Compressing the temporal correlation of two photons to the monocycle regime (3.56 fs, center wavelength: 1064 nm) is expected to open up new perspectives in quantum metrology, allowing applications such as submicron quantum optical coherence tomography and novel nonlinear optical experiments. To achieve this, the two-photon state must essentially be ultra-broadband in the frequency domain and ultra-short in the time domain. Here, we report the successful generation of such ultra-broadband, frequency-correlated two-photon states via type-0, cw-pumped (532 nm) spontaneous parametric down conversion using four PPMgSLT crystals with different chirp rates of their poling periods. For the collinear condition, single-photon spectra are detected using a Si-CCD and an InGaAs photodiode array with a monochromator, while for a noncollinear condition, an NbN meander-type superconducting single photon detector (SNSPD) and an InP/GaAs photomultiplier tube (PMT) with a laser line Bragg tunable bandpass filter are used. The broadband sensitivity of the SNSPD and PMT in the near-infrared wavelength range enable singleshot observations with a maximum bandwidth of 820 nm among the four samples. Such spectra can in principle achieve a temporal correlation as short as 1.2 cycles (4.4 fs) with the use of appropriate phase compensation, which can be measured using the sum-frequency signal. We also discuss several detection strategies for measuring coincidence counts in the presence of wavelength-dependent optical elements as a step towards frequency correlation measurements.
Compressing the temporal correlation of two photons to the monocycle regime (3.56 fs, center wavelength: 1064 nm) is expected to open up new perspectives in quantum metrology, allowing applications such as submicron quantum optical coherence tomography and novel nonlinear optical experiments. To achieve this, the two-photon state must essentially be ultra-broadband in the frequency domain and ultra-short in the time domain. Here, we report the successful generation of such ultra-broadband, frequency-correlated two-photon states via type-0, cw-pumped (532 nm) spontaneous parametric down conversion using four PPMgSLT crystals with different chirp rates of their poling periods. For the collinear condition, single-photon spectra are detected using a Si-CCD and an InGaAs photodiode array with a monochromator, while for a noncollinear condition, an NbN meander-type superconducting single photon detector (SNSPD) and an InP/GaAs photomultiplier tube (PMT) with a laser line Bragg tunable bandpass filter are used. The broadband sensitivity of the SNSPD and PMT in the near-infrared wavelength range enable singleshot observations with a maximum bandwidth of 820 nm among the four samples. Such spectra can in principle achieve a temporal correlation as short as 1.2 cycles (4.4 fs) with the use of appropriate phase compensation, which can be measured using the sum-frequency signal. We also discuss several detection strategies for measuring coincidence counts in the presence of wavelength-dependent optical elements as a step towards frequency correlation measurements.
Quantum entanglement of two photons created by spontaneous parametric downconversion (SPDC) can be used to probe quantum optical phenomena during a single cycle of light. Harris [Opt. Express 98, 063602 (2007)] suggested using ultrabroad parametric fluorescenc generated from a quasi-phase-matched (QPM) device whose poling period is chirped. In the Harris's original proposal, it is assumed that the photons are collinearly generated and then spatially separated by frequency filtering Here, we alternatively propose using noncollinearly generated SPDC. In our numerical calculation, to achieve 1.2 cycle temporal correlation for a 532 nm pump laser, only 10% -chirped device is sufficien when noncollinear condition is applied, while a largely chirped (50%) device is required in collinear condition. We also experimentally demonstrate an octave-spanning (790-1610 nm) noncollinear parametric fluorescenc from a 10% chirped MgSLT crystal using both a superconducting nanowire single-photon detector and photomultiplier tube as photon detectors. The observed SPDC bandwidth is 194 THz, which is the largest width achieved to date for a chirped QPM device. From this experimental result, our numerical analysis predicts that the bi-photon can be compressed to 1.2 cycles with appropriate phase compensation.
The frequency entangled biphoton source generated via spontaneous parametric down-conversion (SPDC) process has found important applications in the fields of quantum clock synchronization, quantum communication, quantum information processing, etc. As quantum technologies evolve, quantitative characterization of the frequency entanglement becomes necessary and has been implemented by measuring the spectral properties of the biphoton state. However, due to the high dark rate and low quantum efficiency of the InGaAs single-photon detectors, direct measurement of the spectral properties of the biphoton state at optical communication wavelength is hard to implement. In this paper, we report the measurement of the spectral properties of a biphoton state at optical communication wavelength which is generated from periodically poled potassium titanyl phosphate (PPKTP) pumped by an ultra-short pulsed optical source at 787 nm. Based on the coincidence measurement setup together with two infrared spectrometers, the spectra of the signal and idler photons are obtained with their center wavelengths being 1574.4 nm and 1574.9 nm, while their 3-dB bandwidths being 35.3 nm and 37.6 nm respectively. The joint spectrum of the photon pair is observed as well and shows a coincident-frequency entanglement and a joint spectrum bandwidth of 3 nm. According to the ratio of the single-photon spectral bandwidth to the joint spectral bandwidth of the photon pairs, the degree of frequency entanglement is quantified to be 12, denoting a relatively high quality of the entanglement.
