Ultra-broadband frequency entangled biphotons have exceptionally short temporal duration and can achieve narrow Hong–Ou–Mandel (HOM) interference patterns, making them vital for quantum metrology applications. However, the bandwidth of previously demonstrated biphotons used for HOM interference has been limited to less than 400 nm, which is not wide enough to achieve ultra-high precision in quantum metrology. In order to push the precision to its limit, we have theoretically designed a 20-mm-long chirped periodically poled lithium niobate (CPPLN) crystal with type-II phase matching. Pumped by a 405 nm laser, the down-converted signal and idler photons can cover the wavelength range from 420 to 5200 nm, approaching the transparent upper bound of the LN crystal. In the simulated Hong–Ou–Mandel (HOM) interference, the full-width at half-maximum of the interference pattern is 965 attoseconds, with a visibility of 99.44%. Following a similar approach, we also designed a type-0 CPPLN crystal to achieve higher brightness. These ultra-broadband biphoton sources can generate ultra-narrow quantum interference patterns, which have the potential for attosecond-level high-precision quantum metrology.
Ultra-broadband frequency entangled biphotons have exceptionally short temporal duration and can achieve narrow Hong–Ou–Mandel (HOM) interference patterns, making them vital for quantum metrology applications. However, the bandwidth of previously demonstrated biphotons used for HOM interference has been limited to less than 400 nm, which is not wide enough to achieve ultra-high precision in quantum metrology. In order to push the precision to its limit, we have theoretically designed a 20-mm-long chirped periodically poled lithium niobate (CPPLN) crystal with type-II phase matching. Pumped by a 405 nm laser, the down-converted signal and idler photons can cover the wavelength range from 420 to 5200 nm, approaching the transparent upper bound of the LN crystal. In the simulated Hong–Ou–Mandel (HOM) interference, the full-width at half-maximum of the interference pattern is 965 attoseconds, with a visibility of 99.44%. Following a similar approach, we also designed a type-0 CPPLN crystal to achieve higher brightness. These ultra-broadband biphoton sources can generate ultra-narrow quantum interference patterns, which have the potential for attosecond-level high-precision quantum metrology.
Broadband nonlinear optical devices play a critical role in both classical and quantum optics. Here, we design and fabricate a 6.82-mm-long step-chirped periodically poled lithium niobate~(CPPLN) waveguide on lithium niobate on insulator, which enables quasi-phase matching over a broad bandwidth for second-harmonic generation~(SHG) and spontaneous parametric down-conversion~(SPDC). The SHG achieves an average efficiency of 54.4\%/W/cm2 over the first-harmonic wavelength range of 1510~nm-1620~nm, paving the way for realizing SPDC across a wide range of pump wavelengths. For SPDC, by tuning the pump wavelength to 775~nm, 780~nm, and 785~nm, we achieve broadband photon-pair generation with a maximum full bandwidth and brightness up to 99~THz~(846~nm) and 20~GHz/mW/nm, respectively. Our findings provide an efficient and experiment-friendly approach for generating broadband photon pairs, which holds significant promise for advancing applications in quantum metrology.
Broadband nonlinear optical devices play a critical role in both classical and quantum optics. Here, we design and fabricate a 6.82-mm-long step-chirped periodically poled lithium niobate (CPPLN) waveguide on lithium niobate on insulator, which enables quasi-phase matching over a broad bandwidth for second-harmonic generation (SHG) and spontaneous parametric down-conversion (SPDC). The SHG achieves an average efficiency of 91%/W/cm 2 over the first-harmonic wavelength range of 1510 nm–1620 nm, paving the way for realizing SPDC across a wide range of pump wavelengths. For SPDC, by tuning the pump wavelength to 775 nm, 780 nm, and 785 nm, we achieve broadband photon-pair generation with a maximum full bandwidth and brightness up to 99 THz (846 nm) and 21 MHz/mW/nm, respectively. Our findings provide an efficient and experiment-friendly approach for generating broadband photon pairs, which holds significant promise for advancing applications in quantum metrology.
