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Optics and Spectroscopy

Model of stochastization of the oscillatory regime of superradiance

Ashat M. Basharov, N. V. Znamenskiı̆, A. Yu. Shashkov

Published Feb 1, 2008• 1 citation
Publisher

Abstract

Based on the analysis of the experimental data on the observation of the fluorescence and superradiance of praseodymium ions in a matrix of lanthanum trifluoride, a model of superradiance of three-level radiators with two close upper levels is developed in the mean-field approximation and studied. The uppermost level is coherently pumped by an ultrashort pulse of electromagnetic field, after which the excitation is transferred to the close energy level, from which the superradiance transition occurs to the lower level. In limiting cases, the considered model is reduced to the known models of superradiance and describes the ordinary regimes of monopulse and multipulse (oscillatory) superradiance. However, in a certain region of parameters, the model under discussion describes such a multipulse superradiance signal in which electromagnetic field spikes composing it follow in time with random intervals and amplitudes, so that the regime of regular chaotic dynamics is demonstrated in a single superradiance signal. In a certain time interval, the proposed model can be described by the Lorenz equations with the parameters corresponding to the chaotic dynamics of spikes composing the superradiance signal. The presented results of the numerical simulation of the model equations qualitatively correspond to the picture of stochastic pulsations observed experimentally.

DOI
10.1134/s0030400x08020161

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Based on the analysis of the experimental data on the observation of the fluorescence and superradiance of praseodymium ions in a matrix of lanthanum trifluoride, a model of superradiance of three-level radiators with two close upper levels is developed in the mean-field approximation and studied. The uppermost level is coherently pumped by an ultrashort pulse of electromagnetic field, after which the excitation is transferred to the close energy level, from which the superradiance transition occurs to the lower level. In limiting cases, the considered model is reduced to the known models of superradiance and describes the ordinary regimes of monopulse and multipulse (oscillatory) superradiance. However, in a certain region of parameters, the model under discussion describes such a multipulse superradiance signal in which electromagnetic field spikes composing it follow in time with random intervals and amplitudes, so that the regime of regular chaotic dynamics is demonstrated in a single superradiance signal. In a certain time interval, the proposed model can be described by the Lorenz equations with the parameters corresponding to the chaotic dynamics of spikes composing the superradiance signal. The presented results of the numerical simulation of the model equations qualitatively correspond to the picture of stochastic pulsations observed experimentally.
Experimental data and theoretical model describing stochastic pulsations within oscillatory mode of superradiant emission from the LaF3 medium doped with impurity praseodymium ions are presented. The model deals with three-level system with close upper levels and reflects our experimental data on fluorescence of praseodymium ions. The mean-field approximation is used to develop the superradiance theory. In determined case basic equations of the developed model are reduced to well known Lorenz equations of deterministic chaotic dynamics.
A new effect has been observed in the superradiance of praseodymium ions in a lanthanum trifluoride matrix: the effect of selecting transverse pumping structures upon the oblique-incidence pumping of superradiant media. A simple explanation for this effect is given. The possible reasons for the stochastization of the oscillatory regime of superradiance, a phenomenon observed upon both the normal and oblique incidence of pumping radiation on a crystal and when the crystal is placed in a resonator with an eigenfrequency close to the frequency of the superradiant transition, are analyzed.
Experimental results and a theoretical model describing superradiance of praseodymium ions in the trifluoro lanthanum matrix at the 3 P 0 — 3 H 6 transition upon coherent excitation of the adjacent 3 H 4 — 3 P 0 transition are presented. It is found that when a superradiant medium is placed into a resonator, whose eigenfrequency is close to the superradiant transition ( 3 P 0 — 3 H 6 ) frequency, the superradiant pulse duration decreases and its modulation appears, which is independent of the resonator length. It is shown that these properties are qualitatively described within the framework of the mean-field model of coherent radiation of superradiant media in a resonator.
The two-level quantum model proposed by Preparata, according to which the interaction of a material system with a electromagnetic field can cause the loss of stability of the lower level, is examined. As a result of this instability, the role of the ground state is played by a periodic process generating superradiance (in contrast to laser radiation induced by overpopulation of the upper level). A classical analogue of a super-radiant quantum transition, a system of van der Pol-Duffing oscillators (generators) weakly coupled via a linear oscillator, is for the first time described. Such an analogue is a strongly modulated oscillatory process of almost complete periodic energy exchange between the generators. It is shown that a necessary condition for the transition to intense energy exchange in the classical system is the instability of one of the nonlinear normal modes, similar to how the condition for a superradiant transition to occur is the instability of the ground state of a two-level quantum system coupled with a resonant electromagnetic field.
The possibility of realizing the superradiant regime of electromagnetic emission by the assembly of quantum dots is considered. The overall dynamical process is analyzed in detail. It is shown that there can occur several qualitatively different stages of evolution. The process starts with dipolar waves triggering the spontaneous radiation of individual dots. This corresponds to the fluctuation stage, when the dots are not yet noticeably correlated with each other. The second is the quantum stage, when the dot interactions through the common radiation field become more important, but the coherence is not yet developed. The third is the coherent stage, when the dots radiate coherently, emitting a superradiant pulse. After the superradiant pulse, the system of dots relaxes to an incoherent state in the relaxation stage. If there is no external permanent pumping, or the effective dot interactions are weak, the system tends to a stationary state during the last stationary stage, when coherence dies out to a low, practically negligible, level. In the case of permanent pumping, there exists the sixth stage of pulsing superradiance, when the system of dots emits separate coherent pulses.
Under analysis is the influence of the local field upon the competition of transitions in the process of superradiance from incompletely excited thin layer of three level atoms ((Lambda) -diagram of the operating transitions). It is highlighted that while the upper sublevel of the lower doublet starts degenerating, there is a superradiant regime, where the combinative transition leads the development of the superradiance pulse, and the time of the pulse delay depends on the parameters of the local field and splitting of the lower doublet.