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Russian Journal of Physical Chemistry B

Superradiant transition and its classical analogue

Margarita A. Kovaleva, L. I. Manevich

Published Sep 1, 2013• 6 citations
Publisher

Abstract

The two-level quantum model proposed by Preparata, according to which the interaction of a material system with a electromagnetic field can cause the loss of stability of the lower level, is examined. As a result of this instability, the role of the ground state is played by a periodic process generating superradiance (in contrast to laser radiation induced by overpopulation of the upper level). A classical analogue of a super-radiant quantum transition, a system of van der Pol-Duffing oscillators (generators) weakly coupled via a linear oscillator, is for the first time described. Such an analogue is a strongly modulated oscillatory process of almost complete periodic energy exchange between the generators. It is shown that a necessary condition for the transition to intense energy exchange in the classical system is the instability of one of the nonlinear normal modes, similar to how the condition for a superradiant transition to occur is the instability of the ground state of a two-level quantum system coupled with a resonant electromagnetic field.

DOI
10.1134/s1990793113050291

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The two-level quantum model proposed by Preparata, according to which the interaction of a material system with a electromagnetic field can cause the loss of stability of the lower level, is examined. As a result of this instability, the role of the ground state is played by a periodic process generating superradiance (in contrast to laser radiation induced by overpopulation of the upper level). A classical analogue of a super-radiant quantum transition, a system of van der Pol-Duffing oscillators (generators) weakly coupled via a linear oscillator, is for the first time described. Such an analogue is a strongly modulated oscillatory process of almost complete periodic energy exchange between the generators. It is shown that a necessary condition for the transition to intense energy exchange in the classical system is the instability of one of the nonlinear normal modes, similar to how the condition for a superradiant transition to occur is the instability of the ground state of a two-level quantum system coupled with a resonant electromagnetic field.
The paper discusses the similarity between dissipative generation and superradiance regimes for systems of excited quantum emitters placed in an open cavity. In the case of the existence of a resonator field due to reflections from the ends of the system, a dissipative generation regime is usually realized. In this case, the decrement of oscillations in the waveguide in the absence of radiators turns out to be greater than the increment of the arising instability of the system of radiators placed in the resonator. When describing this mode, the influence of the emitters on each other and the sum of their own fields is neglected. The resonator field forces the oscillators to emit or absorb quanta synchronously with it, depending on the local value of the population inversion. Lasing takes on a weakly oscillatory character due to an asynchronous change in the population inversion of the system of emitting dipoles (nutations), which have a ground and excited energy levels. To describe the process, the equations of the semiclassical theory based on the use of the density matrix are quite sufficient. In the case when there is no resonator or waveguide field, taking into account the eigenfields of the oscillators becomes essential. To simulate the superradiance process, large emitting particles are used, to describe which one should use the equations for the density matrix. It is shown that the interaction of quantum emitters in this case is due to electromagnetic fields under conditions when the overlap of their wave functions is insignificant. Equations are obtained that allow considering the process of interaction of emitters. When the emitters interact, an integral field is formed in the resonator, an increase in the intensity of which leads to synchronization of the emitters. It is shown that the characteristic times of the development of the process, as well as the attainable amplitudes of the excited fields for dissipative regimes of generation and regimes of superradiance of emitters filling an open resonator, are comparable.
Based on the analysis of the experimental data on the observation of the fluorescence and superradiance of praseodymium ions in a matrix of lanthanum trifluoride, a model of superradiance of three-level radiators with two close upper levels is developed in the mean-field approximation and studied. The uppermost level is coherently pumped by an ultrashort pulse of electromagnetic field, after which the excitation is transferred to the close energy level, from which the superradiance transition occurs to the lower level. In limiting cases, the considered model is reduced to the known models of superradiance and describes the ordinary regimes of monopulse and multipulse (oscillatory) superradiance. However, in a certain region of parameters, the model under discussion describes such a multipulse superradiance signal in which electromagnetic field spikes composing it follow in time with random intervals and amplitudes, so that the regime of regular chaotic dynamics is demonstrated in a single superradiance signal. In a certain time interval, the proposed model can be described by the Lorenz equations with the parameters corresponding to the chaotic dynamics of spikes composing the superradiance signal. The presented results of the numerical simulation of the model equations qualitatively correspond to the picture of stochastic pulsations observed experimentally.
