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Physical Review Letters

Pseudospin symmetry and new collective modes of the Hubbard model

Shoucheng Zhang

Published Jul 2, 1990• 189 citations
Publisher

Abstract

The Hubbard model possesses a SU(2) pseudospin symmetry, which contains the U(1) phase symmetry as a subgroup. The existence of such symmetry leads to interesting experimental consequences if the U(1) phase symmetry is spontaneously broken, i.e., if the ground state is superconducting. In this case, there must exist a pair of massive collective modes which together with the usual Goldstone mode form a triplet representation of the psuedospin group. These collective modes are collisionless and couple directly to external charge disturbances with wave number \ensuremath{\pi} and can therefore be detected experimentally as sharp resonances.

DOI
10.1103/physrevlett.65.120

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The Hubbard model possesses a SU(2) pseudospin symmetry, which contains the U(1) phase symmetry as a subgroup. The existence of such symmetry leads to interesting experimental consequences if the U(1) phase symmetry is spontaneously broken, i.e., if the ground state is superconducting. In this case, there must exist a pair of massive collective modes which together with the usual Goldstone mode form a triplet representation of the psuedospin group. These collective modes are collisionless and couple directly to external charge disturbances with wave number \ensuremath{\pi} and can therefore be detected experimentally as sharp resonances.
In this paper, we discuss the physical consequences of pseudospin SU(2)-symmetry breaking in a negative-U Hubbard model at half-filling. If pseudospin symmetry is spontaneously broken while its unique subgroup U(1) remains invariant, this will lead to a charge-density-wave (CDW) ground state. Furthermore, if the U(1) symmetry is also broken, the ground state will have off-diagonal long-range order, signalling a superconductor. In this case, CDW and superconductivity coexist and form a supersolid. Finally, we show that CDW suppress, but do not destroy superconductivity.
The one band Hubbard model on a bi-partite lattice possess a global SO(4) symmetry group which is a direct product of the spin SU(2) and the pseudospin SU(2) symmetry group. Recently, the group theorectical consequence of this symmetry property has been investigated systematically. It is shown that this symmetry property can be used to reduce the complexity of diagonalizing the Hubbard Hamiltonian, and classify all the eigenstates according to the representation of the SO(4) group. It also leads to an exact one-to-one corespondence of the eigenstates at half-filling to that away from half-filling. Most importantly however, it is shown that this symmetry property leads to a direct experimental prediction for the high Tc superconductivity. If the high Tc superconductivity is correctly described by the Hubbard model, then the SO(4) symmetry dictates the existence of a collective mode that only appears below the superconducting transition temperature. Such a mode can be detected in an electron energy loss experiment as a sharp resonance feature. The location of the peak measure the parameters in the Hubbard model, the intensity is proportional to the superconducting order parameter and the width measures the departure of the Hubbard model from reality.
We make use of a canonical transformation relating the positive U and negative U sectors of the one band Hubbard model to study the global SU(2) pseudospin symmetry in the model, and to investigate the structure of the collective excitation spectrum from a superconducting ground state in the model. New collective modes in this model associated with the SU(2) pseudospin symmetry, recently discussed by Zhang, appear in the pseudo-spinwave spectrum of the transformed problem. Consequences of this mapping for a self dual generalization of the Hubbard model are also discussed.
Motivated by recent experiments on the triangular lattice Mott-Hubbard system $\ensuremath{\kappa}\text{\ensuremath{-}}{(\mathrm{BEDT}\text{\ensuremath{-}}\mathrm{TTF})}_{2}{\mathrm{Cu}}_{2}{(\mathrm{C}\mathrm{N})}_{3}$, we develop a general formalism to investigate quantum spin liquid insulators adjacent to the Mott transition in Hubbard models. This formalism, dubbed the SU(2) slave-rotor formulation, is an extension of the SU(2) gauge theory of the Heisenberg model to the case of the Hubbard model. Furthermore, we propose the honeycomb lattice Hubbard model (at half filling) as a candidate for a spin liquid ground state near the Mott transition; this is an appealing possibility, as this model can be studied via quantum Monte Carlo simulation without a sign problem. The pseudospin symmetry of Hubbard models on bipartite lattices turns out to play a crucial role in our analysis, and we develop our formalism primarily for the case of a bipartite lattice. We also sketch its development for a general Hubbard model. We develop a mean-field theory to describe spin liquids and some competing states, and apply it to the honeycomb lattice. On the insulating side of the Mott transition, we find an SU(2) algebraic spin liquid (ASL), described by gapless S=1∕2S=1∕2S=1∕2 Dirac fermions (spinons) coupled to a fluctuating SU(2) gauge field. This result contrasts with that obtained via a U(1) slave-rotor approach, which instead found a U(1) ASL. That formulation does not respect the pseudospin symmetry, and is therefore not correct on the honeycomb lattice. We construct a low-energy effective theory describing the ASL phase, the conducting semimetal phase and the Mott transition between them. This physics can be detected in numerical simulations via the simultaneous presence of substantial antiferromagnetic and valence-bond solid correlations. In the SU(2) ASL, these observables have slowly decaying fluctuations in space and time, described by power laws with the same critical exponent. We recover the results of the U(1) slave-rotor formulation in the presence of a strong breaking of pseudospin symmetry. Our analysis suggests that both a third-neighbor electron hopping, and/or pseudospin-breaking terms such as a nearest-neighbor density interaction, may help to stabilize a spin liquid phase.