Background 1 1.22This thesis 2 Chapterr 2 Theoretical background 5 2.11 Rubidium 5 2.22 Magnetic trapping 5 2.33 Bose-Einstein condensation 8 2.44 BEC formation and phase coherence 2.55 Evaporative cooling 2.5.11Evaporative cooling Lensing Chapterr 4 Broad-area diode laser system 4.11 Abstract 4.22 Introduction 4.33 Experimental setup 4.44 Characteristics 4.55 MOT application 4.66 Summary Chapterr 5 Hydrodynamic properties of dense atomic clouds Vlll l 5.11 Introduction 5.22 Density and temperature analysis 5.33 Anisotropic expansion of hydrodynamic clouds 5.44 Frequency shifts and damping of shape oscillations Chapterr 6 Condensation into non-equilibrium states and focusing of a condensate 6.11 Introduction 6.22 Preparation of degenerate samples out of equilibrium 6.33 Kinetics of the condensate growth 6.44 Formation of a non-equilibrium BEC 6.4.11Local critical temperature 6.4.22 Truncation and local temperature 6.55 Oscillation modes 6.66 Non-equilibrium phase fluctuations 6.77 Focusing of a condensate 6.7.11Focusing principle 6.7.22 Focal broadening 6.7.33 Applications of BEC focusing 6.88 High condensate fractions in non-equilibrium states Bibliographyy Summaryy Samenvattingg AcknowledgementssMostt of the theoretical groundwork on the interacting quantum gases has been developedd in the 50's and the 60's in the context of superfluidity of 4 He.However, a detailedd comparison between theory and experiment is extremely difficult in the case of liquidd helium because its density is rather high and can be varied only within a narrow range..In the 70's the observation of BEC in dilute atomic gases under equilibrium conditionss was known to be impossible.Therefore, the efforts shifted towards investigationss of metastable systems.Thee first attempts to reach BEC were done in spin-polarised atomic hydrogen.Foundationss for many techniques and methods were laid in the course of that work.Hydrogenn quantum gas was first stabilised in a cryogenic environment by Silvera and Walravenn [93] and by Cline et al. [23].Magnetic trapping was first demonstrated in sodium [79]] and in hydrogen by Hess et al. [50] and van Roijen et al. [87].Another critically importantt technique, evaporative cooling, was first experimentally demonstrated in hydrogenn [51] and further developed in [74,97, 105].Bose-Einsteinn condensation in alkali systems was achieved in magnetic traps throughh the combination of optical cooling methods with the evaporative cooling technique.iss obtained by observation of the anisotropic character of the expansion.Finally, we measuree frequency shifts and damping of shape oscillations.Inn the final part of the Thesis, Chapter 6, we describe the results produced in the experimentss on formation of condensates far from equilibrium.We compare our work with previouss experiments on condensate formation and describe how the process of formation iss triggered in our system.A brief section deals with the growth of the condensate fraction.Further,, we show how the concepts of local sample temperature and the critical temperature arisee in elongated clouds with high elastic collision rates.We present a simple model, whichh illustrates how the non-equilibrium character of the condensates leads to the quadrupolee oscillations.We also discuss non-equilibrium phase fluctuations, which manifestt themselves in the form of stripes in the time-of-flight absorption images.Condensatee focusing is introduced as a novel method for investigation of Bose-Einstein condensates..The focusing of a condensate in free flight arises from axial contraction of the expandingg cloud when the gas is released from the trap during the inward phase of a shape oscillation.. Possible applications of BEC focusing are discussed, with an estimate of the coherencee length given as an example.The last part of the chapter covers condensation into non-equilibriumm states with high condensate fractions.The situations of large and small condensatee fractions are compared.
