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Frontiers in Optics

Raman Scattering for Quantum Technologies

Duncan G. England, Philip J. Bustard, J. Nunn, Benjamin Sussman

Published Jan 1, 2013• 0 citations
Publisher

Abstract

Quantum mechanics has remained one of the most fascinating topics in physics ever since it was first formalized by the Copenhagen interpretation in the 1920’s. While much of the early experimental work focused on verification of quantum mechanical theory, focus has now shifted towards utilizing the remarkable features of quantum mechanics in emerging quantum technologies. For example, the evolution of complex quantum-mechanical systems could be used to perform calculations beyond the capability of classical computers and the inherent randomness involved in making measurements on a quantum state provides a source of unbreakable cryptographic keys for secure communications. In this talk, we introduce a high-speed quantum random number generator based on integrated photonics, and a high-bandwidth quantum memory for light; we will discuss the impact of these technologies on long-distance quantum communication and local photonic quantum processing.

DOI
10.1364/ls.2013.lw1g.3

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Quantum mechanics has remained one of the most fascinating topics in physics ever since it was first formalized by the Copenhagen interpretation in the 1920’s. While much of the early experimental work focused on verification of quantum mechanical theory, focus has now shifted towards utilizing the remarkable features of quantum mechanics in emerging quantum technologies. For example, the evolution of complex quantum-mechanical systems could be used to perform calculations beyond the capability of classical computers and the inherent randomness involved in making measurements on a quantum state provides a source of unbreakable cryptographic keys for secure communications. In this talk, we introduce a high-speed quantum random number generator based on integrated photonics, and a high-bandwidth quantum memory for light; we will discuss the impact of these technologies on long-distance quantum communication and local photonic quantum processing.
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This thesis is divided into five parts, each with an accompanying publication. In Chapter 1, I motivate the broad scientific pursuit that underlies this thesis: the quest to build universal, fault-tolerant technology that operates on the principles of quantum mechanics and quantum information theory. I motivate the use of single photons as the quantum particles of choice for this task, and I describe the open challenges facing the field of researchers embarking on this quest. This motivation pervades each subsequent chapter of this thesis, which focus in turn on overcoming four distinct technological and scientific hurdles related to these open challenges. The first of these open challenges is to demonstrate experimentally a useful single-photon source. This source of single photons ought to release just one photon at a time, in an on-demand fashion, with high-rate, low-latency, and high quantum-state purity and indistinguishability, in a single spatial mode, at the right wavelengths for a given application, and ought to satisfy certain practical constraints on size, weight, power, and sensitivity to environmental noise and perturbation. This is a long list of performance metrics, some of which are orthogonal, some not, and non-trivial tradeoffs often exist between metrics. While in this thesis we do not present a solution to this general open problem, we modestly expand scientific knowledge of one of the fundamental mechanisms behind single-photon generation. In particular, we present a new formalism for describing the quantum properties of spontaneous Stokes scattering in the Raman interaction, and we probe its effects on the quantum state purity of resulting Stokes photons both experimentally and theoretically. This is the focus of Chapter 2. Another open challenge to universal, fault-tolerant photonic quantum processing is the experimental demonstration of a useful photonic quantum memory—a device that is capable of storing and releasing single photons in a quantum-information-conserving manner, and which possesses sufficiently high performance across, again, a large set of non-orthogonal metrics. On this challenge, we have made several substantial contributions. Chapter 3 describes a novel approach to optimizing the efficiency of photonic quantum memories in atomic ensembles possessing a three-level Lambda-type energy level structure, in an experimentally friendly fashion. Chapter 4 discusses the practical side of implementing robust quantum memory in these atomic systems, where we carefully consider the theoretical sensitivity of these systems to experimental noise and perturbation. These two Chapters lead up to the experimental work described in Chapter 5, where we experimentally demonstrate a state-of-the-art and best-in-class photonic quantum memory in neutral barium vapor that possesses simultaneously high efficiency, broad bandwidth, and low noise. Our experimental demonstration features >95% storage efficiency, at roughly 3 orders of magnitude larger bandwidth (higher speed) than the previous state of the art, as well as record-low noise for Lambda-type atomic memories. The noise is so low, and the bandwidth so large, that we are able to perform a novel characterization experiment to extract the temporal amplitude and phase of the photons retrieved from our memory, based on spectral interferometry with a known reference. This is the most demanding possible characterization of one of these memories, and has direct implications for using this type of memory in quantum processing tasks that require temporally indistinguishable photons. In Chapter 6 I do the requisite summing up of the thesis, and discuss ongoing and future work on the memory project. In the various and sundry appendices I include information that will chiefly be useful for my successors in the lab, but may be of passing interest to other readers.