The time-energy entangled photon source is a core resource in quantum key distribution, quantum teleportation, and quantum metrology. The output of orthogonally polarized photon pairs can enhance the effective coincidence counts of the entangled source in these applications. Additionally, an all-fiber entangled source offers small size and high mobility advantages. However, most current orthogonally polarized all-fiber time-energy entangled sources are limited to a bandwidth of around 1 nm, which is detrimental to the effective utilization of channel resources in fiber networks and restricts precision in quantum metrology. To address this issue, we employ a fiber-coupled 775 nm narrow linewidth pump laser in a periodically poled lithium niobate (PPLN) waveguide to achieve type-II spontaneous parametric down-conversion (SPDC). This results in an all-fiber orthogonally polarized time-energy entangled photon source with a bandwidth greater than 7 nm. We measured the single counts, coincidence counts, coincidence to accidental coincidence ratio (CAR), single photon spectra, and joint spectral intensity of the entangled source, calculating the Schmidt number S = 7.8. Furthermore, we measured Hong-Ou-Mandel (HOM) interference by inserting two 2 nm bandpass filters, and the interference visibility remained around 95.8% after continuous operation for 3 hours. The experimental results indicate that while maintaining an all-fiber structure, this source possesses a broadband range, low noise, and high stability, providing efficient and reliable biphoton resources for applications in quantum communication, quantum networks, and precision metrology.
Many optical quantum applications rely on broadband frequency correlated photon pair sources. We previously reported a scheme for collinear emission of high-efficiency and ultra-broadband photon pairs using chirped quasi-phase matching (QPM) periodically poled stoichiometric lithium tantalate (PPSLT) ridge waveguides. However, collinearly emitted photon pairs cannot be directly adopted for applications that are based on two-photon interference, such as quantum optical coherence tomography (QOCT). In this work, we developed a chirped QPM device with a slab waveguide structure. This device was designed to produce spatially separable (photon pair non-collinear emission) parametric fluorescence photon pairs with an ultra-broadband bandwidth in an extremely efficient manner. Using a non-chirped QPM slab waveguide, we observed a photon pair spectrum with a full-width-at-half-maximum (FWHM) bandwidth of 26 nm. When using a 3% chirped QPM slab waveguide, the FWHM bandwidth of the spectrum increased to 190 nm, and the base-to-base width is 308 nm. We also confirmed a generation efficiency of 2.4×10 6 pairs/( μ W·s) using the non-chirped device, and a efficiency of 8×10 5 pairs/( μ W·s) using the 3% chirped device under non-collinear emission conditions after single-mode fiber coupling. This is, to the best of our knowledge, the first report of frequency correlated photon pairs generation using slab waveguide device as a source. In addition, using slab waveguides as photon pair sources, we performed two-photon interference experiments with the non-chirped device and obtained a Hong–Ou–Mandel (HOM) dip with a FWHM of 7.7 μ m and visibility of 98%. When using the 3% chirped device as photon pair source, the HOM measurement gave a 2 μ m FWHM dip and 74% visibility.
Two-photon interference, commonly known as Hong-Ou-Mandel (HOM) interference [1] , has attracted a great deal of interest in quantum sensing, including the precision timing measurements [2] and quantum optical coherence tomography [3] . While the dip of the HOM interference is the direct measure of the purity of the single-photon, the width of the HOM dip relates to the coherence time of the interfering photons. The broad consensus for using the HOM interferometer for sensing application remained the HOM dip width as the limiting factor for the precision measurements. As a consequence, the ultra-broadband photon sources have long been hailed as a vital prerequisite for ultra-precise HOM interferometry. Here, we have studied the variation in the width of the HOM dip with the crystal length for the continuous-wave pump laser and measured the HOM dip as low as 8.2 ± 0.2 µm corresponding to the spectral width of the single-photon source of 79.6±1.9 nm useful for sensitive sensing applications.
Entanglement swapping enables the distribution of quantum states over long distances. In this protocol, a Bell state measurement projects photons, which were created in separate entangled photon sources, into an entangled state when their corresponding pairs interfere at a beamsplitter. This process is optimally realized when the photons are indistinguishable in all degrees of freedom, resulting in Hong-Ou-Mandel (HOM) interference. Since its initial proposal by [1], several experimental realizations have used pulsed, synchronized pumps, as in [2] to achieve temporal indistiguishability. In the case of continuous wave (CW) pumping, the sources are not synchronized, requiring post-selection of the coincidence events after detection. This requires detectors with a temporal resolution greater than the coherence time of the photons. Previous experiments have successfully observed HOM interference using periodically poled Lithium Niobate (ppLN) waveguides and superconducting nanowire single-photon detectors (SNSPDs) [3], also with hybrid sources to improve coincidence rates and HOM visibility [4], [5].