically driven coupled-two-level-system---each weakly coupled to a Markovian bath. Comparing the F-GME to a time-independent dressed-basis master equation, we show that even for a flat-bath spectral density and weak dissipation, the two approaches can yield qualitatively different steady-state populations and emission spectra. We resolve dissipation into drive-assisted sideband processes decaying via Floquet extended-space quasienergy channels, and show these channels can hybridize through nonsecular couplings into collective Floquet--Liouville modes governing observable spectral resonances. This analysis demonstrates that time-independent dissipative descriptions can incorrectly weight multiphoton Floquet transitions by collapsing quasienergy-resolved decay pathways into static energy gaps. The F-GME framework provides a systematic diagnostic for identifying regimes where Floquet-consistent dissipation is essential and clarifies the physical origin of discrepancies between commonly used master-equation approaches.