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Driven dissipative dynamics of an interacting Rydberg gas

Cristiano Simonelli, Ricardo Gutiérrez, Matteo Archimi, Francesco Castellucci, E. Arimondo, D. Ciampini, Matteo Marcuzzi, Igor Lesanovsky, O. Morsch

Published Jan 1, 2017• 0 citations
OpenAlex

Abstract

One of the most fascinating and challenging topics of recent years is many- body physics. Owing to the large number of components of real physi- cal systems an analytical approach or numerical solutions are typically not practicable. However, an experimental approach to this problem is possible thanks to an unprecedented level of matter control on the atomic scale. In our setup we use atoms excited to high-lying energy states, called Rydberg atoms, which have peculiar properties like the extremely long lifetime and strong interactions. These experimental features make a cold ensem- ble of Rydberg atoms a very controllable example of a strongly interacting many-body system and provide a promising framework for quantum simulation.

Related papers

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The remarkable progress in control over cold atomic gases has led to a point where people are no longer satisfied with merely studying these systems, but rather put them to use to understand complex quantum many-body systems. The basis of this development is a deep understanding of the interaction between atoms, and how to exploit those in order to engineer interesting and novel quantum-systems. The aim of this particular thesis is to contribute to this third quantum revolution [1] and hence help to understand the inner workings of complex many-body systems. We present a method to control the shape and character of the interaction between cold atoms based on dressing the atomic ground-state with a Rydberg-state. The latter induces a van der Waals interaction between all the atoms in the ensemble, and allows for control via the coupling light-field. We find that with increasing atom densities the ensemble shows a direct transition into a collective regime that preempts the onset of three-body interactions associated with a break-down of the first Born-approximation. The reason for this intriguing behavior is the strong interaction between Rydberg atoms that gives rise to the blockade-mechanism, and prevents the simultaneous excitation to the Rydberg-state for spatially close atoms. The non-trivial behavior of the interaction-potential within the collective regime yields a novel tool for shaping the interaction between ground-state atoms beyond s-wave scattering. We study this collective regime and the resulting interaction-potential between the atoms within a variational/mean-field approach, and discuss its effects on a trapped Bose-Einstein condensate. Artificial atoms show remarkable properties, that are often superior to real atoms. In particular, since they are built out of many constituents, such systems often exhibit an enhanced coupling to the light-field as well as strong optical non-linearities even for small light-fields. On the other hand, noise in quantum-mechanical systems can not only destroy coherence, but rather can be used in order to robustly drive a system into an interesting state. We study the effect of a controlled dephasing onto an artificial atom in the context of an ensemble of atoms coherently coupled to a Rydberg state and demonstrate that such an enhanced artificial atom allows for the deterministic absorption of a single photon from an arbitrary incoming probe field. Such behavior yields a unique tool in light-matter interaction, and opens the path to realise quantum-networks or to fabricate novel quantum-devices. Here, we discuss the applicability of this single-photon absorber as a single-photon transistor, a high fidelity n-photon counter, and a device that allows for the deterministic creation of non-classical states of light via photon-subtraction. A non-trivial topological order of quantum-states leads to conservation of certain properties and, hence, increases their robustness against external perturbations. This can even stabilize quantum-states against local fluctuations. The latter usually corrupts the coherence within a macroscopic object and thereby prevents quantum-phenomena to occur in our macroscopic world. As an example of such a topological state, we study the behavior of vortex-excitations in a two-dimensional superfluid confined to a periodic potential, as can be realised within a cold atomic gas in an optical lattice. For large superfluid filling factors and strong interactions, the healing-length and, accordingly, the vortex core is much smaller than the lattice spacing. 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During this thesis, the Physics of interacting systems has been investigated experimentally using Cold Rydberg gases. Rydberg atoms are very excited atoms and have the particularity to interact strongly together through long-range electrostatic interaction. A first highlight of the thesis is a direct experimental observation of a 4-body process. This process consists in internal exchanges of excitations between 4 Rydberg atoms due to their mutual interactions. In addition to its experimental observation, the process has been succefully described theoretically at a quantum level. A second highlight of this thesis has concerns the study of the laser excitation of strongly interacting Rydberg gases. In this regime, many-body quantum correlations play a central role leading to fascinating many-body behavior. In addition to fundamental interests, such systems could be used to implement quantum simulator or non-classical light sources. The system has been investigated during this thesis through the counting statistics of the Rydberg excitation. A highly sub-poisonian, i.e correlated, statistics has been observed in the regim of strong interactions proving the many-body nature of the system. A third highlight of this thesis is the development of an original theoretical model to describe the laser excitation of strongly interacting Rydberg gases. Using the so-called Dicke collective states, it has been possible to catch several interesting features of this many-body problem.

