Highly excited Rydberg atoms have many exaggerated properties. In particular, the interaction strength between such atoms can be varied over an enormous range. In a mesoscopic ensemble, such strong, long-range interactions can be used for fast preparation of desired many-particle states. We generated Rydberg excitations in an ultra-cold atomic gas and subsequently converted them into light. As the principal quantum number n was increased beyond ~70, no more than a single excitation was retrieved from the entire mesoscopic ensemble of atoms. These results hold promise for studies of dynamics and disorder in many-body systems with tunable interactions and for scalable quantum information networks.
Highly excited Rydberg atoms have many exaggerated properties. In particular, the interaction strength between such atoms can be varied over an enormous range. In a mesoscopic ensemble, such strong, long-range interactions can be used for fast preparation of desired many-particle states. We generated Rydberg excitations in an ultra-cold atomic gas and subsequently converted them into light. As the principal quantum number n was increased beyond ~70, no more than a single excitation was retrieved from the entire mesoscopic ensemble of atoms. These results hold promise for studies of dynamics and disorder in many-body systems with tunable interactions and for scalable quantum information networks.
Interacting Rydberg excitations in cold atomic ensembles can exhibit large quantum nonlinearities that enable engineering of strong interactions between individual photons. Consequently, Rydberg ensembles are a promising platform for quantum information applications and the study of more fundamental physics of few- and many-body phenomena with interacting photons. This thesis presents a series of experiments that study and exploit different regimes of Rydberg-mediated interactions. We report the realization of an efficient on-demand single-photon source. The strong long-range Rydberg interactions allow the excitation of only a single collective Rydberg state within the entire atomic medium. The collective excitation can be subsequently retrieved as a single-photon. We use this scheme to generate highly pure and highly indistinguishable photons, which are suitable for scalable quantum information applications. These photons can be compatible with other atomic systems due to their narrow bandwidth, which makes building practical hybrid quantum systems feasible. Here, we demonstrate high visibility two-photon quantum interference between our Rydberg-produced photons, and photons emitted by a remote single-trapped ion. We also study Rydberg atoms under electromagnetically induced transparency conditions, where coherent superpostions of photons and Rydberg excitations propagate through the atomic medium as lossless dark-state polaritons. In the experiment, we use the external control fields to tune the interactions to a many-body regime where we can observe resonant scattering of dark-state polaritons to lossy channels. We show that the enhanced scattering process arises as a pure three-body effect.
The advances in laser cooling and trapping techniques allow samples of ultra-cold atoms to be created and controlled for the study of quantum physics. In this thesis, we focus on using ensembles of cold atoms to investigate novel quantum effects and their applications in quantum optics. Realization of a scalable intercontinental quantum system, e.g. a global quantum internet, relies on quantum memories with long lifetimes on the order of seconds. We have reduced the differential light shifts of the atomic ground states to a sub-Hz level and achieved a lifetime of 16 seconds. Achieving fast and efficient quantum operations, on the other hand, requires strongly-interacting systems. We explore highly excited Rydberg atoms towards this goal and demonstrate Rydberg excitation blockade, many-body Rabi oscillations, trapping of Rydberg atoms, deterministic single photon source, and atom-photon entanglement. Finally, we integrate the two essential capabilities for quantum information processing, fast quantum state generation and long-term storage, by simultaneously exploiting Rydberg levels for interactions and ground atomic levels for the storage of quantum state. Our work advances the control of coherence properties and interactions in cold atomic ensembles to a new level and opens new opportunities for studies of complex quantum systems.
