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Physical Review A

Cavity QED with high- Q whispering gallery modes

David W. Vernooy, Akira Furusawa, N. Ph. Georgiades, Vladimir S. Ilchenko, Harry J. Kimble

Published Apr 1, 1998• 285 citations
Publisher

Abstract

We report measurements of cavity-QED effects for the radiative coupling of atoms in a dilute vapor to the external evanescent field of a whispering-gallery mode (WGM) in a fused silica microsphere. The high $Q$ $(5\ifmmode\times\else\texttimes\fi{}{10}^{7})$, small mode volume (10${}^{\ensuremath{-}8}$ cm${}^{3})$, and unusual symmetry of the microcavity evanescent field enable velocity-selective interactions between fields with photon number of order unity in the WGM and ${N}_{T}\ensuremath{\sim}1$ atoms in the surrounding vapor.

DOI
10.1103/physreva.57.r2293

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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Feb 25, 1999•0 citations
We report measurements of cavity-QED effects for the radiative coupling of atoms in a dilute vapor to the external evanescent field of a whispering-gallery mode (WGM) in a fused silica microsphere. The high QQQ (5\ifmmode×\else\texttimes\fi107)(5\ifmmode\times\else\texttimes\fi{}{10}^{7})(5\ifmmode×\else\texttimes\fi107), small mode volume (10\ensuremath−8{}^{\ensuremath{-}8}\ensuremath−8 cm3){}^{3})3), and unusual symmetry of the microcavity evanescent field enable velocity-selective interactions between fields with photon number of order unity in the WGM and NT\ensuremath∼1{N}_{T}\ensuremath{\sim}1NT​\ensuremath∼1 atoms in the surrounding vapor.
Summary form only given, as follows: The high Q whispering gallery modes of silica microspheres are promising for quantum optics and nonlinear optics experiments involving atoms and photons stored in very small volumes. We have developed the technology of these resonators, learning how to couple light in and out through optical fibers, how to obtain and measure record Q factors, and how to probe, by near-field optical microscopy, the electric field distribution immediately outside the sphere. Whispering gallery mode lasers have also been obtained with microspheres made of silica doped with neodymium ions. We describe these experiments and discuss projects involving the coupling of whispering gallery modes to single atoms or ions to perform cavity QED experiments in the optical domain.
The whispering gallery modes (WGMs) of quartz microspheres are investigated for the purpose of strong coupling between single photons and atoms in cavity quantum electrodynamics (cavity QED). Within our current understanding of the loss mechanisms of the WGMs, the saturation photon number n0{n}_{0}n0​ and critical atom number N0{N}_{0}N0​ cannot be minimized simultaneously, so that an ``optimal'' sphere size is taken to be the radius for which the geometric mean n0N0,\sqrt{{n}_{0}{N}_{0}},n0​N0​​, is minimized. While a general treatment is given for the dimensionless parameters used to characterize the atom-cavity system, detailed consideration is given to the D2{D}_{2}D2​ transition in atomic cesium at ${\ensuremath{\lambda}}_{0}=852\mathrm{nm}$ using fused-silica microspheres, for which the maximum coupling coefficient ${g}_{a}/(2\ensuremath{\pi})\ensuremath{\approx}750\mathrm{MHz}$ occurs for a sphere radius $a=3.63\ensuremath{\mu}\mathrm{m}$ corresponding to the minimum for ${n}_{0}\ensuremath{\approx}6.06\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6}.$ By contrast, the minimum for ${N}_{0}\ensuremath{\approx}9.00\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6}$ occurs for a sphere radius of $a=8.12\ensuremath{\mu}\mathrm{m},$ while the optimal sphere size for which n0N0\sqrt{{n}_{0}{N}_{0}}n0​N0​​ is minimized occurs at $a=7.83\ensuremath{\mu}\mathrm{m}.$ On an experimental front, we have fabricated fused-silica microspheres with radii $a\ensuremath{\sim}10\ensuremath{\mu}\mathrm{m}$ and consistently observed quality factors $Q>~0.8\ifmmode\times\else\texttimes\fi{}{10}^{7}.$ These results for the WGMs are compared with corresponding parameters achieved in Fabry-Perot cavities to demonstrate the significant potential of microspheres as a tool for cavity QED with strong coupling.
We have tuned the whispering-gallery modes of a fused-silica microresonator over nearly 1 nm at 800 nm, i.e., over half a free spectral range, or 10(6) linewidths of the resonator. This result has been achieved by use of a new method based on the stretching of a two-stem microsphere. We describe devices that will permit new cavity QED experiments with this high- Q optical resonator when it is desirable to optimize its coupling to emitters with given transition frequencies. The demonstrated tuning capability is compatible with both UHV and low-temperature operation, which should be useful for future experiments with laser-cooled atoms or single quantum dots.
The bound state structure and dynamics for an atom trap formed from the whispering gallery modes (WGMs) of a dielectric microsphere are investigated. The coupling of the quantized internal and external atomic degrees of freedom plays a fundamental role in the quantum dynamics of this atom gallery. The radiative processes for a cold atom near a microsphere are modified due to the special symmetry of the atom gallery, the WGM mode structure, and the finite extent of the center-of-mass (c.m.) wave packet. Finally, interesting implications of the quantized c.m. for atomic matter waves and cavity QED with a quantum field are mentioned.
Silica microspheres behave as efficient optical microresonators when small-volume whispering-gallery modes (WGMs) are used. We have realized a cryogenic set-up to work with microspheres immersed in a superfluid helium bath. Quality factors up to 109 have been obtained at 2 K. In this environment, we have been able to observe a dispersive bistable behavior of the WGM resonances, due to the weak intrinsic Kerr optical nonlinearity of silica, with a threshold power of 10 (mu) W only. This result opens the way to the realization of thresholdless microlaser, based on a rare-earth doped silica microsphere and to other Cavity-QED projects with microspheres at low temperatures.