•Mar 12, 2013•0 citations

Lattice gauge theories and constrained systems: from quantum simulation to non-equilibrium dynamics

Federica Maria Surace

In the last decade the non-equilibrium dynamics of isolated quantum systems has raised a huge interest for both its conceptual and practical implications. Simulation of quantum dynamics represents by now a very active research effort, with highly controllable quantum devices composed of hundreds of qubits already being realized in numerous setups. These offer the unprecedented possibility to access real-time quantum dynamics and strongly correlated quantum many-body states, opening numerous avenues not only for future quantum technologies, but also for long-standing theoretical problems. One of the most sought-after applications is the computation of real-time evolution in theories of fundamental interactions. Since Wilson's proposal in 1974, the equilibrium phase diagrams of lattice gauge theories have been successfully investigated with Monte Carlo simulations in a wide range of parameters. Nonequilibrium properties, on the other hand, cannot be accessed with conventional techniques. Thanks to the recent advances in numerics (e.g. tensor networks) and experiments (quantum simulation), new promising tools are now available for tackling these questions. Remarkable works have already demonstrated that applying these techniques to simple theories, such as one-dimensional quantum electrodynamics, can help to detect the signatures of confinement and pair creation. Despite these impressive achievements, investigating the non-equilibrium dynamics of gauge theories with quantum simulators turned out to be extremely challenging. This is mostly due to the complex constrained dynamics of these theories, which make their simulation with realistic atomic platforms particularly difficult. At the same time, the dynamical constraints can play a key role in determining novel interesting phenomena and peculiar non-equilibrium properties. These phenomena -- which include, for example, quantum scars, fractons, Hilbert space fragmentation -- can lead to anomalous dynamics, eventually evading the paradigm of thermalization, which predicts the relaxation of physical observable to their thermodynamic values. The aim of this thesis is twofold: first, we want to address through a combination of numerical and analytical tools some of the open questions regarding the non-equilibrium dynamics of quantum many-body systems with constrained Hilbert spaces, including lattice gauge theories. In addition, the work reported here is part of a large effort of the community towards the quantum simulation of complex phenomena of condensed matter and high-energy physics.