Long-term storage of quantum information has diverse applications in quantum information science. This work presents an experimental realization of quantum memories with lifetimes greater then 0.1 s. The memories are based on cold rubidium atoms confined in one-dimensional optical lattices. First realization of lattice-based quantum memory and entanglement between a light field and a spin wave is presented in Chapter II. Chapter III describes two different methods (two-photon and magnetic) of compensation for inhomogeneous differential light shifts between the memory levels due to optical trapping potentials, and demonstration of entanglement between a telecom-band light field and a light-shift compensated memory qubit. Highly excited Rydberg atoms present a unique platform for study of strongly correlated systems and quantum information, because of their enormous dipole moments and consequent strong, long-range interactions. In the experiment described in Chapter IV single collective Rydberg excitations are created in a cold atomic gas. After a variable storage period the excitations are converted into light. As the principal quantum number n of the Rydberg level is increased beyond ~ 70, no more than a single excitation is retrieved from the entire mesoscopic ensemble of atoms. In Chapter V, by spatially selective conversion of the spin wave into a light field, we demonstrate that Rydberg-level interactions create long-range correlations of collective atomic excitations. These results hold promise for studies of dynamics and disorder in many-body systems with tunable interactions and for scalable quantum information networks. Chapter VI presents initial observations of coherent many-body Rabi oscillations between the ground level and a Rydberg level using several hundred cold rubidium atoms. The strongly pronounced oscillations indicate a nearly complete excitation blockade of the entire mesoscopic ensemble by a single excited atom.
We examine state mixing in a dense, cold Rydberg gas. Cold Rb atom clouds in an optical dipole trap are excited into nD5/2 Rydberg levels using narrow-bandwidth laser pulses. For n=43, two atoms excited to 43D5/2 states can be converted to 41F7/2 and 45P3/2 product states via a F\"orster resonance. We find, unexpectedly, that up to 50% of the Rydberg atoms are detected in such product states after only 100 ns of interaction time. The experiment is modeled using many-body quantum simulations. To reproduce the mixing fractions measured near F\"orster resonances, we use an exact, nonperturbative many-atom Hamiltonian in which product states are treated on an equal basis with the laser-excited nD5/2 Rydberg level. Simplified many-body interaction models based on sums over pairwise atomic potentials cannot reproduce the measured mixing fractions.
One of the most fascinating and challenging topics of recent years is many- body physics. Owing to the large number of components of real physi- cal systems an analytical approach or numerical solutions are typically not practicable. However, an experimental approach to this problem is possible thanks to an unprecedented level of matter control on the atomic scale. In our setup we use atoms excited to high-lying energy states, called Rydberg atoms, which have peculiar properties like the extremely long lifetime and strong interactions. These experimental features make a cold ensem- ble of Rydberg atoms a very controllable example of a strongly interacting many-body system and provide a promising framework for quantum simulation.
Interacting ultracold atomic quantum gases provide an ideal test bed to study strongly correlated quantum matter. The interactions between atoms in such an ultracold quantum gas are typically short-ranged and well described by an effective contact potential. Introducing longer-range interactions promises the realization of novel quantum phases which are absent in systems with only short-range interactions. Trapped atoms, resonantly laser-coupled to highly excited, strongly interacting Rydberg states have been proposed as a versatile platform to realize such long-range interacting quantum matter. In a first experiment presented in this thesis, we combined the single-atom-sensitive local preparation and detection enabled by a quantum gas microscope to prepare and microscopically characterize an ensemble of rubidium-87 atoms trapped in an optical lattice in the regime of strong Rydberg blockade. There, we observe collectively enhanced optical coupling in an effective two-level system, the so-called “superatom”, and infer the presence of entanglement. Detuned optical coupling to Rydberg states, termed “Rydberg dressing”, has been proposed as an alternative approach to induce long-range interactions. Rather than directly exciting an atom to a Rydberg state, the properties of the latter are admixed to a ground state, which consequently acquires long-range interactions. In the context of this thesis, we have designed a laser system in the ultraviolet spectral range to admix Rydberg P-state character to the ground state of atoms in an optical lattice. In an emerging Ising quantum magnet, the presence of Rydberg-dressed interactions was demonstrated by an interferometric technique combined with spatially resolved spin correlation measurements. The theoretically predicted tunability of the isotropy and range of the interaction were confirmed experimentally. While these initial measurements exhibited unexpected dissipation, in a subsequent experiment in a one-dimensional spin chain this dissipation was overcome. We substantiated the improved coherence times by tracking the time evolution of the magnetization upon suddenly switching on interactions and observing coherent collapse and revival dynamics, one of the hallmarks of coherent quantum evolution. Our results establish Rydberg-dressed interactions in ultracold gases and pave the way to realize and study novel exotic quantum phases.