We discuss the characterization of dense elongated clouds of 87 Rb in the context of the process of Bose-Einstein condensation under hydrodynamic conditions. The condensation is induced by shock- cooling of thermal clouds. This gives rise to strong temperature gradients and results in a non-equilibrium shape of the (quasi)condensate with strong phase fluctuations just after formation.
We discuss the characterization of dense elongated clouds of 87 Rb in the context of the process of Bose-Einstein condensation under hydrodynamic conditions. The condensation is induced by shock- cooling of thermal clouds. This gives rise to strong temperature gradients and results in a non-equilibrium shape of the (quasi)condensate with strong phase fluctuations just after formation.
Dilute gas Bose-Einstein condensates are ultracold quantum gases that display many peculiar hydrodynamic properties, such as superfluidity, i.e. dissipation-less flow, a variety of solitonic textures and quantized vortex structures. Small amplitude excitations within a Bose-Einstein condensate are described by the Bogoliubov dispersion, and have been extensively studied in the past. This dissertation extends previous studies by focusing on strong, nonlinear excitations and shock structures generated in elongated Rb-87 Bose-Einstein condensates, elucidating novel dynamics in these quantum systems.\nThis dissertation is separated into two major parts. In the first part, the building and characterization of a new Bose-Einstein condensate apparatus at Washington State University is described. This apparatus has been built to generate ultracold clouds of Rb-87 and, more recently, K-41atoms. A description of the setups for both isotopes are provided. The apparatus reliably produces Bose-Einstein condensates of 7 x 10^5 Rb-87 atoms every 20 seconds.\nIn the second part of this dissertation, three experiments in a channel geometry are described that have been conducted with the new apparatus. In this part of the dissertation, quantum hydrodynamic properties are probed by using time-dependent optical potentials to generate nonlinear excitations and shock structures in an elongated Bose-Einstein condensate. An emergence of viscous-like shock dynamics, unidirectionality of a non-magnetic spin switch device, and the structure of dispersive shock waves in new types of higher order dispersions are observed. The work described in this dissertation establishes a novel platform for studying strong nonlinear effects in ultracold quantum gases.
When a gas of bosonic atoms is cooled sufficiently near to absolute zero, it undergoes a startling transition from a collection of randomly-behaved individual atoms to a phase in which thousands, even millions, of atoms act in collective unison. In this new phase, known as a Bose-Einstein condensate (BEC), the atoms all occupy the exact same quantum mechanical ground state and can be collectively described by a single phase-coherent wavefunction of macroscopic size. But how exactly does this harmonious behaviour arise within a collection of incoherent atoms as their temperature decreases? Does the condensate wavefunction grow from a single central nucleus, or does it emerge simultaneously throughout the system? And how does the situation differ when the gas is cooled suddenly, away from thermodynamic equilibrium? Can non-equilibrium behaviour be inherited by the condensate that forms? In this thesis we aim to answer these and other questions by studying the formation dynamics of Bose-Einstein condensates and the development of phase coherence. The research described herein makes use of several theoretical tools, which we lay out on the workbench in Chapter 2: Semi-classical Hartree-Fock theory provides a mean-field description of a condensate and thermal cloud at equilibrium; Quantum kinetic theory is used to calculate the dynamics of condensate growth into an equilibrium state, from a non-equilibrium thermal cloud; The stochastic projected Gross-Pitaevskii equation (SPGPE) employs a classical-field description to encapsulate the non-equilibrium dynamics of the condensate and low-energy region of the atom cloud, coupled to an equilibrium thermal cloud. This thesis is composed of four principal studies, each constituting a separate chapter.In Chapter 3 we study the formation of a Bose-Einstein condensate in a cigar-shaped 3D harmonic trap, induced by the controlled addition of an attractive ``dimple'' potential along the weak axis in a recent experiment [Garrett et al., Phys. Rev. A 83, 013630 (2011)]. In this manner condensation is induced without cooling due to a localized increase in the phase space density. We perform a quantitative analysis of the thermodynamic transformation in both the sudden and adiabatic regimes for a range of dimple widths and depths. We find good agreement with equilibrium calculations based on self-consistent semi-classical Hartree-Fock theory describing the condensate and thermal cloud. We observe there is an optimal dimple depth that results in a maximum in the condensate fraction. We also study the non-equilibrium dynamics of condensate formation in the sudden turn-on regime, finding good agreement for the observed time dependence of the condensate fraction with calculations based on quantum kinetic theory. In Chapter 4 we study the onset of phase coherence during the formation of a BEC following a sudden quench to below the transition temperature. Using the SPGPE, we simulate a recent experiment performed at ANU in which a sudden RF quench is applied to a dilute gas of metastable Helium atoms confined in an elongated 3D harmonic magnetic trap. At regularly-spaced intervals following the quench, broadband RF pulses are applied to homogeneously outcouple small (<5%) pulses of atoms, which expand and fall to a microchannel plate detector. The second-order correlation function at the detector, postulated to provide a measure of phase coherence of the in-situ cloud from which they were outcoupled, is measured versus time and compared with the condensate growth curve. A delay was observed in the relaxation of the second-order correlation function, relative to the peak in the number of condensate atoms. In our simulations we incorporate the effects of periodic outcoupling both the condensate and thermal cloud, and monitor the time-dependence of first- and second-order correlation functions in both position and momentum space. We observe long-range phase coherence in the final equilibrium state, though mild persistent phase fluctuations are present. We also observe the curious phenomenon of ``superbunching'' - an enhancement of density fluctuations - at