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Nano Letters

One-by-One Coupling of Single Defect Centers in Nanodiamonds to High-Q Modes of an Optical Microresonator

Stefan Schietinger, Tim Schröder, Oliver J. Benson

Published Sep 24, 2008• 135 citations
Publisher

Abstract

In this letter, we present the on-demand coupling of single NV(-) defect centers in nanodiamonds to a polystyrene microspherical resonator. From an ensemble on a coverslip, we select single nanodiamonds containing a single defect proven by a pronounced antibunching dip. With the help of a scanning near-field probe, we can attach these nanodiamonds to a microsphere resonator one-by-one. A clearly modulated fluorescence spectrum demonstrates coupling of the single defect centers to high-Q whispering-gallery modes. Our experiments establish a toolbox to assemble complex systems consisting of single quantum emitters and (coupled) microresonators.

DOI
10.1021/nl8023627

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We present the on-demand coupling of single NV- defect centers in nanodiamonds to a polystyrene microspherical resonator. From an ensemble on a coverslip we select out single nanodiamonds containing a single defect proven by a pronounced antibunching dip. With the help of a scanning near-field probe we can attach these nanodiamonds to a microsphere resonator one-by-one. A clearly modulated fluorescence spectrum demonstrates coupling of the single defect centers to high- whispering-allery modes. Our experiments establish a toolbox to assemble complex systems consisting of single quantum emitters and (coupled) microresonators.

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Coupling nitrogen vacancy centers in diamond nanopillars to whispering gallery microresonators

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Applied Physics Letters•Oct 12, 2009•36 citations
In this letter, we present the on-demand coupling of single NV(-) defect centers in nanodiamonds to a polystyrene microspherical resonator. From an ensemble on a coverslip, we select single nanodiamonds containing a single defect proven by a pronounced antibunching dip. With the help of a scanning near-field probe, we can attach these nanodiamonds to a microsphere resonator one-by-one. A clearly modulated fluorescence spectrum demonstrates coupling of the single defect centers to high-Q whispering-gallery modes. Our experiments establish a toolbox to assemble complex systems consisting of single quantum emitters and (coupled) microresonators.
We present the on-demand coupling of single NV- defect centers in nanodiamonds to a polystyrene microspherical resonator. From an ensemble on a coverslip we select out single nanodiamonds containing a single defect proven by a pronounced antibunching dip. With the help of a scanning near-field probe we can attach these nanodiamonds to a microsphere resonator one-by-one. A clearly modulated fluorescence spectrum demonstrates coupling of the single defect centers to high- whispering-allery modes. Our experiments establish a toolbox to assemble complex systems consisting of single quantum emitters and (coupled) microresonators.
In this paper, we report the controlled coupling of fluorescence from a single NV-centre in a single nanodiamond to the high-Q modes of a preselected microsphere. Microspheres from an ensemble with a finite size distribution can be characterized precisely via white light Mie-scattering. The mode spectrum of individual spheres can be determined with high precision. A sphere with an appropriate spectrum can be selected, and a nanodiamond containing a single NV-centre can be coupled to it. The spectral position of the calculated lowest order whispering gallery modes are found to be in very good agreement with the experimentally observed resonances of the coupled fluorescence from the single NV-centre.
For cavity quantum electrodynamics systems (cavity-QED) to play a role in quantum information processing applications and in quantum networks, they must be robust and scalable in addition to having a suitable method for the generation, processing and storage of quantum bits. One solution is to develop a composite system that couples a nitrogen vacancy (NV) center in diamond to a whispering gallery mode supported by a fused silica microsphere. Such a system is motivated by the optical and electron-spin properties of the NV center. The NV center is the leading spin-qubit and exhibits atomic like linewidths at cryogenic temperatures and has spin coherence times greater than milliseconds at room temperature. These long coherence times, coupled with nanosecond scale spin readout and manipulation times, allow for millions of quantum operations to be processed. Silica whispering gallery resonators are the only class of microresonators with quality factor high enough to reach the strong coupling regime, which is necessary for some quantum information processing applications. \n \nIntegrating these two components into a system that could position a diamond nanopillar near the surface of a deformed-double stemmed microsphere system, with nanometer precision, at 10 K was a major achievement of this research. Cavity resonances in deformed microspheres can be excited with a free-space coupling technique which simplifies their integration into cryogenic environments. In these intentionally deformed resonators, an enhanced evanescent field decay length was observed at specific locations along the ray orbit. The double-stem arrangement enables the cavity resonance to be tuned over 450 GHz, with sub-10 MHz resolution, at 10 K. These two features, the enhanced decay length and broad range tuning with high resolution, are indispensible tools for cavity-QED studies with silica microspheres. \n \nDiamond nanopillars were fabricated from single crystal diamond with diameters as small as 140 nm in order to maintain a high quality factor. Studies were conducted on NV centers in nanopillars and bulk diamond to determine their suitability for cavity-QED applications. In an attempt to increase the light-matter interaction between NV centers and whispering gallery modes, diamond substrates were optically characterized that were irradiated with nitrogen ions.
We have developed a technique for creating high quality tellurite microspheres with embedded nanodiamonds (NDs) containing nitrogen-vacancy (NV) centres. This hybrid method allows fluorescence of the NVs in the NDs to be directly, rather than evanescently, coupled to the whispering gallery modes of the tellurite microspheres at room temperature. As a demonstration of its sensing potential, shifting of the resonance peaks is also demonstrated by coating a sphere surface with a liquid layer. This new approach is a robust way of creating cavities for use in quantum and sensing applications.
We theoretically investigate a cavity quantum electrodynamics system in which a high-QQQ whispering-gallery-mode (WGM) microresonator interacts with multiple diamond nanocrystals each containing a single nitrogen-vacancy (NV) center. With a tapered fiber waveguide coupling the WGMs, the transmission spectrum of the system exhibits a twofold-splitting phenomenon, where the first fold of splitting originates from the nanocrystals' Rayleigh scattering and the second fold stems from the NV center dipole coupling with the WGMs. The interacting system can serve as a platform to generate quantum entanglement between two NV centers embedded in distant diamond nanocrystals. Our further study reveals that the Rayleigh scattering of the nanocrystals plays a positive role in generating entanglement in some cases. The analytical results show that the relatively strong scattering leads to a larger concurrence for the fixed dipole-cavity detunings. This investigation may hold potential for solid-state quantum information processing applications.
The coupling of a quantum emitter to the modes of a silica toroid is presented. A fiber taper is used to manipulate and transfer a preselected diamond nanocrystal onto the toroid. Optical coupling of few nitrogen vacancy (NV) color centers contained inside the nanocrystal to the resonator modes is demonstrated by detecting the fluorescence via a tapered optical fiber coupler. A clear antibunching in the photon correlation measurement is observed indicating emission from only six NV centers residing inside the nanocrystal. The latter is confirmed by a photoluminescence spectrum at liquid helium temperature resolving individual zero phonon lines.