Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Journal of Physics B Atomic Molecular and Optical Physics

Coupling single NV-centres to high-Qwhispering gallery modes of a preselected frequency-matched microresonator

Stefan Schietinger, Oliver J. Benson

Published May 15, 2009• 31 citations
Publisher

Abstract

In this paper, we report the controlled coupling of fluorescence from a single NV-centre in a single nanodiamond to the high-Q modes of a preselected microsphere. Microspheres from an ensemble with a finite size distribution can be characterized precisely via white light Mie-scattering. The mode spectrum of individual spheres can be determined with high precision. A sphere with an appropriate spectrum can be selected, and a nanodiamond containing a single NV-centre can be coupled to it. The spectral position of the calculated lowest order whispering gallery modes are found to be in very good agreement with the experimentally observed resonances of the coupled fluorescence from the single NV-centre.

DOI
10.1088/0953-4075/42/11/114001

Related papers

One-by-One Coupling of Single Defect Centers in Nanodiamonds to High-Q Modes of an Optical Microresonator

Stefan Schietinger, Tim Schröder, Oliver J. Benson

In this letter, we present the on-demand coupling of single NV(-) defect centers in nanodiamonds to a polystyrene microspherical resonator. From an ensemble on a coverslip, we select single nanodiamonds containing a single defect proven by a pronounced antibunching dip. With the help of a scanning near-field probe, we can attach these nanodiamonds to a microsphere resonator one-by-one. A clearly modulated fluorescence spectrum demonstrates coupling of the single defect centers to high-Q whispering-gallery modes. Our experiments establish a toolbox to assemble complex systems consisting of single quantum emitters and (coupled) microresonators.

Nano Letters•Sep 24, 2008•135 citations

One-by-one coupling of single photon emitters to high-Q modes of optical microresonators

Stefan Schietinger, Tim Schröder, Oliver J. Benson

We present the on-demand coupling of single NV- defect centers in nanodiamonds to a polystyrene microspherical resonator. From an ensemble on a coverslip we select out single nanodiamonds containing a single defect proven by a pronounced antibunching dip. With the help of a scanning near-field probe we can attach these nanodiamonds to a microsphere resonator one-by-one. A clearly modulated fluorescence spectrum demonstrates coupling of the single defect centers to high- whispering-allery modes. Our experiments establish a toolbox to assemble complex systems consisting of single quantum emitters and (coupled) microresonators.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Feb 12, 2009•1 citation

Atom–Photon Coupling from Nitrogen-vacancy Centres Embedded in Tellurite Microspheres

Yinlan Ruan, Brant C. Gibson, Desmond W. M. Lau +6 more

We have developed a technique for creating high quality tellurite microspheres with embedded nanodiamonds (NDs) containing nitrogen-vacancy (NV) centres. This hybrid method allows fluorescence of the NVs in the NDs to be directly, rather than evanescently, coupled to the whispering gallery modes of the tellurite microspheres at room temperature. As a demonstration of its sensing potential, shifting of the resonance peaks is also demonstrated by coating a sphere surface with a liquid layer. This new approach is a robust way of creating cavities for use in quantum and sensing applications.

Scientific Reports•Jun 22, 2015•10 citations

Coupling nitrogen vacancy centers in diamond nanopillars to whispering gallery microresonators

Khodadad N. Dinyari

For cavity quantum electrodynamics systems (cavity-QED) to play a role in quantum information processing applications and in quantum networks, they must be robust and scalable in addition to having a suitable method for the generation, processing and storage of quantum bits. One solution is to develop a composite system that couples a nitrogen vacancy (NV) center in diamond to a whispering gallery mode supported by a fused silica microsphere. Such a system is motivated by the optical and electron-spin properties of the NV center. The NV center is the leading spin-qubit and exhibits atomic like linewidths at cryogenic temperatures and has spin coherence times greater than milliseconds at room temperature. These long coherence times, coupled with nanosecond scale spin readout and manipulation times, allow for millions of quantum operations to be processed. Silica whispering gallery resonators are the only class of microresonators with quality factor high enough to reach the strong coupling regime, which is necessary for some quantum information processing applications. \n \nIntegrating these two components into a system that could position a diamond nanopillar near the surface of a deformed-double stemmed microsphere system, with nanometer precision, at 10 K was a major achievement of this research. Cavity resonances in deformed microspheres can be excited with a free-space coupling technique which simplifies their integration into cryogenic environments. In these intentionally deformed resonators, an enhanced evanescent field decay length was observed at specific locations along the ray orbit. The double-stem arrangement enables the cavity resonance to be tuned over 450 GHz, with sub-10 MHz resolution, at 10 K. These two features, the enhanced decay length and broad range tuning with high resolution, are indispensible tools for cavity-QED studies with silica microspheres. \n \nDiamond nanopillars were fabricated from single crystal diamond with diameters as small as 140 nm in order to maintain a high quality factor. Studies were conducted on NV centers in nanopillars and bulk diamond to determine their suitability for cavity-QED applications. In an attempt to increase the light-matter interaction between NV centers and whispering gallery modes, diamond substrates were optically characterized that were irradiated with nitrogen ions.

