We have studied quantum entanglement generation using nonlinear interaction of slowly propagating quantum field in a solid medium. Due to enhanced nonlinearity based on electromagnetically induced transparency and standing light phenomenon, a reversible nondegenerate four-wave mixing processing results in quantum entanglement generation. Our attention is to determine nonlinear perspectives of the entanglement with single photon fields. To accomplish the quantum entanglement based on the slow light involved standing light scheme, non-Doppler broadening has been required, where multiple atomic coherences have been the basis in a time-reversed manner. This study is potential for nonlinear optics application to quantum information science such as quantum computing and quantum memories using macroscopic optical medium.
We have studied quantum entanglement generation using nonlinear interaction of slowly propagating quantum field in a solid medium. Due to enhanced nonlinearity based on electromagnetically induced transparency and standing light phenomenon, a reversible nondegenerate four-wave mixing processing results in quantum entanglement generation. Our attention is to determine nonlinear perspectives of the entanglement with single photon fields. To accomplish the quantum entanglement based on the slow light involved standing light scheme, non-Doppler broadening has been required, where multiple atomic coherences have been the basis in a time-reversed manner. This study is potential for nonlinear optics application to quantum information science such as quantum computing and quantum memories using macroscopic optical medium.
Summary form only given. Exciting observations of ultra-slow group velocities and very large nonlinearities in coherently driven atomic media open up interesting prospectives for nonlinear optical processes at low light levels. Recent experiments, for instance, demonstrated that very efficient nonlinear phenomena can be induced by laser fields of tiny energies. These developments stimulate the studies of ultimate efficiency limits for nonlinear optics based on electromagnetically induced transparency (EIT) as well as its possible applications for generation and manipulation of quantum entangled states of the light fields and matter. We describe a particular method that allows for two slow light fields of energies corresponding to that of a single photon to interact coherently.
Generating nonclassical light offers a benchmark tool for fundamental research and potential applications in quantum optics. Conventionally, it has become a standard technique to produce nonclassical light through the nonlinear optical processes occurring in nonlinear crystals. We describe this process using cold atomic-gas media to generate such nonclassical light, especially focusing on narrowband biphoton generation. Compared with the standard procedure the new biphoton source has such properties as long coherence time, long coherence length, high spectral brightness, and high conversion efficiency. Although there exist two methodologies describing the physical process, we concentrate on the theoretical aspect of the entangled two-photon state produced from the four-wave mixing in a multilevel atomic ensemble using perturbation theory. We show that both linear and nonlinear optical responses to the generated fields play an important role in determining the biphoton waveform and, consequently, on the two-photon temporal correlation. There are two characteristic regimes determined by whether the linear or nonlinear coherence time is dominant. In addition, our model provides a clear physical picture that brings insight into understanding biphoton optics with this new source. We apply our model to recent work on generating narrowband (and even subnatural linewidth) paired photons using the technique of electromagnetically induced transparency and slow-light effect in cold atoms and find good agreement with experimental results.
Coherent preparation by laser light of quantum states of atoms and molecules can lead to quantum interference in the amplitudes of optical transitions. In this way the optical properties of a medium can be dramatically modified, leading to electromagnetically induced transparency and related effects, which have placed gas-phase systems at the center of recent advances in the development of media with radically new optical properties. This article reviews these advances and the new possibilities they offer for nonlinear optics and quantum information science. As a basis for the theory of electromagnetically induced transparency the authors consider the atomic dynamics and the optical response of the medium to a continuous-wave laser. They then discuss pulse propagation and the adiabatic evolution of field-coupled states and show how coherently prepared media can be used to improve frequency conversion in nonlinear optical mixing experiments. The extension of these concepts to very weak optical fields in the few-photon limit is then examined. The review concludes with a discussion of future prospects and potential new applications.
