Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physical Review Letters

Superresolution of Pulsed Multiphoton Raman Transitions

F. S. Cataliotti, R. Scheunemann, Theodor W. Hänsch, Martin Weitz

Published Aug 23, 2001• 21 citations
Publisher

Abstract

We have investigated higher order multiphoton Raman resonances with two pulsed optical frequencies. Multiphoton transfer with up to 50 photons is observed with milliwatts of laser power. We demonstrate that the spectral width of the multiphoton resonances can be far below the Fourier transform linewidth of the driving optical pulses. The functional dependence of the transition linewidth on the number of exchanged photons is found to vary with the pulse shape. Our experiment is performed with laser-cooled rubidium atoms confined in a CO2-laser optical dipole trap.

DOI
10.1103/physrevlett.87.113601

Related papers

CONTROLLED PHOTON EMISSION AND RAMAN TRANSITION EXPERIMENTS WITH A SINGLE TRAPPED ATOM.

M. P. A. Jones, Benoît Darquié, J. Beugnon +6 more

We present recent results on the coherent control of an optical transition in a single rubidium atom, trapped in an optical tweezer. We excite the atom using resonant light pulses that are short (4 ns) compared with the lifetime of the excited state (26 ns). By varying the intensity of the laser pulses, we can observe an adjustable number of Rabi oscillations, followed by free decay once the light is switched off. To generate the pulses we have developed a novel laser system based on frequency doubling a telecoms laser diode at 1560 nm. By setting the laser intensity to make a pi-pulse, we use this coherent control to make a high quality triggered source of single photons. We obtain an average single photon rate of 9600 s-1 at the detector. Measurements of the second-order temporal correlation function show almost perfect antibunching at zero delay. In addition, we present preliminary results on the use of Raman transitions to couple the two hyperfine levels of the ground state of our trapped atom. This will allow us to prepare and control a qubit formed by two hyperfine sub-levels.

•Jan 1, 2005•1 citation

Raman-type resonances in two-laser multiphoton ionisation

R. Parzyński

Higher-order multiphoton ionisation enhanced resonantly by Raman-type transitions is studied theoretically. This higher-order process is found to be stronger than the non-resonant lowest-order one by approximately two orders of magnitude. The shape, position, width, height and area of the resonance peaks that appear due to this process are calculated. Qualitative agreement is found between the theory and the experiment of Feldmann et al. (1986).

Journal of Physics B Atomic and Molecular Physics•Jan 14, 1987•5 citations

CONTROLLED PHOTON EMISSION AND RAMAN TRANSITION EXPERIMENTS WITH A SINGLE TRAPPED ATOM

M. P. A. JONES, Benoît Darquié, J. Beugnon +6 more

We present recent results on the coherent control of an optical transition in a single rubidium atom, trapped in an optical tweezer. We excite the atom using resonant light pulses that are short (4 ns) compared with the lifetime of the excited state (26 ns). By varying the intensity of the laser pulses, we can observe an adjustable number of Rabi oscillations, followed by free decay once the light is switched off. To generate the pulses we have developed a novel laser system based on frequency doubling a telecoms laser diode at 1560 nm. By setting the laser intensity to make a pi-pulse, we use this coherent control to make a high quality triggered source of single photons. We obtain an average single photon rate of 9600 s-1 at the detector. Measurements of the second-order temporal correlation function show almost perfect antibunching at zero delay. In addition, we present preliminary results on the use of Raman transitions to couple the two hyperfine levels of the ground state of our trapped atom. This will allow us to prepare and control a qubit formed by two hyperfine sub-levels.

arXiv:quant-ph/0508119•Laser Spectroscopy•Dec 1, 2005•1 citation

Multiphoton transitions in a spin-polarized 3D optical lattice

Andreas Hemmerich, Claus Zimmermann, Theodor W. Hänsch

We have observed novel resonances occuring at subharmonic frequencies in probe transmission spectra of ultracold atoms confined in the antinodes of a 3D optical standing wave by means of dipole forces. We interpret these resonances in terms of multiphoton Raman transitions between vibrational states of the trapped atoms.

Physical Review Letters•Jan 31, 1994•44 citations

Coherent quantum control of multiphoton transitions by shaped ultrashort optical pulses

Doron Meshulach, Yaron R. Silberberg

Multiphoton transitions can be reached by many routes through a continuum of virtual levels. We show that the transition probability of two-photon and multiphoton processes can be controlled by tailoring the shape of an ultrashort excitation pulse, so that the many paths leading to the final state interfere to give a desired probability amplitude. We analyze the effect of pulse shapes on N-photon absorption as well as on Raman transitions. We show theoretically that certain tailored dark pulses do not excite the system at all, while other shaped pulses induce transitions as effectively as transform limited pulses, even when their peak amplitudes are greatly reduced. These results are confirmed experimentally for two-photon transitions in atomic cesium.

