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Physical Review A

Squeezed-state generation via forward degenerate four-wave mixing

Prem Kumar, Jeffrey H. Shapiro

Published Sep 1, 1984• 93 citations
Publisher

Abstract

Degenerate four-wave mixing has been suggested as a possible generation scheme for squeezed-state light. A recent analysis of the quantum effects of probe-conjugate loss in backward degenerate four-wave mixing has shown that such loss puts an absolute limit on the squeezing that can be obtained via this generation scheme. In this Rapid Communication we show that it is the counter-propagating beam geometry of backward degenerate four-wave mixing that makes it ill suited for squeezed-state generation. On the other hand, the nominally copropagating beam geometry of forward degenerate four-wave mixing is shown to alleviate the absolute probe-conjugate loss limit on squeezing.

DOI
10.1103/physreva.30.1568

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Conference on Lasers and Electro-Optics•Jan 1, 2022•0 citations
Degenerate four-wave mixing has been suggested as a possible generation scheme for squeezed-state light. A recent analysis of the quantum effects of probe-conjugate loss in backward degenerate four-wave mixing has shown that such loss puts an absolute limit on the squeezing that can be obtained via this generation scheme. In this Rapid Communication we show that it is the counter-propagating beam geometry of backward degenerate four-wave mixing that makes it ill suited for squeezed-state generation. On the other hand, the nominally copropagating beam geometry of forward degenerate four-wave mixing is shown to alleviate the absolute probe-conjugate loss limit on squeezing.
The suitability of degenerate four-wave mixing (DFWM) as a source of squeezed-state (two-photon coherent state) light is investigated, both theoretically and experimentally. In previous semiclassical theory, which neglected pump quantization and loss in the nonlinear medium, Yuen and Shapiro [Opt. Lett. 4, 334 (1979)] showed that such states would be generated by 50%-50% combination of the transmitted probe (TP) and the phase-conjugate (PC) output beams of DFWM. Here the effects of quantum fluctuations in the amplitudes and phases of the pump beams are calculated in a traveling-wave finite-interaction-length DFWM configuration. It is shown that in the limit of strong pump beams and weak nonlinear coupling, the classical-pumps assumption of Yuen and Shapiro is valid. With use of this assumption, loss in the nonlinear medium is incorporated into the model by coupling the interacting modes to a set of reservoir modes. It is shown that loss presents an absolute limit on the degree of squeezing that can be achieved with DFWM. Also, for comparison with experimental work, the photoelectron statistics of the TP, PC, and 50%-50% combination modes are calculated for lossy DFWM; significant deviations are found from the predictions for lossless operation. Quantum-noise measurements on the PC and TP beams generated in sodiumvapor DFWM are described. The mixer is pumped and probed by the nearly transform-limited pulses produced by a continuous-wave-oscillator-pulse-amplifier chain dye laser at 589 nm wave-length. The normalized second-factorial moment g2{g}_{2}g2​ of the PC and TP beams is determined from photoelectron-counting measurements. Inability to simultaneously achieve high DFWM reflectivity and acceptably low scattered-plus-fluorescent background, coupled with low photomultiplier quantum efficiency, restrict the experiment to a DFWM regime wherein theory predicts Poisson statistics. Experimental g2{g}_{2}g2​ values corroborate this prediction, indicating that systematic and excess noises have been eliminated. No attempt was made to measure the quantum statistics of the 50%-50% combination mode.
A quantum theory of degenerate four-wave mixing is presented in which the atomic medium consists of stationary four-level atoms, each with three degenerate excited states, and the interacting light beams are allowed to be in different states of polarization. This vector-field theory differs from the scalar-field theory of Reid and Walls [Phys. Rev. A 31, 1622 (1985)] in that there are new atomic variables in the Langevin equations which are related to the induced coherence between the upper atomic states. It is found, for the assumed set of atomic levels, that this seemingly different mechanism of four-wave-mixing gain does not circumvent the degrading effect of spontaneous emission on squeezing obtainable via degenerate four-wave mixing. The theory is applied to both forward and backward degenerate four-wave mixing with nearly collinear geometry, and specialized to the case in which the polarization states of the two pump modes are mutually orthogonal. It is found that for both forward and backward configurations, the range of pump intensity for which squeezing can be achieved in the vector-field case is larger than that in the scalar-field case, and the maximum amount of squeezing obtainable at a particular pump detuning is comparable in both cases.