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Soviet Journal of Quantum Electronics

Role of quasienergy levels in the processes of amplification of light by stimulated emission of radiation

R. N. Shakhmuratov

Published Feb 28, 1986• 1 citation
Publisher

Abstract

A theoretical study is made of the influence of changes in the relaxation of a three-level system in a resonance field on the dispersion, absorption, and difference between the populations of levels activated by noncoherent pumping. This change in the relaxation is due to a tendency of a thermal reservoir to create an additional difference between the populations of quasienergy states that appear under the influence of the resonance field. It is shown that as a consequence there is a considerable change in the nature of the interaction with the radiation field in laser crystals with three-level active centers when the pump power is close to the threshold. The lasing conditions are found subject to such changes. It is shown that the threshold pump power can be reduced in this case to a value at which the difference between the populations of the active levels vanishes and lasing appears because of an inversion of the populations in a system of quasienergy levels. Under transient conditions the lasing frequency near the threshold should then depend on the pump

DOI
10.1070/qe1986v016n02abeh005734

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arXiv:quant-ph/0512009•Dec 1, 2005•1 citation
A theoretical study is made of the influence of changes in the relaxation of a three-level system in a resonance field on the dispersion, absorption, and difference between the populations of levels activated by noncoherent pumping. This change in the relaxation is due to a tendency of a thermal reservoir to create an additional difference between the populations of quasienergy states that appear under the influence of the resonance field. It is shown that as a consequence there is a considerable change in the nature of the interaction with the radiation field in laser crystals with three-level active centers when the pump power is close to the threshold. The lasing conditions are found subject to such changes. It is shown that the threshold pump power can be reduced in this case to a value at which the difference between the populations of the active levels vanishes and lasing appears because of an inversion of the populations in a system of quasienergy levels. Under transient conditions the lasing frequency near the threshold should then depend on the pump
An analysis is made of the interaction of a three-level cascade atomic system with a resonant laser field. An investigation is made of the dynamics of the populations of the quasienergy states and of the atomic levels over times greater than the spontaneous transition times. In the steady-state regime the distribution of atoms over various quasienergy states is obtained under two-photon resonance conditions and for the case when all the resonances are strong. It is found that a suitable selection of the interaction parameters can establish an inversion between the quasienergy states and also due to atomic transitions. The total probability of spontaneous scattering is calculated. It is shown that, under two-photon resonance conditions, the scattering intensity increases sharply due to a self-induced resonance.
We characterize analytically the nature of the lasing solutions of a laser operating without population inversion. We consider models involving three-level media interacting with a strong driving field and a lasing field in the vicinity of the lasing threshold. We assess the influence of different relaxation and pumping schemes on the dynamics of these lasers. We use the atom-field detuning, the cavity detuning, and the linear gain as bifurcation parameters. Depending on their values, the stable lasing solution is shown to be cw or self-pulsing. We show that the optimal lasing operation is achieved if both the driving field frequency and the cavity frequency are out of resonance with the atomic frequencies. Physically, the lasing regimes arise from nonlinearly interacting sidebands induced in the lasing medium by atomic interference.
An analysis is made of the intermolecular relaxation processes in activated solutions, which transform a two-level system of vibronic states of the activator molecules to a four-level system. It is shown that this alters considerably the main relationships in the theory of amplification and generation of light in activated solutions. More rigorous relationships obtained in the new model predict changes (in the course of pumping) not only of the intensity but generally also of the position and form of the absorption and luminescence spectra of such solutions, which should help in the interpretation of the known and new stimulated emission phenomena.
A new version of obtaining short-wave lasing on transition between highly excited states and the ground state of active atoms in the buffer gas atmosphere is studied theoretically. The mechanism of obtaining population inversion on such a transition is associated with the establishment of the local Boltzmann distribution of populations in a group of highly excited levels due to frequent collisions. If the excitation of the upper-lying level is performed by two laser radiation sources with frequencies ω 1 and ω 2 , short-wave lasing can be obtained at a frequency close to the total frequency ω 1 + ω 2 . The conditions for the emergence of population inversion are analyzed and simple analytic formulas are derived. It is shown that collision-induced enhancement of short-wave radiation can occur for pumping intensities on the order of 100 W/cm 2 . For pumping intensities on the order of 1000 W/cm 2 , the amplification factor for short-wave radiation may attain values of 3 cm −1 (for an active atom concentration of N ∼ 10 15 cm −3 ), which is sufficient for the development of lasing per path through an active medium (superradiance condition) for a length of the active medium on the order of 10 cm.
The theory of amplification and lasing without population inversion in a three-level medium with inhomogeneous broadening via the formation of an open V configuration is elaborated. The conditions for energy transfer from the infrared into the visible spectral range, i.e., the conditions of up-conversion n b >n c >n a , and the external field required for saturation of the b⇄a transition are established. Two-photon resonant Raman transitions in ensemble of mobile atoms of a gas-discharge plasma are analyzed. The frequency shift of the probe field spectrum as a whole is shown to be governed by the frequency shift of the pump field multiplied by the ratio of the wave numbers of the probe amplification field and the pump field. The interaction of atoms through Ne transitions with the pump field (λ=1.15 εm, 2p 4-2s 2 transition) and the lasing field (λ=0.6328 εm, 3s 2-2p 2 transition) with an increase in the lasing frequency by a factor of 1.82 with respect to the absorbed radiation is calculated.
We show lasing without population inversion in a closed four-level atomic system which is no longer incoherently pumped on the transition at which lasing occurs. The four-level system can overcome some limits in the typical lambda-type and V-type three-level systems, furthermore it is possible to achieve lasing even in the absence of the inversion condition for the thermal radiation fields or of the inversion of spontaneous decay rate. We find that when the detuning of probe field is equal to that of coherent coupling field, there is a peak value along with the increase of the detuning. To explain it, we bring forward that there are adiabatic and nonadiabatic stimulated Raman processes when a three-level atomic system is interacted with two coherent fields, so there are two mechanisms influencing the change of probe field. We believe that it can explain more general lasing without inversion processes because of quantum interference induced by coherent fields.