Physical Review A•Aug 1, 1999•366 citations

Stimulated Raman transitions for cooling atoms in an optical dipole trap

Joseph D. Miller, Robert A. Cline, Daniel J. Heinzen

Optical dipole traps can provide strong, state-independent confinement of atoms. Unfortunately, the spatially dependent light shifts of optical transitions in dipole traps can interfere with conventional laser cooling techniques. These limitations may be overcome by cooling trapped atoms with stimulated Raman transitions. In particular, the lights shifts of ground state sublevels can be equal, so that the Raman cooling transition is unperturbed. Cooling in the sideband limit, to the quantum ground state of motion, should be possible. We have confined {sup 85}Rb atoms in a far-detuned optical dipole trap, and indirectly measured extremely low heating rates of the trapped atoms. We have also driven velocity-sensitive stimulated Raman transitions of the trapped atoms. The high resolution of these stimulated Raman resonances should allow us to resolve the motional sidebands and to directly cool the trapped atoms.

Bulletin of the American Physical Society•May 1, 1993•0 citations
We have investigated higher order multiphoton Raman resonances with two pulsed optical frequencies. Multiphoton transfer with up to 50 photons is observed with milliwatts of laser power. We demonstrate that the spectral width of the multiphoton resonances can be far below the Fourier transform linewidth of the driving optical pulses. The functional dependence of the transition linewidth on the number of exchanged photons is found to vary with the pulse shape. Our experiment is performed with laser-cooled rubidium atoms confined in a CO2-laser optical dipole trap.
We present recent results on the coherent control of an optical transition in a single rubidium atom, trapped in an optical tweezer. We excite the atom using resonant light pulses that are short (4 ns) compared with the lifetime of the excited state (26 ns). By varying the intensity of the laser pulses, we can observe an adjustable number of Rabi oscillations, followed by free decay once the light is switched off. To generate the pulses we have developed a novel laser system based on frequency doubling a telecoms laser diode at 1560 nm. By setting the laser intensity to make a pi-pulse, we use this coherent control to make a high quality triggered source of single photons. We obtain an average single photon rate of 9600 s-1 at the detector. Measurements of the second-order temporal correlation function show almost perfect antibunching at zero delay. In addition, we present preliminary results on the use of Raman transitions to couple the two hyperfine levels of the ground state of our trapped atom. This will allow us to prepare and control a qubit formed by two hyperfine sub-levels.
We present recent results on the coherent control of an optical transition in a single rubidium atom, trapped in an optical tweezer. We excite the atom using resonant light pulses that are short (4 ns) compared with the lifetime of the excited state (26 ns). By varying the intensity of the laser pulses, we can observe an adjustable number of Rabi oscillations, followed by free decay once the light is switched off. To generate the pulses we have developed a novel laser system based on frequency doubling a telecoms laser diode at 1560 nm. By setting the laser intensity to make a pi-pulse, we use this coherent control to make a high quality triggered source of single photons. We obtain an average single photon rate of 9600 s-1 at the detector. Measurements of the second-order temporal correlation function show almost perfect antibunching at zero delay. In addition, we present preliminary results on the use of Raman transitions to couple the two hyperfine levels of the ground state of our trapped atom. This will allow us to prepare and control a qubit formed by two hyperfine sub-levels.
Multiphoton transitions can be reached by many routes through a continuum of virtual levels. We show that the transition probability of two-photon and multiphoton processes can be controlled by tailoring the shape of an ultrashort excitation pulse, so that the many paths leading to the final state interfere to give a desired probability amplitude. We analyze the effect of pulse shapes on N-photon absorption as well as on Raman transitions. We show theoretically that certain tailored dark pulses do not excite the system at all, while other shaped pulses induce transitions as effectively as transform limited pulses, even when their peak amplitudes are greatly reduced. These results are confirmed experimentally for two-photon transitions in atomic cesium.
Optical dipole traps can provide strong, state-independent confinement of atoms. Unfortunately, the spatially dependent light shifts of optical transitions in dipole traps can interfere with conventional laser cooling techniques. These limitations may be overcome by cooling trapped atoms with stimulated Raman transitions. In particular, the lights shifts of ground state sublevels can be equal, so that the Raman cooling transition is unperturbed. Cooling in the sideband limit, to the quantum ground state of motion, should be possible. We have confined {sup 85}Rb atoms in a far-detuned optical dipole trap, and indirectly measured extremely low heating rates of the trapped atoms. We have also driven velocity-sensitive stimulated Raman transitions of the trapped atoms. The high resolution of these stimulated Raman resonances should allow us to resolve the motional sidebands and to directly cool the trapped atoms.