•Sep 29, 2021•0 citations
One of the most fascinating and challenging topics of recent years is many- body physics. Owing to the large number of components of real physi- cal systems an analytical approach or numerical solutions are typically not practicable. However, an experimental approach to this problem is possible thanks to an unprecedented level of matter control on the atomic scale. In our setup we use atoms excited to high-lying energy states, called Rydberg atoms, which have peculiar properties like the extremely long lifetime and strong interactions. These experimental features make a cold ensem- ble of Rydberg atoms a very controllable example of a strongly interacting many-body system and provide a promising framework for quantum simulation.
The remarkable progress in control over cold atomic gases has led to a point where people are no longer satisfied with merely studying these systems, but rather put them to use to understand complex quantum many-body systems. The basis of this development is a deep understanding of the interaction between atoms, and how to exploit those in order to engineer interesting and novel quantum-systems. The aim of this particular thesis is to contribute to this third quantum revolution [1] and hence help to understand the inner workings of complex many-body systems. We present a method to control the shape and character of the interaction between cold atoms based on dressing the atomic ground-state with a Rydberg-state. The latter induces a van der Waals interaction between all the atoms in the ensemble, and allows for control via the coupling light-field. We find that with increasing atom densities the ensemble shows a direct transition into a collective regime that preempts the onset of three-body interactions associated with a break-down of the first Born-approximation. The reason for this intriguing behavior is the strong interaction between Rydberg atoms that gives rise to the blockade-mechanism, and prevents the simultaneous excitation to the Rydberg-state for spatially close atoms. The non-trivial behavior of the interaction-potential within the collective regime yields a novel tool for shaping the interaction between ground-state atoms beyond s-wave scattering. We study this collective regime and the resulting interaction-potential between the atoms within a variational/mean-field approach, and discuss its effects on a trapped Bose-Einstein condensate. Artificial atoms show remarkable properties, that are often superior to real atoms. In particular, since they are built out of many constituents, such systems often exhibit an enhanced coupling to the light-field as well as strong optical non-linearities even for small light-fields. On the other hand, noise in quantum-mechanical systems can not only destroy coherence, but rather can be used in order to robustly drive a system into an interesting state. We study the effect of a controlled dephasing onto an artificial atom in the context of an ensemble of atoms coherently coupled to a Rydberg state and demonstrate that such an enhanced artificial atom allows for the deterministic absorption of a single photon from an arbitrary incoming probe field. Such behavior yields a unique tool in light-matter interaction, and opens the path to realise quantum-networks or to fabricate novel quantum-devices. Here, we discuss the applicability of this single-photon absorber as a single-photon transistor, a high fidelity n-photon counter, and a device that allows for the deterministic creation of non-classical states of light via photon-subtraction. A non-trivial topological order of quantum-states leads to conservation of certain properties and, hence, increases their robustness against external perturbations. This can even stabilize quantum-states against local fluctuations. The latter usually corrupts the coherence within a macroscopic object and thereby prevents quantum-phenomena to occur in our macroscopic world. As an example of such a topological state, we study the behavior of vortex-excitations in a two-dimensional superfluid confined to a periodic potential, as can be realised within a cold atomic gas in an optical lattice. For large superfluid filling factors and strong interactions, the healing-length and, accordingly, the vortex core is much smaller than the lattice spacing. As a result, vortices are confined to the plaquettes of the lattice, and can be described in the framework of an effective tight-binding Hamiltonian. Via a first-principle calculation based on coherent-state path-integrals we derive the microscopic parameters of this model and provide an analytic expression for the vortex mass. Moreover, we show that such a quantum vortex is not obliged to follow the superfluid flow, but rather exhibits Bloch-oscillations perpendicular to it, which is a telltale sign for quantum interference of this macroscopic many-body excitation. Recently, Jonathan Simon et al. [2] performed a major step towards simulating quantum many-body systems in cold atomic gases by simulating the paramagnet-antiferro-magnet transition of a one-dimensional Ising-model. Fundamental excitations in the phase with broken translational symmetry are domain-walls carrying fractional statistics. The question is, whether experimentally accessible single-particle excitations, which correspond to two closely-bound domain-walls, decay into fractional excitations or remain closely-bound. By use of perturbation theory, we derive an analytic model for the time-evolution of these fractional excitations in the framework of a tilted Bose-Hubbard model, and demonstrate the existence of a repulsively bound state above a critical center-of-mass momentum. The validity of the perturbative approach is confirmed by the use of t-DMRG simulations. Together with the recent demonstration of single-site addressing and readout in optical lattices, these findings open the path for experimental observation of fractional excitations within cold atomic gases.