The transition to the super-radiant regime in the Dicke model of two-level atoms interacting with a one-mode radiation field has been argued to be impossible for many years. Recently, however, experimental results show that this transition is possible in an open system [1, 2]. Here we exhibit the power of the use of coherent states with restored symmetry to describe the superradiant regime of the Dicke Hamiltonian. These symmetry-adapted states allow for an analytic description of both the ground and first excited states. From these, analytical expressions for all expectation values of interest are obtained, valid for any number of atoms. All these results are exact in the thermodynamic limit.
Several modifications of the Maxwell–Bloch equations are presented for analyzing the emission characteristics of pulsed lasers. The analysis is performed under the condition of coherent interaction between light and a gain medium with resonant phase nonlinearity. For the first time, the interrelated factors of instability of the phase relationship of the light field and the response of the medium, caused by the dipole-dipole interaction and the contribution of quasi-resonant polarization, are taken into account. To describe the superradiance (SR) regime, semi-analytical expressions for the response variables in the Bloch vector formalism are refined. Various approximations of the original model are represented by systems of kinetic equations for the field and response variables of the medium, as well as a nonlinear oscillatory equation for the polar angle of the Bloch vector. Modeling of the coherent SR effect in a resonator showed that the temporal structure of SR is extremely sensitive to the resonant nonlinearity of the material response. It is shown that under nonlinear conditions, the typical nutational intensity structure of synchrotron radiation is transformed into a contrasting quasi-periodic modulation of the trailing edge of the main pulse in the subpicosecond range. A computational analysis of the synchrotron radiation process in a resonator is performed for the parameters of semiconductor quantum dot systems in nanoheterostructures. Such systems are considered promising for use in compact optical electronics and photonics devices.
The problems of phase synchronization in an ensemble of oscillators or dipoles, and the mechanisms of coherent field generation in superradiance mode, are discussed. It is shown that an increase in the spread of the initial amplitudes of an ensemble of oscillators suppresses their phase synchronization and reduces the efficiency of field generation. The influence of noise is discussed; it is shown that, below the generation threshold, even an external initiating field cannot synchronize the phases of an ensemble of particles. When the generation threshold is exceeded, the initiating field may not be required. It is shown that the convergence of the oscillator phases with the field phases at the locations of moving oscillators is noticeable only near their exit from the system. At the same time, a complete coincidence of the phases of synchronized oscillators and the field phases in the region of their localization is not observed. Nevertheless, the intensity of the generation field in the superradiance mode significantly exceeds the spontaneous level, which allows us to speak about the signs of induced radiation. The features of the development of the quantum process of superradiance of an ensemble of dipoles are discussed, and a system of equations for its description is given. The features of the quantum analog of superradiance are qualitatively modeled, and the role of the Rabi frequency determining the dynamics of the population inversion is noted. The nutation of the population inversion in the region occupied by the field affect the field intensity not only in this local zone, but also in subsequent regions of the active zone. This explains the unusual nature of the generation development: the field growth in a certain region of the active zone first stabilizes and then decreases significantly. This decrease in intensity also occurs in the direction of radiation in the peripheral regions of the active zone, despite the large energy reserve in them in the form of unperturbed population inversion.
The semiclassical theory of light-matter interactions describes the interaction between a classical electromagnetic field with a quantum mechanical two-level system.We show that the quantum mechanical two-level system can be modeled by a system of two coupled classical harmonic oscillators whose eigenstates are split in frequency according to the coupling strength and play the roles of the two levels of the quantum mechanical two-level system. The effect of the light field on the mechanical system is modeled as a modulation of the spring constants of the individual oscillators. Using this fully classical model, we derive the Bloch equations for a two-level system and discuss the mechanical analogues of Rabi oscillations and coherent control experiments