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Journal of Physics Conference Series

Exploring the Zeeman effect in spectroscopy for laser frequency manipulation in optical systems

Nuttanan Tanasanchai, Phatwarach Siriworakoonchai, Parinya Udommai, Waranont Anukool

Published Dec 1, 2023• 0 citations
Publisher

Abstract

Abstract In optical systems, acousto-optic modulators (AOMs) and electro-optic modulators (EOMs) are commonly utilized for laser frequency manipulation. However, these devices come with drawbacks such as high cost and the requirement of optical adjustments to change the frequency shift direction. In this study, we propose an alternative method that harnesses the Zeeman effect in the saturated-absorption spectroscopy to shift the energy levels in atom. With this technique, the laser frequency can be shifted without the need for AOMs or EOMs. The stability of laser locking was investigated for any case of polarization of probe and pump beam. We found when the polarization of the probe and pump beams is linear and perpendicular, it results in the highest level of stability in laser locking compared to other polarization configurations.

DOI
10.1088/1742-6596/2653/1/012035

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Abstract In optical systems, acousto-optic modulators (AOMs) and electro-optic modulators (EOMs) are commonly utilized for laser frequency manipulation. However, these devices come with drawbacks such as high cost and the requirement of optical adjustments to change the frequency shift direction. In this study, we propose an alternative method that harnesses the Zeeman effect in the saturated-absorption spectroscopy to shift the energy levels in atom. With this technique, the laser frequency can be shifted without the need for AOMs or EOMs. The stability of laser locking was investigated for any case of polarization of probe and pump beam. We found when the polarization of the probe and pump beams is linear and perpendicular, it results in the highest level of stability in laser locking compared to other polarization configurations.
The stabilizing and shifting of laser frequency are very important for the interaction between the laser and atoms. The modulation transfer spectroscopy for the 87 Rb atom with D2 line transition F = 2 → F′ = 3 is used for stabilizing and shifting the frequency of the external cavity grating feedback diode laser. The resonant phase modulator with electro—optical effect is used to generate frequency sideband to lock the laser frequency. In the locking scheme, circularly polarized pump- and probe-beams are used. By optimizing the temperature of the vapor, the pump- and probe-beam intensity, the laser linewidth of 280 kHz is obtained. Furthermore, the magnetic field generated by a solenoid is added into the system. Therefore the system can achieve the frequency locking at any point in a range of hundreds of megahertz frequency shifting with very low power loss.
A sub-MHz frequency stability of the laser is crucial in the quantum-atom experiment where precise atomic transition is required for control and manipulation of atom like in the atom quantum computing. In this work, we have built the frequency stabilization system for the lasers used in our cold Rubidium atom experiment in the magneto-optical trap (MOT) and the optical tweezers. We utilized a Rubidium vapour glass cell as a frequency reference, which provides atomically absolute reference point with low complexity setup. By mean of the absorption of the laser beam by the Rubidium vapour, the Doppler-free saturated absorption (DFSA) experiment was setup to produce the D2 line spectra. The acousto-optic modulator (AOM) was used to sinusoidally dither the laser frequency and consequently the resonance peaks in the spectra. Detailing in this work, the AOM sinusoidal dithering and the dithered DFSA signal had orthogonality and were processed together to produce the error signal used to stabilize the laser frequency to the resonant peak. This frequency stabilization system achieved the frequency standard deviation below 0.75 MHz over 200 minutes period. The system also allowed for stabilized frequency tunability over a range of 55-60 MHz about the target resonance peak. This performance is significant for stabilizing the lasers in the MOT experiment and related quantum-atom research.