Background 1 1.22This thesis 2 Chapterr 2 Theoretical background 5 2.11 Rubidium 5 2.22 Magnetic trapping 5 2.33 Bose-Einstein condensation 8 2.44 BEC formation and phase coherence 2.55 Evaporative cooling 2.5.11Evaporative cooling Lensing Chapterr 4 Broad-area diode laser system 4.11 Abstract 4.22 Introduction 4.33 Experimental setup 4.44 Characteristics 4.55 MOT application 4.66 Summary Chapterr 5 Hydrodynamic properties of dense atomic clouds Vlll l 5.11 Introduction 5.22 Density and temperature analysis 5.33 Anisotropic expansion of hydrodynamic clouds 5.44 Frequency shifts and damping of shape oscillations Chapterr 6 Condensation into non-equilibrium states and focusing of a condensate 6.11 Introduction 6.22 Preparation of degenerate samples out of equilibrium 6.33 Kinetics of the condensate growth 6.44 Formation of a non-equilibrium BEC 6.4.11Local critical temperature 6.4.22 Truncation and local temperature 6.55 Oscillation modes 6.66 Non-equilibrium phase fluctuations 6.77 Focusing of a condensate 6.7.11Focusing principle 6.7.22 Focal broadening 6.7.33 Applications of BEC focusing 6.88 High condensate fractions in non-equilibrium states Bibliographyy Summaryy Samenvattingg AcknowledgementssMostt of the theoretical groundwork on the interacting quantum gases has been developedd in the 50's and the 60's in the context of superfluidity of 4 He.However, a detailedd comparison between theory and experiment is extremely difficult in the case of liquidd helium because its density is rather high and can be varied only within a narrow range..In the 70's the observation of BEC in dilute atomic gases under equilibrium conditionss was known to be impossible.Therefore, the efforts shifted towards investigationss of metastable systems.Thee first attempts to reach BEC were done in spin-polarised atomic hydrogen.Foundationss for many techniques and methods were laid in the course of that work.Hydrogenn quantum gas was first stabilised in a cryogenic environment by Silvera and Walravenn [93] and by Cline et al. [23].Magnetic trapping was first demonstrated in sodium [79]] and in hydrogen by Hess et al. [50] and van Roijen et al. [87].Another critically importantt technique, evaporative cooling, was first experimentally demonstrated in hydrogenn [51] and further developed in [74,97, 105].Bose-Einsteinn condensation in alkali systems was achieved in magnetic traps throughh the combination of optical cooling methods with the evaporative cooling technique.iss obtained by observation of the anisotropic character of the expansion.Finally, we measuree frequency shifts and damping of shape oscillations.Inn the final part of the Thesis, Chapter 6, we describe the results produced in the experimentss on formation of condensates far from equilibrium.We compare our work with previouss experiments on condensate formation and describe how the process of formation iss triggered in our system.A brief section deals with the growth of the condensate fraction.Further,, we show how the concepts of local sample temperature and the critical temperature arisee in elongated clouds with high elastic collision rates.We present a simple model, whichh illustrates how the non-equilibrium character of the condensates leads to the quadrupolee oscillations.We also discuss non-equilibrium phase fluctuations, which manifestt themselves in the form of stripes in the time-of-flight absorption images.Condensatee focusing is introduced as a novel method for investigation of Bose-Einstein condensates..The focusing of a condensate in free flight arises from axial contraction of the expandingg cloud when the gas is released from the trap during the inward phase of a shape oscillation.. Possible applications of BEC focusing are discussed, with an estimate of the coherencee length given as an example.The last part of the chapter covers condensation into non-equilibriumm states with high condensate fractions.The situations of large and small condensatee fractions are compared.