•Jan 1, 2012•0 citations

Achieving maximum entanglement between two nitrogen-vacancy centers coupling to a whispering-gallery-mode microresonator

Siping Liu, Jiahua Li, Rong Yu +1 more

We investigate the entanglement generation between two nitrogen-vacancy (NV) centers in diamond nanocrystal coupled to a high-Q counterpropagating twin whispering-gallery modes (WGMs) of a microtoroidal resonator. For looking into the degree and dynamics of the entanglement, we calculate the concurrence using the microscopic master equation approach. The influences of the coupling strength between the WGMs (or the size of the two spherical NV centers), the distance between two NV centers, the frequency detuning between the NV center and microresonator, and the initial state of the system on the dynamics of concurrence are discussed in detail. It is found that the maximum entanglement between the two NV centers can be created by properly adjusting these controllable system parameters. Our results may provide further insight into future solid-state cavity quantum electrodynamics (CQED) system for quantum information engineering.

Optics Express•Feb 4, 2013•26 citations

Coupling of a single nitrogen vacancy colour centre in diamond, to a planar microcavity

Yannick Dumeige, Romain Alléaume, Philippe Grangier +2 more

Single negatively charged nitrogen-vacancy (NV-) defect centres in diamond are attractive systems for the implementation of solid state quantum information processing (QIP) and quantum key distribution (QKD). In both approaches, the coupling of an individual NV-centre to a resonant microcavity is of interest: it would improve the optical readout of the NV-centre electron spin state in QIP and enhance the collection efficiency of the single photon fluorescence in QKD while increasing the coherence length of the emission. We theoretically demonstrate that, at room temperature, the coupling to a single-mode Fabry-Perot microcavity can be used to obtain a fluorescence spectrum narrowing without loss of total intensity. We also experimentally demonstrate the control of the fluorescence spectrum of a single NV-centre by adjusting the thickness of the microcavity. Finally, we report a doubling of the emission spectral density with respect to the single mirror configuration.