We propose a far off-resonance laser frequency stabilization method that can accurately adjust the frequency lock points based on the Faraday rotation spectroscopy. The atomic magnetometer based on the spin-exchange relaxation-free (SERF) theory needs to stabilize the frequency of the probe laser on the detuning of several gigahertz (GHz) away from the resonance of the alkali metal atom, to reduce the absorption of the probe light by the alkali metal vapor cell. We propose a laser frequency stabilization method that can accurately adjust the frequency lock points using an acousto-optic modulator based on Faraday rotation spectroscopy. We reveal the principles of the method and simulate the new Faraday rotation spectra. Besides, we study the effect of the amount of frequency shift of the acousto - optic modulator and the temperature of the alkali metal vapor cell on the frequency lock points of the spectra, and give the formula for calculating the frequency point. Our proposed laser frequency stabilization method can stabilize the laser frequency on the detuning of several gigahertz (GHz) away from the resonance of the alkali metal atom and can adjust the frequency lock points quickly and accurately. This method can be used in atomic magnetometer, degenerate Raman sideband cooling (DRSC) and two photon excitation of Rydberg states.
The stabilizing and shifting of laser frequency are very important for the interaction between the laser and atoms. The modulation transfer spectroscopy for the87 Rb atom with D2 line transition F = 2 → F = 3 is used for stabilizing and shifting the frequency of the external cavity grating feedback diode laser. The resonant phase modulator with electro–optical effect is used to generate frequency sideband to lock the laser frequency. In the locking scheme, circularly polarized pump- and probe-beams are used. By optimizing the temperature of the vapor, the pump- and probe-beam intensity, the laser linewidth of 280 kHz is obtained. Furthermore, the magnetic field generated by a solenoid is added into the system. Therefore the system can achieve the frequency locking at any point in a range of hundreds of megahertz frequency shifting with very low power loss.
Utilizing the Zeeman Faraday effect in atomic vapor cells, a novel setup is introduced both for laser intensity stabilization and laser intensity modulation. The method is based on the closed loop control of the polarization rotation angle of the laser light in an atomic vapor cell for adjustment of the laser intensity. Characterizing the implemented setup, it is shown that more than 30 dB attenuation of the optical fluctuation is achieved in the frequency range from DC to 1 kHz. Meanwhile, the laser intensity could be efficiently locked to a modulating voltage signal, which results in amplitude modulation of the laser beam. We believe that this simple method could be effectively used in different atomic physics experiments, including the stabilization of the laser intensity in applications where near resonance frequency sweeping is required or applications that contain optical modulation of lasers in lock-in detection schemes.
Precise laser stabilization is a fundamental aspect of modern metrology, directly influencing the accuracy of fundamental measurements in fields such as high-precision metrology, atomic sensor applications, and quantum technologies. Saturation absorption spectroscopy (SAS) is one of the most effective techniques for achieving high spectral stability, as it enables laser frequencies to be locked to atomic resonances. This technique exploits the nonlinear interaction between a weaker probe beam and a stronger pump beam within a rubidium (Rb) atomic vapor cell. By eliminating Doppler broadening, SAS allows well-defined hyperfine transitions to be resolved, providing a reliable optical frequency reference. This study aims to optimize laser frequency stabilization using the SAS technique by investigating the effects of laser light polarization, atomic vapor cell temperature, and pump-probe power adjustments. Polarization-dependent selection rules influence transition probabilities, thereby affecting spectral contrast and frequency stability. Additionally, atomic density variations, which depend on the vapor cell temperature, influence signal strength and linewidth, necessitating precise temperature control for optimal performance. Furthermore, the pump power must be sufficient to induce saturation without excessive power broadening, while the probe power must remain low enough to prevent spectral line distortion. By optimizing polarization, temperature, and power parameters, the stabilization of the Rb atomic laser can be enhanced, leading to improved reproducibility and consistency in high-precision measurements. SAS-based laser stabilization is particularly crucial for atomic sensor applications and quantum technologies, where highly stable, narrow-linewidth lasers are essential for precision measurements. Applications such as atomic magnetometers, gyroscopes, and inertial navigation systems depend on precisely stabilized lasers for optimal performance. By enhancing the reliability of laser frequency stabilization, this work contributes to the advancement of next-generation atomic sensors with improved sensitivity and stability.