When a gas of bosonic atoms is cooled sufficiently near to absolute zero, it undergoes a startling transition from a collection of randomly-behaved individual atoms to a phase in which thousands, even millions, of atoms act in collective unison. In this new phase, known as a Bose-Einstein condensate (BEC), the atoms all occupy the exact same quantum mechanical ground state and can be collectively described by a single phase-coherent wavefunction of macroscopic size. But how exactly does this harmonious behaviour arise within a collection of incoherent atoms as their temperature decreases? Does the condensate wavefunction grow from a single central nucleus, or does it emerge simultaneously throughout the system? And how does the situation differ when the gas is cooled suddenly, away from thermodynamic equilibrium? Can non-equilibrium behaviour be inherited by the condensate that forms? In this thesis we aim to answer these and other questions by studying the formation dynamics of Bose-Einstein condensates and the development of phase coherence. The research described herein makes use of several theoretical tools, which we lay out on the workbench in Chapter 2: Semi-classical Hartree-Fock theory provides a mean-field description of a condensate and thermal cloud at equilibrium; Quantum kinetic theory is used to calculate the dynamics of condensate growth into an equilibrium state, from a non-equilibrium thermal cloud; The stochastic projected Gross-Pitaevskii equation (SPGPE) employs a classical-field description to encapsulate the non-equilibrium dynamics of the condensate and low-energy region of the atom cloud, coupled to an equilibrium thermal cloud. This thesis is composed of four principal studies, each constituting a separate chapter.In Chapter 3 we study the formation of a Bose-Einstein condensate in a cigar-shaped 3D harmonic trap, induced by the controlled addition of an attractive ``dimple'' potential along the weak axis in a recent experiment [Garrett et al., Phys. Rev. A 83, 013630 (2011)]. In this manner condensation is induced without cooling due to a localized increase in the phase space density. We perform a quantitative analysis of the thermodynamic transformation in both the sudden and adiabatic regimes for a range of dimple widths and depths. We find good agreement with equilibrium calculations based on self-consistent semi-classical Hartree-Fock theory describing the condensate and thermal cloud. We observe there is an optimal dimple depth that results in a maximum in the condensate fraction. We also study the non-equilibrium dynamics of condensate formation in the sudden turn-on regime, finding good agreement for the observed time dependence of the condensate fraction with calculations based on quantum kinetic theory. In Chapter 4 we study the onset of phase coherence during the formation of a BEC following a sudden quench to below the transition temperature. Using the SPGPE, we simulate a recent experiment performed at ANU in which a sudden RF quench is applied to a dilute gas of metastable Helium atoms confined in an elongated 3D harmonic magnetic trap. At regularly-spaced intervals following the quench, broadband RF pulses are applied to homogeneously outcouple small (<5%) pulses of atoms, which expand and fall to a microchannel plate detector. The second-order correlation function at the detector, postulated to provide a measure of phase coherence of the in-situ cloud from which they were outcoupled, is measured versus time and compared with the condensate growth curve. A delay was observed in the relaxation of the second-order correlation function, relative to the peak in the number of condensate atoms. In our simulations we incorporate the effects of periodic outcoupling both the condensate and thermal cloud, and monitor the time-dependence of first- and second-order correlation functions in both position and momentum space. We observe long-range phase coherence in the final equilibrium state, though mild persistent phase fluctuations are present. We also observe the curious phenomenon of ``superbunching'' - an enhancement of density fluctuations - at specific values of the momentum, which we relate to anomalous correlations of fluctuations. Despite obtaining a good quantitative fit to the experimentally-measured condensate growth curve in our SPGPE simulations, we do not observe any evidence of the delay in coherence observed in the experiment, which remains unexplained. In Chapter 5 we use the SPGPE to study the crossover from a true BEC with long-range phase coherence to a quasicondensate dominated by phase fluctuations, for the case of a Bose gas in an highly-elongated 3D harmonic trap. We use parameters corresponding to an experiment in which a sudden quench resulted in the formation of a non-equilibrium condensate, the dynamics of which we study in the chapter that follows. Sweeping through a range of temperatures and chemical potentials within the crossover region, we reveal the behaviour of phase fluctuations through analysis of correlation functions. We compare the ideal-gas approximation for the transition temperature with the more accurate value obtained via the Binder cumulant. By comparing the phase coherence length with the spatial extent across which density fluctuations are suppressed, we identify the BEC/quasicondensate crossover point. We compare directly with predictions of mean-field theory [Petrov et al., Phys. Rev. Lett. 87, 050404 (2001)] and find that phase fluctuations persist to lower temperatures in our SPGPE simulations. We calculate anomalous correlations of the fluctuation field and show that the resulting correction to the mean-field condensate self-interaction energy is significant within the quasicondensate regime. In Chapter 6 we study the formation of a BEC into a non-equilibrium state by simulating an experiment in which a dilute gas of Rubidium-87 atoms in a highly-elongated 3D harmonic magnetic trap is rapidly quenched to below the transition temperature. Following the quench, a condensate is observed to form with an excessively elongated shape, and subsequently undergo damped quadrupole shape oscillations [Shvarchuck et al., Phys. Rev. Lett. 89, 270404 (2002)]. We simulate this experiment by modifying the SPGPE to incorporate a hydrodynamic thermal cloud, parametrized by axially and temporally-dependent temperature and chemical potential. Comparison against simulations without this axial dependence suggests the hydrodynamic behaviour of the thermal cloud plays a crucial role in the formation of a non-equilibrium condensate. Analyses of the first-order correlation function and the condensate wavefunction reveal the spontaneous formation of quantum vortices, as well as strong phase fluctuations at equilibrium indicating quasicondensate behaviour.
