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Journal of the Optical Society of America B

Persistent spectral hole burning in an organic material for temporal pattern recognition

Ming Tian, F. Grelet, I. Lorgeré, Jean‐Pierre Galaup, J.-L. Le Gouët

Published Jan 1, 1999• 18 citations
Publisher

Abstract

A broad-bandwidth persistent spectral hole-burning organic material is used as a fast optical processor that compares an input temporal-frequency profile with a recorded reference spectral shape. This pattern-recognition procedure relies on a subpicosecond temporal cross-correlation process. The size of the phase-encoding spectral interval exceeds 1 THz. The storage material, the spectral encoder, and the interferometric detector are examined in detail for optimal pattern discrimination. Experimental temporal pattern-recognition results are reported.

DOI
10.1364/josab.16.000074

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A broad-bandwidth persistent spectral hole-burning organic material is used as a fast optical processor that compares an input temporal-frequency profile with a recorded reference spectral shape. This pattern-recognition procedure relies on a subpicosecond temporal cross-correlation process. The size of the phase-encoding spectral interval exceeds 1 THz. The storage material, the spectral encoder, and the interferometric detector are examined in detail for optimal pattern discrimination. Experimental temporal pattern-recognition results are reported.
Spectral hole burning (SHB) allows to extend conventional spatial-domain optical data storage and coherent processing into the dimensions of frequency and time. To achieve ultrafast performance, on the time scale of 10-12 - 10-13s, we use organic dye-doped polymer materials at liquid-helium temperature. These materials enable SHB recording and coherent transient responses with a broad optical band width of 5 - 10 THz. We discuss applications of organic SHB systems for associative recall of time-and-space domain events, spectral programming of pulse trains, Stark switching of holograms, THz-bit-rate multiplication, cross- spectral processing and photon gated recording of erasure resistant coherent transients.
In previous investigations of optical data storage in persistent spectral-hole-burning materials, either the spectral or the temporal positions of the data were used as memory addresses. We suggest having the address represented by the spectral shape of the writing field and retrieving information with the aid of pattern recognition of this spectral shape. This procedure is expected to accelerate access to the stored data. To evaluate the validity of the method, we consider various physical effects that may give rise to cross talk among the different addresses. A numerical simulation under realistic conditions is presented.
The persistent spectral hole-burning (PSHB) phenomenon has been known since 1974. It is still an important research area for the study of the intimacy of complex molecular systems in the solid state, revealing high-resolution spectra, photophysics, photochemistry, and dynamics of molecular doped amorphous media, organic as well as inorganic. From another point of view, PSHB allows the engraving of any spectral structures in the inhomogeneous absorption band profile of molecular doped amorphous hosts or ion doped crystals cooled down to liquid helium temperatures. Therefore, a PSHB material is programmable in the spectral domain and consequently it can be transformed in an optical processor capable of achieving user-defined optical functions. Some aspects of both fields are illustrated in the present paper. Concerning the search for efficient PSHB materials, the hole-burning performances and the photophysics of polymer and xerogel based systems are compared. The problem of high-temperature persistent spectral hole-burning materials and the search for new frequency selective photosensitive systems for fast optical pulse processing at 800nm are considered. Regarding the points treated, inorganic hosts based on silicate xerogels or porous glasses have shown the best results. Moreover, by combining inorganic and organic capabilities or by grafting organic species to the host, hybrid xerogels have not yet revealed all possibilities. Also, the interest of two-photon materials for engraving spectral features with near-infrared or infrared light is developed. As an introduction to possible applications of PSHB material, the basics of spectro-temporal holography are remembered and a demonstrative experiment using a naphthalocyanine-doped polymer film is described, proving that the temporal aberration free recompression of ultrashort light pulses is feasible, therefore opening a way for applications in ultrashort light pulse shaping. Aspects for a comparison between cw hole-burning and femtosecond spectro-temporal experiments are considered, and prospects for coherent control of light fields or photochemical processes are also evoked.
We study theoretically and experimentally the synthesis of arbitrary time-domain pulse shapes, using short laser pulses scattered by holograms stored in a spectrally selective hole-burning material. In general, writing holograms in spectrally selective materials results in cross talk and interference between different frequencies because of Kramers–Kronig dispersion relations. We discuss different ways to exclude the cross talk that disturbs faithful reproduction of the desired time-domain pulse shapes. In particular, we show that one can exclude the cross talk by writing holograms in a way that simulates a time-domain offset of the object pulse. To confirm our theoretical considerations we carry out experiments by writing persistent spectral hole-burning holograms with a tunable dye laser in an organic dye–polymer system at low temperature. By reading out the time-domain response with subpicosecond white-light pulses we demonstrate the feasibility of spectral synthesis of light pulses with complicated amplitude and phase properties on the time scale of hundreds of picoseconds with a subpicosecond time resolution.