specific values of the momentum, which we relate to anomalous correlations of fluctuations. Despite obtaining a good quantitative fit to the experimentally-measured condensate growth curve in our SPGPE simulations, we do not observe any evidence of the delay in coherence observed in the experiment, which remains unexplained. In Chapter 5 we use the SPGPE to study the crossover from a true BEC with long-range phase coherence to a quasicondensate dominated by phase fluctuations, for the case of a Bose gas in an highly-elongated 3D harmonic trap. We use parameters corresponding to an experiment in which a sudden quench resulted in the formation of a non-equilibrium condensate, the dynamics of which we study in the chapter that follows. Sweeping through a range of temperatures and chemical potentials within the crossover region, we reveal the behaviour of phase fluctuations through analysis of correlation functions. We compare the ideal-gas approximation for the transition temperature with the more accurate value obtained via the Binder cumulant. By comparing the phase coherence length with the spatial extent across which density fluctuations are suppressed, we identify the BEC/quasicondensate crossover point. We compare directly with predictions of mean-field theory [Petrov et al., Phys. Rev. Lett. 87, 050404 (2001)] and find that phase fluctuations persist to lower temperatures in our SPGPE simulations. We calculate anomalous correlations of the fluctuation field and show that the resulting correction to the mean-field condensate self-interaction energy is significant within the quasicondensate regime. In Chapter 6 we study the formation of a BEC into a non-equilibrium state by simulating an experiment in which a dilute gas of Rubidium-87 atoms in a highly-elongated 3D harmonic magnetic trap is rapidly quenched to below the transition temperature. Following the quench, a condensate is observed to form with an excessively elongated shape, and subsequently undergo damped quadrupole shape oscillations [Shvarchuck et al., Phys. Rev. Lett. 89, 270404 (2002)]. We simulate this experiment by modifying the SPGPE to incorporate a hydrodynamic thermal cloud, parametrized by axially and temporally-dependent temperature and chemical potential. Comparison against simulations without this axial dependence suggests the hydrodynamic behaviour of the thermal cloud plays a crucial role in the formation of a non-equilibrium condensate. Analyses of the first-order correlation function and the condensate wavefunction reveal the spontaneous formation of quantum vortices, as well as strong phase fluctuations at equilibrium indicating quasicondensate behaviour.
Background 1 1.22This thesis 2 Chapterr 2 Theoretical background 5 2.11 Rubidium 5 2.22 Magnetic trapping 5 2.33 Bose-Einstein condensation 8 2.44 BEC formation and phase coherence 2.55 Evaporative cooling 2.5.11Evaporative cooling Lensing Chapterr 4 Broad-area diode laser system 4.11 Abstract 4.22 Introduction 4.33 Experimental setup 4.44 Characteristics 4.55 MOT application 4.66 Summary Chapterr 5 Hydrodynamic properties of dense atomic clouds Vlll l 5.11 Introduction 5.22 Density and temperature analysis 5.33 Anisotropic expansion of hydrodynamic clouds 5.44 Frequency shifts and damping of shape oscillations Chapterr 6 Condensation into non-equilibrium states and focusing of a condensate 6.11 Introduction 6.22 Preparation of degenerate samples out of equilibrium 6.33 Kinetics of the condensate growth 6.44 Formation of a non-equilibrium BEC 6.4.11Local critical temperature 6.4.22 Truncation and local temperature 6.55 Oscillation modes 6.66 Non-equilibrium phase fluctuations 6.77 Focusing of a condensate 6.7.11Focusing principle 6.7.22 Focal broadening 6.7.33 Applications of BEC focusing 6.88 High condensate fractions in non-equilibrium states Bibliographyy Summaryy Samenvattingg AcknowledgementssMostt of the theoretical groundwork on the interacting quantum gases has been developedd in the 50's and the 60's in the context of superfluidity of 4 He.However, a detailedd comparison between theory and experiment is extremely difficult in the case of liquidd helium because its density is rather high and can be varied only within a narrow range..In the 70's the observation of BEC in dilute atomic gases under equilibrium conditionss was known to be impossible.Therefore, the efforts shifted towards investigationss of metastable systems.Thee first attempts to reach BEC were done in spin-polarised atomic hydrogen.Foundationss for many techniques and methods were laid in the course of that work.Hydrogenn quantum gas was first stabilised in a cryogenic environment by Silvera and Walravenn [93] and by Cline et al. [23].Magnetic trapping was first demonstrated in sodium [79]] and in hydrogen by Hess et al. [50] and van Roijen et al. [87].Another critically importantt technique, evaporative cooling, was first experimentally demonstrated in hydrogenn [51] and further developed in [74,97, 105].Bose-Einsteinn condensation in alkali systems was achieved in magnetic traps throughh the combination of optical cooling methods with the evaporative cooling technique.iss obtained by observation of the anisotropic character of the expansion.Finally, we measuree frequency shifts and damping of shape oscillations.Inn the final part of the Thesis, Chapter 6, we describe the results produced in the experimentss on formation of condensates far from equilibrium.We compare our work with previouss experiments on condensate formation and describe how the process of formation iss triggered in our system.A brief section deals with the growth of the condensate fraction.Further,, we show how the concepts of local sample temperature and the critical temperature arisee in elongated clouds with high elastic collision rates.We present a simple model, whichh illustrates how the non-equilibrium character of the condensates leads to the quadrupolee oscillations.We also discuss non-equilibrium phase fluctuations, which manifestt themselves in the form of stripes in the time-of-flight absorption images.Condensatee focusing is introduced as a novel method for investigation of Bose-Einstein condensates..The focusing of a condensate in free flight arises from axial contraction of the expandingg cloud when the gas is released from the trap during the inward phase of a shape oscillation.. Possible applications of BEC focusing are discussed, with an estimate of the coherencee length given as an example.The last part of the chapter covers condensation into non-equilibriumm states with high condensate fractions.The situations of large and small condensatee fractions are compared.
