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Physical Review Letters

Dynamics of the Pairing Interaction in the Hubbard and t−J Models of High-Temperature Superconductors

Thomas Maier, Didier Poilblanc, Douglas J. Scalapino

Published Jun 10, 2008• 147 citations
Publisher

Abstract

The question of whether one should speak of a "pairing glue" in the Hubbard and t-J models is basically a question about the dynamics of the pairing interaction. If the dynamics of the pairing interaction arises from virtual states, whose energies correspond to the Mott gap, and give rise to the exchange coupling J, the interaction is instantaneous on the relative time scales of interest. In this case, while one might speak of an "instantaneous glue," this interaction differs from the traditional picture of a retarded pairing interaction. However, as we will show, the dominant contribution to the pairing interaction for both of these models arises from energies reflecting the spectrum seen in the dynamic spin susceptibility. In this case, the basic interaction is retarded, and one speaks of a spin-fluctuation glue which mediates the d-wave pairing.

DOI
10.1103/physrevlett.100.237001

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The question of whether one should speak of a "pairing glue" in the Hubbard and t-J models is basically a question about the dynamics of the pairing interaction. If the dynamics of the pairing interaction arises from virtual states, whose energies correspond to the Mott gap, and give rise to the exchange coupling J, the interaction is instantaneous on the relative time scales of interest. In this case, while one might speak of an "instantaneous glue," this interaction differs from the traditional picture of a retarded pairing interaction. However, as we will show, the dominant contribution to the pairing interaction for both of these models arises from energies reflecting the spectrum seen in the dynamic spin susceptibility. In this case, the basic interaction is retarded, and one speaks of a spin-fluctuation glue which mediates the d-wave pairing.
The question of whether one should speak of a "pairing glue" in the Hubbard and t-J models is basically a question about the dynamics of the pairing interaction. If the dynamics of the pairing interaction arises from virtual states, whose energies correspond to the Mott gap, and give rise to the exchange coupling J, the interaction is instantaneous on the relative time scales of interest. In this case, while one might speak of an "instantaneous glue", this interaction differs from the traditional picture of a retarded pairing interaction. However, if the energies correspond to the spectrum seen in the dynamic spin susceptibility, then the interaction is retarded and one speaks of a spin-fluctuation glue which mediates the d-wave pairing. Here we present results from numerical studies which provide insight into this question.
The occurrence of retarded (with glue) and unretarded (without glue) pairing is thoroughly discussed in cuprates. We analyze some aspects of this problem in the context of the $t\text{\ensuremath{-}}J\text{\ensuremath{-}}V$ model in a large-NNN approximation. When 1/N1/N1/N renormalizations are neglected the mean-field result is recovered, where the unretarded ddd-wave superconducting pairing triggered by the spin-exchange interaction JJJ is obtained. However, the presence of a nonnegligible nearest-neighbors Coulomb interaction V(q)V(\mathbf{q})V(q) kills superconductivity. If the non-double-occupancy constraint and its fluctuations are considered, the situation changes drastically. In this case, V(q)V(\mathbf{q})V(q) is screened making ddd-wave superconductivity very robust. In addition, we show that the early proposal for the presence of an unretarded pairing contribution triggered by the spin-exchange interaction JJJ can be discussed in this context.
Cluster dynamical mean-field calculations are used to construct the superconducting gap function of the two-dimensional Hubbard model. The frequency dependence of the imaginary part of the gap function indicates that the pairing is dominated by fluctuations at two characteristic frequencies: one at the scale of the hopping matrix element ttt and one at a much lower scale. The lower-frequency component becomes more important as the doping is reduced into the pseudogap regime. Comparison to information on the spin-fluctuation spectrum of the model suggests that superconductivity arises from exchange of spin fluctuations. The inferred pairing glue function is in remarkable qualitative consistency with the pairing function inferred from optical conductivity data.
We study the dynamics of the Cooper pairing across the T = 0 phase diagram of the two-dimensional Hubbard model, relevant for high-temperature superconductors, using a cluster extension of dynamical mean-field theory. We find that the superconducting pairing function evolves from an unconventional form in the overdoped region into a more conventional boson-mediated retarded form in the underdoped region of the phase diagram. The boson, however, promotes the rise of a pseudogap in the electron density of states rather than a superconducting gap as in the standard theory of superconductivity. We discuss our results in terms of Mott-related phenomena, and we show that they can be observed in tunneling experiments.
Many theoretical approaches find ddd-wave superconductivity in the prototypical one-band Hubbard model for high-temperature superconductors. At strong coupling ($U\ensuremath{\ge}W$, where UUU is the on-site repulsion and W=8tW=8tW=8t the bandwidth) pairing is controlled by the exchange energy J=4t2/UJ=4{t}^{2}/UJ=4t2/U. One may then surmise, ignoring retardation effects, that near-neighbor Coulomb repulsion VVV will destroy superconductivity when it becomes larger than JJJ, a condition that is easily satisfied in cuprates, for example. Using cellular dynamical mean-field theory with an exact diagonalization solver for the extended Hubbard model, we show that pairing at strong coupling is preserved, even when $V\ensuremath{\gg}J$, as long as $V\ensuremath{\lesssim}U/2$. While at weak coupling VVV always reduces the spin fluctuations and hence ddd-wave pairing, at strong coupling, in the underdoped regime, the increase of $J=4{t}^{2}/(U\ensuremath{-}V)$ caused by VVV increases binding at low frequency while the pair-breaking effect of VVV is pushed to high frequency. These two effects compensate in the underdoped regime, in the presence of a pseudogap. While the pseudogap competes with superconductivity, the proximity to the Mott transition that leads to the pseudogap, and retardation effects, protect ddd-wave superconductivity from VVV.
A microscopic theory of superconductivity in the extended Hubbard model which takes into account the intersite Coulomb repulsion and electron-phonon interaction is developed in the limit of strong correlations. The Dyson equation for normal and pair Green functions expressed in terms of the Hubbard operators is derived. The self-energy is obtained in the noncrossing approximation. In the normal state, antiferromagnetic short-range correlations result in the electronic spectrum with a narrow bandwidth. We calculate superconducting Tc by taking into account the pairing mediated by charge and spin fluctuations and phonons. We found the d-wave pairing with high-Tc mediated by spin fluctuations induced by the strong kinematic interaction for the Hubbard operators. Contributions to the d-wave pairing coming from the intersite Coulomb repulsion and phonons turned out to be small.