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Journal of Physics B Atomic Molecular and Optical Physics

Saturated absorption spectroscopy of calcium in a hollow-cathode lamp

Umakanth Dammalapati, I Norris, Erling Riis

Published Jul 20, 2009• 21 citations
Publisher

Abstract

We report on a technique for obtaining dispersive saturated absorption features by two pump beams derived from an acousto-optic modulator. One of the beams is frequency shifted by the modulator allowing for a variable frequency offset of the resulting signal. They are used to saturate the atomic transition in the low-density vapour of the lamp. The sensitivity of the technique is sufficient to observe clear signals from isotopes of calcium unresolved by the inhomogeneous broadening and with natural abundances of less than 0.2%. The technique is used for offset locking the frequency of a Ti:Sapphire laser used for laser cooling and trapping of calcium.

DOI
10.1088/0953-4075/42/16/165001

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We report on a technique for obtaining dispersive saturated absorption features by two pump beams derived from an acousto-optic modulator. One of the beams is frequency shifted by the modulator allowing for a variable frequency offset of the resulting signal. They are used to saturate the atomic transition in the low-density vapour of the lamp. The sensitivity of the technique is sufficient to observe clear signals from isotopes of calcium unresolved by the inhomogeneous broadening and with natural abundances of less than 0.2%. The technique is used for offset locking the frequency of a Ti:Sapphire laser used for laser cooling and trapping of calcium.
We report the development of a simple method for eliminating coherent background noise and fluctuations from saturation spectroscopy signals. With this technique, which utilizes a traveling-wave acousto-optic modulator to simultaneously frequency-shift and modulate the saturating beam, we have routinely observed zero background, Doppler-free saturation resonances in the I2I_{2}I2​ at 514.5 nm. With a low-noise laser or high pump modulation frequency, we have achieved detection sensitivity approaching the fundamental quantum limit.
We demonstrate a spectroscopy method that can be applied in an atomic beam, light-pressure-induced spectroscopy (LiPS). A simple pump and probe experiment yields a dispersivelike spectroscopy signal that can be utilized for laser frequency stabilization. The underlying principles are discussed and compared to Monte Carlo simulations. The shape of the dispersive signal is well described by the simulations. The zero crossing point of the signal is redshifted with respect to the atomic resonance by $\ensuremath{\sim}3\text{ }\text{MHz}$ (one-tenth of the natural linewidth) and depends slightly on the laser intensity. The shift of the zero crossing is determined by laser-induced fluorescence and compared with results of Doppler-free saturation spectroscopy. To check the potential of LiPS for frequency stabilization purposes, it was used to frequency-stabilize the laser for 400 min. Frequency fluctuations of only 0.12 MHz were measured.
We describe an inexpensive lock-in amplifier that can be built using discrete off-the-shelf RF components and home-built analog circuits. This lock-in has been used in a feedback loop to lock the frequency of a laser to an atomic transition. The frequency stability was tested by trapping rubidium atoms. The feedback loop involves obtaining a modulated saturated absorption signal from a vapor cell using an acousto-optic modulator to modulate the laser frequency. The absorption signal is sent to the lock-in to generate an error signal, proportional to the first derivative of the absorption, which is fed back to the laser to complete the feedback loop. We also demonstrate a simplified optical setup for viewing the saturated absorption spectrum. In this case, the signal consists of narrow saturated absorption spectra riding on top of a Doppler-broadened pedestal. We show that it is possible to greatly reduce the effect of this background and lock the laser to the atomic resonance by modifying the home-built lock-in to generate an error signal proportional to the third derivative of the absorption. The results of this work can be adapted for advanced undergraduate laboratory work.PACS Nos.: 01.50Pa, 07.50.–e, 42.62Fi, 42.60Fc
The thermal velocity distribution of a calcium atomic beam was compressed into a narrow velocity distribution with selectable velocities. Subsequently these slow atoms were deflected by an angle of 30° by a one-dimensional optical molasses. In the deflected beam we obtained an estimated flux of several 1010 atoms/s at mean longitudinal velocities near 35 m/s and a velocity width of approximately 13 m/s. The transverse velocities of the deflected atoms were close to the one-dimensional Doppler limit. We have observed saturated absorption signals in the deflected laser-cooled beam. The reduced transit time broadening allowed us to resolve the recoil splitting in saturated absorption.
Abstract In optical systems, acousto-optic modulators (AOMs) and electro-optic modulators (EOMs) are commonly utilized for laser frequency manipulation. However, these devices come with drawbacks such as high cost and the requirement of optical adjustments to change the frequency shift direction. In this study, we propose an alternative method that harnesses the Zeeman effect in the saturated-absorption spectroscopy to shift the energy levels in atom. With this technique, the laser frequency can be shifted without the need for AOMs or EOMs. The stability of laser locking was investigated for any case of polarization of probe and pump beam. We found when the polarization of the probe and pump beams is linear and perpendicular, it results in the highest level of stability in laser locking compared to other polarization configurations.
We present and analyze a bichromatic version of the well-known saturation absorption spectroscopy technique used to stabilize lasers to atomic resonances without Doppler broadening. We show that the spectroscopic properties can be transferred between two transitions at very different wavelengths by spectral hole burning in a Doppler-broadened atomic ensemble. Specifically, we demonstrate that this technique can be used to stabilize a laser to the D1 line of Rb87 by obtaining a saturation absorption spectrum with a strong pump laser stabilized to the D2 line. This allows for more freedom in the choice of the probe laser frequency offsets compared to conventional saturation absorption spectroscopy. We compare our experimental results to an analytical model and numerical results based on rate equations.