International Conference on Transparent Optical Networks•Jun 1, 2011•1 citation
In this paper, we report the controlled coupling of fluorescence from a single NV-centre in a single nanodiamond to the high-Q modes of a preselected microsphere. Microspheres from an ensemble with a finite size distribution can be characterized precisely via white light Mie-scattering. The mode spectrum of individual spheres can be determined with high precision. A sphere with an appropriate spectrum can be selected, and a nanodiamond containing a single NV-centre can be coupled to it. The spectral position of the calculated lowest order whispering gallery modes are found to be in very good agreement with the experimentally observed resonances of the coupled fluorescence from the single NV-centre.
In this letter, we present the on-demand coupling of single NV(-) defect centers in nanodiamonds to a polystyrene microspherical resonator. From an ensemble on a coverslip, we select single nanodiamonds containing a single defect proven by a pronounced antibunching dip. With the help of a scanning near-field probe, we can attach these nanodiamonds to a microsphere resonator one-by-one. A clearly modulated fluorescence spectrum demonstrates coupling of the single defect centers to high-Q whispering-gallery modes. Our experiments establish a toolbox to assemble complex systems consisting of single quantum emitters and (coupled) microresonators.
We present the on-demand coupling of single NV- defect centers in nanodiamonds to a polystyrene microspherical resonator. From an ensemble on a coverslip we select out single nanodiamonds containing a single defect proven by a pronounced antibunching dip. With the help of a scanning near-field probe we can attach these nanodiamonds to a microsphere resonator one-by-one. A clearly modulated fluorescence spectrum demonstrates coupling of the single defect centers to high- whispering-allery modes. Our experiments establish a toolbox to assemble complex systems consisting of single quantum emitters and (coupled) microresonators.
We have developed a technique for creating high quality tellurite microspheres with embedded nanodiamonds (NDs) containing nitrogen-vacancy (NV) centres. This hybrid method allows fluorescence of the NVs in the NDs to be directly, rather than evanescently, coupled to the whispering gallery modes of the tellurite microspheres at room temperature. As a demonstration of its sensing potential, shifting of the resonance peaks is also demonstrated by coating a sphere surface with a liquid layer. This new approach is a robust way of creating cavities for use in quantum and sensing applications.
For cavity quantum electrodynamics systems (cavity-QED) to play a role in quantum information processing applications and in quantum networks, they must be robust and scalable in addition to having a suitable method for the generation, processing and storage of quantum bits. One solution is to develop a composite system that couples a nitrogen vacancy (NV) center in diamond to a whispering gallery mode supported by a fused silica microsphere. Such a system is motivated by the optical and electron-spin properties of the NV center. The NV center is the leading spin-qubit and exhibits atomic like linewidths at cryogenic temperatures and has spin coherence times greater than milliseconds at room temperature. These long coherence times, coupled with nanosecond scale spin readout and manipulation times, allow for millions of quantum operations to be processed. Silica whispering gallery resonators are the only class of microresonators with quality factor high enough to reach the strong coupling regime, which is necessary for some quantum information processing applications. \n \nIntegrating these two components into a system that could position a diamond nanopillar near the surface of a deformed-double stemmed microsphere system, with nanometer precision, at 10 K was a major achievement of this research. Cavity resonances in deformed microspheres can be excited with a free-space coupling technique which simplifies their integration into cryogenic environments. In these intentionally deformed resonators, an enhanced evanescent field decay length was observed at specific locations along the ray orbit. The double-stem arrangement enables the cavity resonance to be tuned over 450 GHz, with sub-10 MHz resolution, at 10 K. These two features, the enhanced decay length and broad range tuning with high resolution, are indispensible tools for cavity-QED studies with silica microspheres. \n \nDiamond nanopillars were fabricated from single crystal diamond with diameters as small as 140 nm in order to maintain a high quality factor. Studies were conducted on NV centers in nanopillars and bulk diamond to determine their suitability for cavity-QED applications. In an attempt to increase the light-matter interaction between NV centers and whispering gallery modes, diamond substrates were optically characterized that were irradiated with nitrogen ions.
We investigate the entanglement generation between two nitrogen-vacancy (NV) centers in diamond nanocrystal coupled to a high-Q counterpropagating twin whispering-gallery modes (WGMs) of a microtoroidal resonator. For looking into the degree and dynamics of the entanglement, we calculate the concurrence using the microscopic master equation approach. The influences of the coupling strength between the WGMs (or the size of the two spherical NV centers), the distance between two NV centers, the frequency detuning between the NV center and microresonator, and the initial state of the system on the dynamics of concurrence are discussed in detail. It is found that the maximum entanglement between the two NV centers can be created by properly adjusting these controllable system parameters. Our results may provide further insight into future solid-state cavity quantum electrodynamics (CQED) system for quantum information engineering.
Single negatively charged nitrogen-vacancy (NV-) defect centres in diamond are attractive systems for the implementation of solid state quantum information processing (QIP) and quantum key distribution (QKD). In both approaches, the coupling of an individual NV-centre to a resonant microcavity is of interest: it would improve the optical readout of the NV-centre electron spin state in QIP and enhance the collection efficiency of the single photon fluorescence in QKD while increasing the coherence length of the emission. We theoretically demonstrate that, at room temperature, the coupling to a single-mode Fabry-Perot microcavity can be used to obtain a fluorescence spectrum narrowing without loss of total intensity. We also experimentally demonstrate the control of the fluorescence spectrum of a single NV-centre by adjusting the thickness of the microcavity. Finally, we report a doubling of the emission spectral density with respect to the single mirror configuration.