The state-of-art technology of a quasi-phase matched (QPM) device has enabled the efficient generation of frequency-entangled photon pairs through parametric fluorescence [1, 2]. Harris [3] has proposed the generation of photon pairs which are correlated on a mono-cycle time scale of optical period. In that paper, the poling period of QPM device is linearly chirped (increased) from the entrance to the exit. Thus, each poling period is phase matched at different wavelengths of photon pairs, spanning ultra-broad spectrum. Recent experiment by Mohan et al as its application to quantum optical coherence tomography [4], has realized the parametric fluorescence from chirped-QPM device which is phase matched from 820nm to 1500nm using stoichiometric lithium tantalate (SLT) crystal as a nonlinear medium with 13% chirping (poling period: from 7.500µm to 8.500µm).
Ultra-broadband frequency entangled biphotons have exceptionally short temporal duration and can achieve narrow Hong–Ou–Mandel (HOM) interference patterns, making them vital for quantum metrology applications. However, the bandwidth of previously demonstrated biphotons used for HOM interference has been limited to less than 400 nm, which is not wide enough to achieve ultra-high precision in quantum metrology. In order to push the precision to its limit, we have theoretically designed a 20-mm-long chirped periodically poled lithium niobate (CPPLN) crystal with type-II phase matching. Pumped by a 405 nm laser, the down-converted signal and idler photons can cover the wavelength range from 420 to 5200 nm, approaching the transparent upper bound of the LN crystal. In the simulated Hong–Ou–Mandel (HOM) interference, the full-width at half-maximum of the interference pattern is 965 attoseconds, with a visibility of 99.44%. Following a similar approach, we also designed a type-0 CPPLN crystal to achieve higher brightness. These ultra-broadband biphoton sources can generate ultra-narrow quantum interference patterns, which have the potential for attosecond-level high-precision quantum metrology.
The frequency entangled photon pairs generated by spontaneous parametric down-conversion (SPDC) possess wide applications in quantum optics and relevant fields.To facilitate the practical quantum information technologies,particularly in optical fiber links,a frequency entangled source at telecommunication wavelength with features of compactness,portability,high efficiency and miniaturization is highly desired.In this paper,we report the experimental generation of a miniaturized frequency entangled source in telecommunication band from a 10 mm-long type-Ⅱ periodically poled lithium niobate (PPLN) waveguide pumped by a 780 nm distributed Bragg reflector (DBR) laser diode.The frequency entangled photon pairs generated by SPDC possess wide applications in quantum optics and relevant fields.When the DBR laser diode is driven by a current of 170 mA at a temperature controlled to 20℃,the output power is measured to be 70.4 mW with a central wavelength of 780.585 nm.Under this pump,the orthogonally-polarized photon pairs are generated and output from the PPLN waveguide.After filtering out the remaining pump by three high-performance long-pass filters mounted on an adjustable U-type fiber bench,the photon-pair generation rate,spectral and temporal properties of the generated frequency entangled source are measured.The results show that the generation rate of the photon pairs,after being corrected for the detection efficiencies of the single photon detectors and the optical losses,is achieved to be 1.86×107 s-1 at a pump power of 44.9 mW (coupled into the waveguide).Optimizing the working temperature of the waveguide and fixing it at 46.5℃,the frequency degeneracy of the SPDC generated photon pairs is realized.Based on the coincidence measurement setup together with two infrared spectrometers,the spectra of the signal and idler photons are obtained with their center wavelengths of 1561.43 nm and 1561.45 nm,and their 3-dB bandwidths of 3.62 nm and 3.60 nm respectively.The joint spectrum of the photon pair is observed,showing a joint spectrum bandwidth of 3.18 nm.The degree of frequency entanglement is quantified to be 1.13 according to the bandwidth ratio between the single photon spectrum and the joint spectrum.Furthermore,based on the Hong-Ou-Mandel (HOM) interferometric coincidence measurement setup,a visibility of about 96.1% is observed,which indicates the very good frequency indistinguishibility of the down-converted biphotons.The measured 3-dB width of the HOM dip is 1.47 ps and shows good agreement with the measured single-photon spectral bandwidth.The experimental results lay a solid foundation for developing portable,miniaturized frequency entangled sources at telecommunication band for the further applications in quantum information areas,such as quantum time synchronization.
Broadband quantum light is a vital resource for quantum metrology and spectroscopy applications such as quantum optical coherence tomography or entangled two photon absorption. For entangled two photon absorption in particular, very high photon flux combined with high time-frequency entanglement is crucial for observing a signal. So far these conditions could be met by using high power lasers driving degenerate, type 0 bulk-crystal spontaneous parametric down conversion (SPDC) sources. This naturally limits the available wavelength ranges and precludes deterministic splitting of the generated output photons. In this work we demonstrate an integrated two-colour SPDC source utilising a group-velocity matched lithium niobate waveguide, reaching both exceptional brightness 1.52⋅10 6 pairssmWGHz and large bandwidth (7.8 THz FWHM) while pumped with a few mW of continuous wave (CW) laser light. By converting a narrow band pump to broadband pulses the created photon pairs show correlation times of Δ τ ≈ 120 fs while maintaining the narrow bandwidth Δ ω p ≪ 1 MHz of the CW pump light, yielding strong time-frequency entanglement. Furthermore our process can be adapted to a wide range of central wavelengths.