Atoms excited to high lying g quantum states, so-called Rydberg atoms, are highly polarizable and, therefore interact strongly with each other at large distances. One result of these interactions is the Rydberg dipole blockade effect, in which strongly interacting atoms excited by the same driving pulse may prevent other atoms from getting excited. This blockade offers several applications, for example the realization of quantum logic gates [1] and the possibility \nof creating entangled states with two atoms [2].
Rydberg atoms, characterized by their strong and long-range dipole-dipole interactions, provide a versatile platform for exploring intriguing collective and many-body effects. Recently, the experimental realization of these effects in dense ensembles and reconfigurable atomic arrays has attracted significant interest, particularly for applications in quantum simulations and non-equilibrium physics. This review focuses on such recent development, discussing the theoretical foundations of the interactions between Rydberg atoms and the ensuing many-body physics, while providing a critical survey of experimental techniques for their precise manipulation and observation. We further discuss recent breakthroughs in leveraging Rydberg collective effects to probe novel many-body phases and non-equilibrium dynamics of these systems. By synthesizing theoretical insights with experimental milestones, we provide a comprehensive perspective on this rapidly evolving field and its transformative potential for future quantum technologies.
During this thesis, the Physics of interacting systems has been investigated experimentally using Cold Rydberg gases. Rydberg atoms are very excited atoms and have the particularity to interact strongly together through long-range electrostatic interaction. A first highlight of the thesis is a direct experimental observation of a 4-body process. This process consists in internal exchanges of excitations between 4 Rydberg atoms due to their mutual interactions. In addition to its experimental observation, the process has been succefully described theoretically at a quantum level. A second highlight of this thesis has concerns the study of the laser excitation of strongly interacting Rydberg gases. In this regime, many-body quantum correlations play a central role leading to fascinating many-body behavior. In addition to fundamental interests, such systems could be used to implement quantum simulator or non-classical light sources. The system has been investigated during this thesis through the counting statistics of the Rydberg excitation. A highly sub-poisonian, i.e correlated, statistics has been observed in the regim of strong interactions proving the many-body nature of the system. A third highlight of this thesis is the development of an original theoretical model to describe the laser excitation of strongly interacting Rydberg gases. Using the so-called Dicke collective states, it has been possible to catch several interesting features of this many-body problem.
In the last decade the non-equilibrium dynamics of isolated quantum systems has raised a huge interest for both its conceptual and practical implications. Simulation of quantum dynamics represents by now a very active research effort, with highly controllable quantum devices composed of hundreds of qubits already being realized in numerous setups. These offer the unprecedented possibility to access real-time quantum dynamics and strongly correlated quantum many-body states, opening numerous avenues not only for future quantum technologies, but also for long-standing theoretical problems. One of the most sought-after applications is the computation of real-time evolution in theories of fundamental interactions. Since Wilson's proposal in 1974, the equilibrium phase diagrams of lattice gauge theories have been successfully investigated with Monte Carlo simulations in a wide range of parameters. Nonequilibrium properties, on the other hand, cannot be accessed with conventional techniques. Thanks to the recent advances in numerics (e.g. tensor networks) and experiments (quantum simulation), new promising tools are now available for tackling these questions. Remarkable works have already demonstrated that applying these techniques to simple theories, such as one-dimensional quantum electrodynamics, can help to detect the signatures of confinement and pair creation. Despite these impressive achievements, investigating the non-equilibrium dynamics of gauge theories with quantum simulators turned out to be extremely challenging. This is mostly due to the complex constrained dynamics of these theories, which make their simulation with realistic atomic platforms particularly difficult. At the same time, the dynamical constraints can play a key role in determining novel interesting phenomena and peculiar non-equilibrium properties. These phenomena -- which include, for example, quantum scars, fractons, Hilbert space fragmentation -- can lead to anomalous dynamics, eventually evading the paradigm of thermalization, which predicts the relaxation of physical observable to their thermodynamic values. The aim of this thesis is twofold: first, we want to address through a combination of numerical and analytical tools some of the open questions regarding the non-equilibrium dynamics of quantum many-body systems with constrained Hilbert spaces, including lattice gauge theories. In addition, the work reported here is part of a large effort of the community towards the quantum simulation of complex phenomena of condensed matter and high-energy physics.