The impact of quantum technology will be profound and far-reaching: secure communication networks for consumers, corporations and government; precision sensors for biomedical technology and environmental monitoring; quantum simulators for the design of new materials, pharmaceuticals and clean energy devices; and ultra-powerful quantum computers for addressing otherwise impossibly large datasets for machine learning and artificial intelligence applications. However, engineering quantum systems and controlling them is an immense technological challenge: they are inherently fragile; and information extracted from a quantum system necessarily disturbs the system itself. Of the various approaches to quantum technologies, photons are particularly appealing for their low-noise properties and ease of manipulation at the single qubit level. We have developed an integrated waveguide approach to photonic quantum circuits for high performance, miniaturization and scalability. We will described our latest progress in generating, manipulating and interacting single photons in waveguide circuits on silicon chips.
The inherent uncertainty in quantum mechanics offers a source of true randomness which can be used to produce unbreakable cryptographic keys. We discuss the development of a high-speed random number generator based on the quantum phase fluctuations in spontaneously initiated stimulated Raman scattering (SISRS). We utilize the tight confinement and long interaction length available in a Potassium Titanyl Phosphate waveguide to generate highly efficient SISRS using nanojoule pulse energies, reducing the high pump power requirements of the previous approaches. We measure the random phase of the Stokes output using a simple interferometric setup to yield quantum random numbers at 145 Mbps.
The impact of quantum technology will be profound and far-reaching: secure communication networks for consumers, corporations and government; precision sensors for biomedical technology and environmental monitoring; quantum simulators for the design of new materials, pharmaceuticals and clean energy devices; and ultra-powerful quantum computers for addressing otherwise impossibly large datasets for machine learning and artificial intelligence applications. However, engineering quantum systems and controlling them is an immense technological challenge: they are inherently fragile; and information extracted from a quantum system necessarily disturbs the system itself. Of the various approaches to quantum technologies, photons are particularly appealing for their low-noise properties and ease of manipulation at the single qubit level. We have developed an integrated waveguide approach to photonic quantum circuits for high performance, miniaturization and scalability. We will described our latest progress in generating, manipulating and interacting single photons in waveguide circuits on silicon chips.
Quantum key distribution (QKD) relies on the fundamental principles of quantum mechanics and can theoretically achieve unconditionally secure communication that is provable by information theory. Quantum random number generators, on the other hand, utilize the inherent randomness of quantum phenomena and are capable of generating a truly random entropy source that is unpredictable, unbiased and unrepeatable. These two technologies are crucial for building highly trustworthy and secure communication systems resistant to quantum attacks. However, their large-scale deployment still faces challenges such as system performance optimization, cost control and scale production. Relying on wafer-level fabrication platforms and micro-nanometer processing, integrated photonics technology integrates the core devices of traditional QKD systems (e.g., light source, modulator, and detector) in a single chip at high density. It significantly improves the miniaturization, operational stability and cost-effectiveness of the system, and enhances the intrinsic security, and becomes a key enabling platform to drive QKD and QRNG from laboratory to engineering applications. In this paper, we systematically review the recent breakthroughs of photonic integrated QKD based on different material platforms (SOI/InP/TFLN/Si3N4) in terms of core metrics, such as transmission distance and key rate, as well as the significant breakthroughs of integrated QRNG in terms of random number generation rate and system integration. Finally, the future development direction of this field is discussed and outlooked from the four dimensions of practical security of QKD systems, on-chip implementation of cutting-edge QKD protocols, practical fully-integrated QKD systems, and synergistic optimization of high performance and high integration of integrated QRNG.