The problem of understanding how a coherent, macroscopic Bose- Einstein condensate (BEC) emerges from the cooling of a thermal Bose gas has attracted significant theoretical and experimental interest over several decades. The pioneering achievement of BEC in weakly interacting dilute atomic gases in 1995 was followed by a number of experimental studies examining the growth of the BEC number, as well as the development of its coherence. More recently, there has been interest in connecting such experiments to universal aspects of nonequilibrium phase transitions, in terms of both static and dynamical critical exponents. Here, the spontaneous formation of topological structures such as vortices and solitons in quenched cold-atom experiments has enabled the verification of the Kibble-Zurek mechanism predicting the density of topological defects in continuous phase transitions, first proposed in the context of the evolution of the early universe. This chapter reviews progress in the understanding of BEC formation and discusses open questions and future research directions in the dynamics of phase transitions in quantum gases. Introduction The equilibrium phase diagram of the dilute Bose gas exhibits a continuous phase transition between condensed and noncondensed phases. The order parameter characteristic of the condensed phase vanishes above some critical temperature T c and grows continuously with decreasing temperature below this critical point. However, the dynamical process of condensate formation has proved to be a challenging phenomenon to address both theoretically and experimentally. This formation process is a crucial aspect of Bose systems and of direct relevance to all condensates discussed in this book, despite their evident system-specific properties. Important questions leading to intense discussions in the early literature include the time scale for condensate formation and the role of inhomogeneities and finite-size effects in “closed” systems. These issues are related to the concept of spontaneous symmetry breaking, its causes, and implications for physical systems (see, for example, Chapter 5 by Snoke and Daley). In this chapter, we give an overview of the dynamics of condensate formation and describe the present understanding provided by increasingly well-controlled cold-atom experiments and corresponding theoretical advances over the past twenty years. We focus on the growth of BECs in cooled Bose gases, which, from a theoretical standpoint, requires a suitable nonequilibrium formalism.
In 1925, Einstein predicted the condensation of bosons into the ground state of the system for low (but finite) temperatures. Several phenomena, including superfluidity and superconductivity have been associated with Bose-Einstein condensation, but these systems interact strongly with their environment and pure Bose-Einstein condensation could not be established. It took 70 years, in which time the laser was discovered, and laser cooling techniques to manipulate atoms in a dilute atomic gas, before Bose-Einstein condensation in dilute atomic gases could be demonstrated in 1995. In the first condensation experiments, BECs were created in a magnetic trap. Since in a magnetic trap not all mF states of the atom can be trapped simultaneously, thereby limiting the number of experiments that can be done, other ways of trapping and generating BECs were sought and found. In 2001, the first all-optical BEC was made, where the dipole force was used to trap atoms in the crossing of two far red detuned laser beams. In an optical dipole trap not only atoms in different internal states can be trapped, but also different atomic species simultaneously. In this thesis, the formation of an all-optical Bose-Einstein condensate with rubidium atoms is presented. Conventional all-optical BECs are usually created in high power CO2 laser dipole traps, or have complicated laser cooling schemes and complex dipole trap setups. In our simple and straightforward setup, we load rubidium atoms from a magneto-optical trap into a crossed optical dipole trap created by a single frequency Yb:YAG laser with a wavelength at 1030 nm. The small wavelength allows for a small diffraction limit, and permits us to use standard optical materials, thus making the experimental setup cost effective. Other attempts to achieve Bose-Einstein condensation in a multi-mode (frequency) fiber laser at 1064 nm failed, because the atom loss was quite high. It is assumed that the multi-mode character of the fiber laser induces Raman transitions in rubidium atoms, thereby heating them. We can trap about ∼ 5E7 atoms in a single beam dipole trap out of ∼ 5E9 atoms trapped in theMOT, and ∼ 350,000 atoms can be trapped in a crossed beam dipole trap due to the smaller trap volume. 