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Journal of the Physical Society of Japan

The Atomic Operators Characteristic of the Split Components in the Study of Resonance Fluorescence from a Two-Level Atom

L. M. Bali, Sharmishtha Roy, Snehlata Kalia

Published Sep 15, 1979• 4 citations
Publisher

Abstract

The atomic operators with characteristic oscillations at the peak frequencies of each of the three split components in the scattering of an intense monochromatic electromagnetic field by a two-level atom are determined. The coupling of the atom-applied-field system with the damping oscillators via these operators is investigated to evaluate the spectrum of the scattered light when the separation of the spectral lines is much larger than their widths.

DOI
10.1143/jpsj.47.903

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The atomic operators with characteristic oscillations at the peak frequencies of each of the three split components in the scattering of an intense monochromatic electromagnetic field by a two-level atom are determined. The coupling of the atom-applied-field system with the damping oscillators via these operators is investigated to evaluate the spectrum of the scattered light when the separation of the spectral lines is much larger than their widths.
The calculation is given of the spectral distribution of resonance fluorescence from an atom that is driven near a j=12j=\frac{1}{2}j=21​ to j=12j=\frac{1}{2}j=21​ transition by a monochromatic, xxx-polarized electric field and that is subject to radiation damping only. In accordance with Mollow's results for a two-level system, the power spectrum of the scattered radiation corresponding to the xxx component of the dipole moment contains a coherent part for all driving-field intensities. The coherent part is absent in the fluorescence radiation corresponding to the yyy and zzz components of the dipole moment. For weak driving fields all power scattered by these latter components is present in a narrow Lorentzian. Consistent with energy conservation, the width of the Lorentzian corresponds to the probability of excitation of the atom out of its ground level due to the presence of the driving field. For strong driving fields the power spectra corresponding to the xxx component and to the yyy or zzz component mainly differ in the heights and widths of their central incoherent band and their Rabi-precession-frequency-shifted side bands.
The spectrum of the resonance fluorescence light from a single two-level atom in a small, high-quality, optical cavity is calculated. The coupling between the atom and cavity is made sufficiently strong compared to the dissipation that single quantum frequency splitting (vacuum Rabi splitting) occurs. Under high excitation qualitatively new fluorescent spectra are predicted. The usual three-peaked resonance fluorescence spectrum now has sidebands whose width is given by the Jaynes-Cummings atom-cavity coupling coefficient rather than by the system dissipation.
The power spectrum of the light scattered by a two-level atom driven near resonance by a monochromatic classical electric field is evaluated. The atom is assumed to relax to equilibrium with the driving field via radiation damping, which is treated by explicitly coupling the atom to the quantized electromagnetic field modes. The power spectrum of the scattered field is directly obtainable from the two-time atomic dipole moment correlation function, which is evaluated by a method based on a Markoff-type assumption analogous to that used to evaluate the time evolution of single-time atomic expectation values.
The phenomenon of resonance fluorescence provides an interesting manifestation of the quantum theory of light and is a “real world” application of the material of the Chapters 8 and 9. In this process, a two-level atom is typically driven by a resonant continuous-wave laser field and the spectral and quantum statistical properties of the fluorescent light emitted by the atom are measured. Experimentally this can be achieved by scattering a laser off a collimated atomic beam such that the directions of the laser beam, atomic beam, and detector axis are mutually perpendicular as shown in Fig. 10.1. If the driving field is monochromatic, then at low excitation intensity the atom absorbs a photon at the excitation frequency and reemits it at the same frequency as a consequence of conservation of energy. The spectral width of the fluorescent light is therefore very narrow. The situation, however, is considerably more complicated when the excitation intensity increases and the Rabi frequency associated with the driving field becomes comparable to, or larger than, the atomic linewidth. At such intensity levels, the Rabi oscillations show up as a modulation of the quantum dipole moment and sidebands start emerging in the spectrum of the emitted radiation. This so-called dynamic Stark splitting is an interesting feature of the atom–field interaction. In addition to that, the fluorescent light exhibits certain nonclassical properties including photon antibunching and squeezing. In this chapter, we develop a theory of resonance fluorescence to explain these phenomena.
The interaction of a two-level atom with two monochromatic electromagnetic fields having arbitrary amplitudes and resonance frequencies is considered. It is shown that the time averaged upper-level population can exceed 0.5 and even reach 0.7. Its dependence on the frequency difference reveals resonance satellite peaks, which are concerned with three- and five-photon combination scattering. The widths and the resonance spectrum shifts of these peaks are found. The frequency spectrum of the spontaneous emission of an atom contains fine structure under some conditions. This structure does not exist in the case of one monochromatic field. An asymmetry in the intensity distribution for the Rabi satellites due to a field non-monochromaticity is predicted.