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Journal of the Physical Society of Japan

Modification of Atomicg-Factor by the Oscillating rf Field

T. Yabuzaki, Noriaki Tsukada, Toru Ogawa

Published Apr 1, 1972• 22 citations
Publisher

Abstract

Behavior of the optically pumped atoms in the oscillating rf field is analized classically in terms of the macroscopic magnetization, in the case that the static magnetic field has components both parallel and perpendicular to the rf field. The theory predicts that the g -factor is modified by the rf field when the Hanle effect and the parametric resonance take place, and that the effect makes its appearance in the variation of width and maxima of lines of the Hanle effect and the parametric resonance. The modification of the g -factor is also derived by the quantum mechanical treatment. The theoretical predictions are quantitatively verified by the experiments with cesium vapor.

DOI
10.1143/jpsj.32.1069

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Behavior of the optically pumped atoms in the oscillating rf field is analized classically in terms of the macroscopic magnetization, in the case that the static magnetic field has components both parallel and perpendicular to the rf field. The theory predicts that the g -factor is modified by the rf field when the Hanle effect and the parametric resonance take place, and that the effect makes its appearance in the variation of width and maxima of lines of the Hanle effect and the parametric resonance. The modification of the g -factor is also derived by the quantum mechanical treatment. The theoretical predictions are quantitatively verified by the experiments with cesium vapor.
By means of the dressed atom concept examined theoretically by Cohen-Tannoudji and Haroche, the misalignment effects of an oscillating rf-field in optical-rf double resonances are investigated. We present a fully quantum mechanical calculation of higher-order effects in the frequency shifts of new coherence resonance for the general case that a spin-1/2 atom interacts with the oscillating rf-field in optical-pumping. It is analytically shown that the new type resonances can occur even by taking account of higher-order effects in the perturbation theory for the oscillating rf-field whose direction makes a special angle from that of a static field, and that the direction of the shift of the resonance field is not along that of the static field but perpendicular to that of the oscillating field. Theoretical results are compared with optical-pumping experiments of cesium vapor.
A theoretical and experimental study has been made of the effect of transverse optical pumping in the optical-rf double resonance of cesium atoms. The solution of Bloch type equations shows that the Hanle effect and new type resonances become notable in the weak magnetic field or for strong rf field, as the effect of the transverse pumping. The new type resonances appear in the unmodulated component and the components modulated at the first and the second harmonics of the applied rf frequency in the pumping light beam transmitted through the sample cell. It is predicted that the new type resonances are not only shifted but also broadened as the intensity of rf field increases. The shift, broadening and the intensity for observed new type resonances are in good agreement with the theoretical prediction.
The evolution of magnetization of optically pumped atoms in the presence of two rotating rf fields with different frequencies is investigated by using the phenomenological Bloch equation. It is shown that the new type resonances, which are due to the effect of the transverse pumping, together with the ordinary magnetic resonance and the multiple quantum transitions are realized under these conditions. It is also shown that the Hanle curve is broadened by a rotating rf field in the same manner as by an oscillating rf field, and is shifted towards high field region as the intensity of the rotating rf field is increased. The results obtained are, in general, applicable to the case of an elliptically rotating rf field, which is superposition of two rotating rf fields.
Energies of the coupled system of a spin-1/2 atom in a static magnetic field and an oscillating rf field are analyzed with the resolvent formalism and numerically calculated by quantizing the rf field, for the general case that the strong rf field is oriented in an arbitrary direction to the static magnetic field. It is shown that, if the component of the static field along the direction of the rf field has particular values, level crossings take place and multiphoton transitions by even or odd numbers of rf photons become forbidden, even when the polarization of the rf field satisfies the parity condition for the multiphoton transitions. Particular attention is given to the direction and amount of the shifts of the level crossings by the rf field, together with the shifts of the anticrossings or of the multiphoton transitions. Theoretical results are verified by the optical-pumping experiments with cesium vapor.
We present an experimental and theoretical analysis of the mechanical Hanle effect, i.e., the modification of the atomic trajectories following the interaction with laser fields in the Hanle configuration. The case of open transitions is examined. In our experiment a thermal sodium atomic beam is crossed perpendicularly by a single-mode linearly polarized laser beam. The laser field is tuned to resonance with an F g F e transition of the sodium D 1 line. A static magnetic field B is applied collinear to the laser light propagation direction. The atomic beam flux at the position corresponding to its maximum in the absence of laser light is studied as a function of the applied magnetic field. For the F g = F F e = F , F -1 transitions the atomic flux shows a sharp increase at B = 0, as a result of the coherent trapping of the population into the ground state. For the F g = 1 F e = 2 transition this effect is absent and no significant variation of the atomic flux with the magnetic field is observed. A theoretical description of the mechanical Hanle effect in open transitions is given and it is clarified why in our experiment the mechanical Hanle/CPT-resonances associated to different hyperfine transitions have different contrasts.