70% of the atoms in the dipole trap is optically pumped into one mF state. Quantum degeneracy is reached by evaporatively cooling the atoms in the crossed dipole trap by ramping down the laser power with three linear ramps. We can independently change the power of each beam by an AOM. This allows us to use one beam as an atom waveguide for future experiments. After evaporation, we typically have about 10,000 atoms at a temperature below the critical temperature. We have proved Bose-Einstein condensation by using the anisotropic expansion of a quantum degenerate gas trapped in an anisotropic potential. The aspect ratio of our atom cloud changed during a time of flight from 0.7 to 1.2 in 10 ms, thus proving that we have reached quantum degeneracy. We have about 5,000 condensed atoms in our optical dipole trap at a temperature less than 100 nK. The remaining atoms are thermal. Bose-Einstein condensation is obtained within 8 s, and we can repeat the experiment every 30 s. It should be mentioned that the Bose-Einstein experiment was moved from the ”Leibniz Universität Hannover” to the ”Technische Universität Darmstadt”, and had to be completely rebuilt. All-optical Bose-Einstein condensation was reached within one year after the move. Our Bose-Einstein condensation setup presents an ideal starting point for using our condensates in combination with miniaturized atom optical setups based on our novel microfabricated optical elements. With our microlenses, we can create a number of possible dipole trap configurations, such as the dipole trap array or the cylindrical microlens array. Using microlenses in miniaturized atom optical setups opens a completely new field of coherent atom optics. Also because the tight confinement of the microtraps allows us to load a 3D BEC, a 1D BEC, or a Tonks-Girardeau gas in the micropotentials depending on the density.
Quantum systems consisting of many particles are both interesting from the physics and the mathematics perspective. One aspect that makes them fascinating from the physics point of view is that they can exhibit quantum effects on macroscopic scales such as Bose-Einstein condensation. This phenomenon, first predicted 100 years ago by Bose [19] and Einstein [44], occurs when a dilute gas of bosons is cooled down to very low temperatures. Below a certain critical temperature a condensate forms, meaning that a macroscopic fraction of the particles is in the same one-particle state, and thus, quantum phenomena become relevant on length scales much larger than the individual atom. The occurrence of Bose-Einstein condensation is also related to superfluidity as suggested in [88]. Bose-Einstein condensation has been achieved experimentally independently by the groups of Cornell and Wieman [3] and Ketterle [40] earning them a Nobel prize in 2001. While Bose and Einstein analyzed theoretically the non-interacting gas, an effective theory describing weakly interacting Bose gases was proposed by Bogoliubov in 1947 with the goal of explaining the occurrence of superfluidity in liquid helium [18]. Using assumptions such as that condensation indeed occurs, his theory yields predictions for the low-energy states of the system. Seen from the mathematics perspective, describing the Bose gas is an interesting challenge due to the strong correlations between particles introduced by the interaction making this case much harder to study than the non-interacting one. In particular, a proof that Bose-Einstein condensation occurs in the thermodynamic limit for continuous systems is still out of reach. However, there has been a lot of work regarding the rigorous analysis of bosonic systems in various relevant regimes. This thesis contains three new contributions establishing rigorous results on bosonic systems in different, physically relevant settings. It is based on the articles [37, 27, 31]. The first result concerns the time-evolution of initially trapped Bose gases in the ultra-dilute Gross-Pitaevskii regime. Under some assumptions on the initial data satisfied in particular by a class of states that are expected to approximate the ground state in a trap, we derive a quasi-free approximation that is close to the true solution in L2-norm. In particular, we show that this approximate wave function is described in terms of a Bose-Einstein condensate in a one-particle state following the time-dependent Gross-Pitaevskii equation together with pair excitations with respect to this condensate. As a corollary, we establish a central limit theorem for bounded one-particle observables. The second result is a simple proof of Bose-Einstein condensation for interacting, ultra-dilute gases. More specifically, we consider scalings interpolating between the Gross-Pitaevskii regime and the thermodynamic limit. While condensation had been shown to hold in these regimes before, the advantage of the method used here is its simplicity. Lastly, the third result establishes an upper bound on the ground state energy of a dilute Bose gas in the thermodynamic limit. It captures rigorously the third order correction to the energy per unit volume for sufficiently low densities as predicted in the physics literature first by Wu and subsequently others. Full-text embargoed until: 2026-01-01
