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Journal of the Physical Society of Japan

Observation of Various Photon Echoes and FID in Ruby by Stark Switching Technique

Shunsuke Nakanishi, O. Tamura, 孝夫 村本, Tsuneo Hashi

Published Oct 1, 1978• 6 citations
Publisher

Abstract

Two-pulse photon echoes, stimulated photon echoes, radiation-locked photon echoes and optical free induction decay (FID) were observed in ruby by using Stark Switching technique and their characteristics were examined. Modulation of FID was found in the off-axis case.
DOI
10.1143/jpsj.45.1437

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Physical Review A•Sep 1, 1980•4 citations
A stimulated photon echo modulation varying in T (separation between the second and third pulses) due to the superhyperfine interaction between a Cr ion and neighboring Al nuclei has been observed in ruby by using a Stark switching technique. The modulation was observed for a time much longer than T 2 , and much higher resolution was obtained than by two-pulse photon echo experiments. An apparent disagreement between theoretical and experimental modulation patterns was noticed in the region where T > T 2 .
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A new method of observing two-photon optical transients is proposed, namely, by intensity switching of incident cw laser beams. This method, which is an alternative to the standard dc Stark or frequency-switching techniques, employs the second-order optical (ac) Stark effect to throw the two-photon active levels in or out of resonance by appropriately switching the intensities of the two laser beams. Theoretical treatment for the three basic transients optical nutation, free induction decay, and two-pulse echo in thin samples using intensity switching, is given for both the cases: co- and counter-propagating beams. The feasibility of the method for the $5{S}_{\frac{1}{2}}\ensuremath{-}3{S}_{\frac{1}{2}}$ transition in Na vapor is demonstrated. An important feature is the apearance of an intensity-dependent beat frequency in the optical FID signal.