The field of Bose-Einstein condensation (BEC) in dilute atomic gases provides a fruitful playground to test well-developed theories of quantum fluids. Research using BECs can address open questions relating to the many-body aspects of two-component quantum liquids, namely the interaction between the hydrodynamic normal and the superfluid component at finite temperatures. After the first realization of BEC some pilot experiments have been carried out, but detailed experiments are missing. This has to be compared to the case of liquid helium II, where many experiments since the 1950s have added to our understanding of novel phenomena in quantum liquids, like collective excitations, first and second sound, and others. One of the drawbacks of liquid helium is that the interactions are so strong that a clear distinction between the two components is difficult and the interpretation of the phenomena remains ambiguous. Most experimental studies of dilute Bose-Einstein condensed gases use clouds, which are in the collisionless regime. The reason for the lack of detailed experiments in BECs to study quantum liquids and in particular the hydrodynamical aspects of it, is the limited number of atoms (typically 1--10 million) in the experiments leaving the thermal atoms virtually collisionless. Efforts to decrease the mean free path by increasing the confinement limits the lifetime of the sample, since the density is limited by three-body decay. Experiments on dilute clouds of cold atoms are generally conducted in highly asymmetric traps. In these elongated, cigar-shaped geometries the mean free path of the atoms can become much shorter than the size of the cloud in the long, axial direction, but at the same time exceeds the size in the other, radial directions. In this so-called hydrodynamic-collisionless regime the system can be considered radially collisionless and axially hydrodynamic. In our setup we have created BECs containing up to 300 million sodium atoms by evaporation of atoms in an axially strongly decompressed trap with an aspect ratio of 1:65. Hot atoms created in three-body collisions are able to leave the sample in this highly asymmetric trap, before they can heat other atoms in an avalanche. The sample is axially hydrodynamic, but due to the large aspect ratio collisionless in the radial direction. Such samples are ideal for the observation of the interaction between the superfluid and normal fluid component of the cloud. In this thesis we describe the setup which is used to reach the hydrodynamic regime and we describe a novel implementation of the well-known phase contrast imaging technique. Next, we study collective excitations in the crossover from the collisionless toward the hydrodynamic regime, we determine the heat conduction in a cold, hydrodynamic thermal cloud and observe the propagation of a thermal wave in the two-fluid regime. Furthermore, we study the friction between the superfluid and normal fluid component of the cloud. In the final chapters of this thesis we study the propagation of second sound, as well as the formation and propagation of shock waves.
Collective excitations of a dilute Bose gas were probed above and below the Bose-Einstein condensation temperature. The temperature dependencies of the frequency and damping rates of condensate oscillations indicate significant interactions between the condensate and the thermal cloud. Hydrodynamic oscillations of the thermal cloud analogous to first sound were observed. An out-of-phase dipolar oscillation of the thermal cloud and the condensate was also studied, analogous to second sound. The excitations were observed in situ using nondestructive imaging techniques.
Summary form only given. We have systematically studied BECs of /sup 87/Rb atoms in the regime of phase-fluctuating condensates. We observe the phase fluctuations by measuring the density distribution of the released cloud after ballistic expansion. By varying the temperature, the number of atoms in the condensate and the aspect ratio of the trapping potential, we studied the continuous transition from the usual 3D regime, where phase fluctuations are low, into the regime of strong phase fluctuations in the condensate. To determine the amount of phase fluctuations experimentally, we measured the formation and structure of stripes in the atomic density distribution after ballistic expansion as a function of the above mentioned parameters. The appearance of stripes after switching off the trapping fields can be understood as conversion of phase fluctuations respect. phase gradients into axial velocity fields and consecutive density distributions. These results are in good agreement with theoretical and numerical studies and set clear limitations on applications of BECs e.g. in interferometric measurements.