In this Thesis we study steady state solutions and dynamical evolutions of two– component atomic Bose–Einstein Condensates. We initially investigate the equilibrium properties of condensate mixtures in harmonic trapping potentials at zero temperature. Subsequently we simulate the coupled growth of these condensates by inclusion of damping terms. Finally, we investigate the evolution of coupled Bose gases via the so-called classical–field method. A recent experiment [D. J. McCarron et al., Phys. Rev. A, 84, 011603(R) (2011)] achieved Bose–Einstein Condensation of a two–species 87Rb–133Cs phase segregated mixture in harmonic trapping potentials. Depending on relative atom numbers of the two species, three distinct regimes of density distributions were observed. For these experimental parameters, we investigate the corresponding time–independent ground state solutions through numerical simulations of the coupled Gross–Pitaevskii equations. By including experimentally relevant shifts between the traps, we observe a range of structures including ‘ball and shell’ formations and axially/radially separated states. These are found to be very sensitive to the trap shifts. For all three experimental regimes, our numerical simulations reveal good qualitative agreement. The observed experimental profiles cannot be guaranteed to be fully equilibrated. This, coupled with the rapid sympathetic cooling of the experimental system, leads to a situation where growth may play a determining factor in the density structures formed. To investigate this further, we introduce phenomenological damping to describe the associated condensate growth/decay, revealing a range of transient structures. However, such a model always predicts the predominance of one condensate species over longer evolution times. Work undertaken by collaborators with the more elaborate Stochastic Projected Gross–Pitaevskii equations, which can describe condensate formation by coupling to a heat bath, predicts the spontaneous formation of dark–bright solitons. Motivated by this, we show how the presence of solitons can affect the condensate distribution, thus highlighting the overall dynamical role in the emerging patterns. Finally, we use classical field methods to analyse the evolution of non trapped Bose gases from strongly nonequilibrium initial distributions. The contrast between miscible (overlapping) and immiscible (phase segregated) components gives rise to important distinctions for condensate fractions and the formation of domains and vortices. In addition, splitting the particles of a single component thermalised state into two components is investigated. We then study the effects of suddenly quenching the strength of the interspecies interactions. Under suitable conditions, this quench generates isotropic vortex tangles. While this tangle subsequently decays over time, we propose how a repeat sequence of quenches at regular intervals could be employed to drive the tangle, thereby potentially providing a novel route to the generation of quantum turbulence.
This thesis features fundamental experiments on the coherence properties of Bose-Einstein condensates (BEC) and atom lasers, made possible by a newly developed apparatus combining a Bose-Einstein condensate with an ultrahigh nesse optical cavity.Using the cavity as a single atom detector, atoms extracted from a trapped cloud are detected with unprecedented sensitivity, and the rst time-resolved counting of single atoms from a quantum degenerate source was demonstrated.O-diagonal long-range order is a dening property of a BEC and equivalent to longrange phase coherence.Its formation is a complex process accompanied by spontaneous symmetry breaking.We witnessed this formation in an ultracold cloud of 87 Rb atoms crossing the phase transition of BEC.Two overlapping atomic beams originating from dierent positions inside the condensate propagated downwards into the cavity.They showed a matter wave interference pattern with a visibility determined by the coherence of the probed regions.The modulation of the ux of atoms, recorded with single-atom resolution, yields the visibility, whereas its mean value gives information about the density of the sample.By shock cooling, a cloud of atoms was prepared in a highly nonequilibrium state slightly above the phase transition.While the ensemble subsequently relaxed, it crossed the phase transition into an equilibrium with a small condensate fraction.Employing our minimally invasive measurement method, the growth of both the rst-order coherence and the density of the sample was tracked in real time while the system crossed the phase transition.The growth of the coherence was found to start later, proceed faster and nish earlier than the increase in density.The coherent region increased at one fth of the speed of sound.Employing time-resolved single atom counting with the cavity detector, the full counting statistics of an atom laser beam was recorded.In a Hanbury Brown and Twiss type experiment, the second-order correlation function was found to be constant g (2) (τ ) = 1.00±0.01,proving the atom laser's second-order coherence and the absence of excess intensity uctuations that were observed in a pseudothermal beam.An analysis of the time interval distributions of atoms in the beam conrmed these ndings.The iii