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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

DC electric field effect on the magnetic field induced frequency mixing in alkali atoms

Polina V. Mironova, Vitalii D Ovsiannikov, Viacheslav V. Tchernouchkine

Published Mar 1, 2006• 0 citations
Publisher

Abstract

A static electric field may induce essential changes to the cross section for the magnetic-field-induced coherent frecuency mixing of two laser waves, modifying the cross-section dependence on the magnetic field and polarization vectors of incident waves, which depends on the ratio of M1/E2 contributions to n1 2P1/2 (3/2) - n2 2P3/2(1/2) radiation transition amplitude. Relations between the M1/E2 ratio and quantitative characteristics of polarization asymmetry in cross section are determined. Calculated numerical data are presented for coherent mixing of two laser waves on Cs, Rb and K atoms.

DOI
10.1117/12.677973

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A static electric field may induce essential changes to the cross section for the magnetic-field-induced coherent frecuency mixing of two laser waves, modifying the cross-section dependence on the magnetic field and polarization vectors of incident waves, which depends on the ratio of M1/E2 contributions to n1 2P1/2 (3/2) - n2 2P3/2(1/2) radiation transition amplitude. Relations between the M1/E2 ratio and quantitative characteristics of polarization asymmetry in cross section are determined. Calculated numerical data are presented for coherent mixing of two laser waves on Cs, Rb and K atoms.
The effect of a dc electric and (or) magnetic field on the cross section for coherent mixing of two laser waves in atoms is determined. Analytic expressions are obtained for the cross-section dependence on polarisation of incident and generated waves, which allow the measurement of the E2/M1 amplitude ratio Q from the efficiency of a constant-field-induced coherent process for collinear waves. Analytic expressions are also derived for the polarisation dependence of the cross section for frequency mixing in indium and thallium atoms.
Polarization dependence of amplitude for resonant magnetic-field-induced coherent mixing of two collinear laser waves may be used for separating M1 and E2 contributions to n1 2P1/2(3/2) - n2 2P3/2(1/2) dipole-forbidden transition in atoms. The interference between E2 and Ml terms of the amplitude may cause linear polarization and circular dichroism effects. The dependencies of the two effects on the width and splitting of resonance levels, on resonance detuning, on relative directions of steady and alternating field vectors are determined. Numerical data are presented for frequency summation of two laser waves on Cs, Rb and K atoms.
Polarization dependence of amplitude for resonant magnetic-field-induced coherent mixing of two collinear laser waves may be used for separating M 1 and E 2 contributions to n 1 2 P 1/2(3/2) – n 2 2 P 3/2(1/2) dipole-forbidden transition in atoms. In particular, the interference between E 2 and M 1 terms of the amplitude may cause linear polarization and circular dichroism effects. The dependencies of the two polarization effects on the width and splitting of resonance levels, on resonance detuning, on relative directions of steady and alternating field vectors are determined. A static electric field may induce essential changes to the cross section for the magnetic-field-induced mixing, modifying its dependence on the magnetic field and incident wave polarization vectors. Relations between the M 1/ E 2 amplitude ratio and quantitative characteristics of polarization asymmetry in cross section are determined. Numerical data are presented for coherent mixing of two laser waves on Cs, Rb and K atoms.
Steady electric and magnetic fields can stimulate frequency mixing of two laser waves in ensemble of free atoms. In addition to coherence conditions, the steady fields may induce additional resonance singularities essentially enhancing the cross section for scattering the sum-frequency wave. Interference between different components of the electric- and magnetic-field induced frequency summation amplitudes may cause significant effects on the efficiency of conversion. The dependence on the incident wave polarization and the atomic resonance structure is calculated analytically for the frequency mixing in atoms with a singlet structure of the ground and resonance states. Numerical estimates for the quantitative characteristics of the effect are presented for helium, alkali-earth and mercury atoms in their groundn1S0-state in the case of the two-photon resonance on excited singlet states with angular momentum 0, 1, and 2.
The effect is determined of a steady electric or/and magnetic field on coherent frequency mixing of a two-colour radiation in atoms. Analytical formulas for the cross section dependence on polarization have been derived which provide information on a possible way to determining E2/M1 amplitude ratio from the efficiency of the de-field-induced coherent process for collinear laser waves. The polarization-dependent properties of the process’ cross section are determined analytically in the case of Indium and Thallium atoms.
The fine-structure splitting of resonance atomic levels causes essential effects on the amplitude of a two-colour frequency mixing in a magnetic field. The fine-structure effects are analysed in the scattering cross section, and particularly in the circular dichroism phenomena, such as the elliptical polarization of the generated wave, when both incident waves are linearly polarized, and the dependence of the cross section on the helicity of one of the incident waves when the other one is linearly polarized. Together with general analytic expressions for the amplitude, the numerical data are presented for three different double-resonant routes involving two dipole and one quadrupole interactions of atoms with a field. The results may be useful for the polarization control of the process in an atomic vapour and for the frequency-mixing spectroscopic studies of atomic structure.