Quantum entanglement has been an extremely active field of research, both theoretically and experimentally. Studies on entanglement are fundamental to improving our basic understanding of quantum mechanics. As our understanding of the phenomenon grows, so does interest in using it to advance various technological fields: communications, computing, and sensing, to name just a few. It is now known that entangled photon pairs can be generated through a process known as Spontaneous Four-Wave Mixing (SFWM). In this paper, we report the generation of entangled photon pairs in time intervals by spontaneous four-wave mixing in a nonlinear fiber optic ring resonator. The requirements for efficient SFWM are quite similar to those for classical FWM, but they require even greater precision, especially for quantum applications. To achieve a measurable pair generation rate, a high-intensity pump laser is essential. The nonlinear medium must have high nonlinearity and confinement. This technique is compatible with contemporary fiber, enabling compact, low-cost, and scalable implementations such as quantum memories.
The fields of quantum and nonlinear optics have given rise to a variety of nonclassical states of light that have been proven to surpass certain limitations set by classical physics. Namely, certain squeezed and entangled states have been shown to beat the shot-noise limit when making precision phase measurements in interferometry, as well as write lithographic patterns that are smaller than classically allowed by the Rayleigh diffraction limit. Additionally, single-photon sources and entangled photon pairs have given rise to provably secure quantum key distribution for cryptography. Producing these quantum states of light has proven a difficult task. Nonlinear crystals, when pumped by a laser, produce pairs of single photons via the process of spontaneous parametric down conversion (SPDC). This process is mediated by the second order nonlinear susceptibility of the material. When pumped in a high gain regime, these crystals give rise to optical parametric amplification, which is a viable source of squeezed light. The vast majority of research in this area has focused on crystals that are seeded by vacuum in their two modes. This dissertation concerns the field of quantum nonlinear optics. It is an investigation into the processes that occur when nonlinear materials interact with the electromagnetic field on the single photon level. I have focused on seeding nonlinear crystals with quantum states of light, including single photons and entangled states. This process results in various states directly applicable to interferometry, imaging, and cryptography. Another application investigated is an absolute radiance measurement via stimulated parametric down conversion resulting from non-vacuum seeding of a nonlinear crystal. Additionally, other nonlinear processes, including four-wave mixing, nonlinear magneto-optical effects and coherent population trapping in warm atomic vapor involving quantum states of light are investigated. The process of seeding third-order nonlinear interactions, such as in atomic vapors, gives rise to a variety of interesting, nonclassical phenomena such as entangled image transfer and nonlocal imaging. Strong analogies between SPDC and four-wave mixing are drawn. I also experimentally show an all optical pi-only phase shift of one light beam via another in warm Cesium vapor.
The recent prospect of efficient, reliable, and secure quantum communication relies on the ability to coherently and reversibly map nonclassical states of light onto long-lived atomic states. A promising technique that accomplishes this employs Electromagnetically Induced Transparency (EIT), in which a strong classical control field modifies the optical properties of a weak signal field in such a way that a previously opaque medium becomes transparent to the signal field. The accompanying steep dispersion in the index of refraction allows for pulses of light to be decelerated, then stored as an atomic excitation, and later retrieved as a photonic mode. This dissertation presents the results of investigations into methods for optimizing the memory efficiency of this process in an ensemble of hot Rb atoms. We have experimentally demonstrated the effectiveness of two protocols for yielding the best memory efficiency possible at a given atomic density. Improving memory efficiency requires operation at higher optical depths, where undesired effects such as four-wave mixing (FWM) become enhanced and can spontaneously produce a new optical mode (Stokes field). We present the results of experimental and theoretical investigations of the FWM-EIT interaction under continuous-wave (cw), slow light, and stored light conditions. In particular, we provide evidence that indicates that while a Stokes field is generated upon retrieval of the signal field, any information originally encoded in a seeded Stokes field is not independently preserved during the storage process. We present a simple model that describes the propagation dynamics and provides an intuitive description of the EIT-FWM process.