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Physical Review A

Self-organized patterns and spatial solitons in liquid-crystal microcavities

Sjoerd Hoogland, Jeremy J. Baumberg, S. Coyle, Joanne C. Baggett, M. J. Coles, Harry J. Coles

Published Nov 8, 2002• 32 citations
Publisher

Abstract

Single-mode microcavities filled with liquid crystals are predominantly nonlinear refractive optical elements. Pumped by lasers tuned above the filled cavity resonance frequency, we show that the phenomena of bistability, spatial pattern formation, and ``optical bullet holes'' appear even in a single-mode microcavity configuration. The solitons have an unexpected dark spatial profile and appear only beyond the bistability threshold.

DOI
10.1103/physreva.66.055801

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Optical bistability and bright and dark resonator solitons exist in semiconductor resonator at room temperature [C.O. Weis and Ye. Larionova, Rep. Prog. Phys. 70 (2007) 255-335], with the usual semiconductor nonlinearity. At low temperature in the strong coupling regime between quantum well excitons and the optical field in a semiconductor microcavity the nonlinearities are strong and based on “polariton nonlinearity”. The strong coupling results in a quasi-particle “exciton-polariton” which gives access to positive and negative reactive and dissipative optical nonlinearities, as opposed to the usual room temperature semiconductor nonlinearities possessing essentially only one sign. The type of nonlinearity and the properties of solitons can be varied widely by the detuning between the photon- and exciton resonances. We show for the first time experimentally the existence of patterns, bright and dark solitons based on polariton nonlinearity. 1. INTRODUCTION Bright and dark spatial solitons were shown to exist in such microresonators with and without population inversion [1-3]. At room temperature the nonlinearity which is at the origin of the soliton existence is the usual mixed absorptive/refractive semiconductor nonlinearity which can have transverse effects (e.g. self-focusing) and longitudinal effects such as nonlinear resonance, both ingredients for soliton stability. At low temperature (or at large exciton binding energies) the exciton, which merges with the absorption band at room temperature, is well separated spectrally from the absorption band so that the nonlinearity becomes that of a 2-level system. If the exciton resonance is strongly coupled with the field inside a resonator the exciton- and the photon resonances mix. At coincidence of the two resonance frequencies, the photon- and the exciton resonances hybridize in an avoided crossing and the two hybrid resonances are ascribed to a quasi-particle, the excitonpolariton. This quasi-particle has unusual optical properties. E.g. is the photon nonlinearity determined by exciton collisions. That the exciton-polariton system has interesting nonlinearities (e.g. induced absorption as opposed to the usual saturable absorption) has been shown previously [4]. It was realized that semiconductor microresonators in the strong field-exciton coupling regime might show optical bistability and first experimental proofs for bistability were given recently [5]. As optical bistability of a resonator is a precondition for the existence of spatial resonator solitons, the question arises whether semiconductor microresonators with polariton nonlinearity can support spatial resonator solitons, which, as a consequence of the large nonlinearity of the polaritons, could be expected to exist at rather small light intensities, as it is of importance for all applications. 2. EXPERIMENTAL ARRANGEMENT AND RESULTS The cooled resonator sample (4 K) is illuminated by light at the polariton resonance wavelengths, and the light reflected from the resonator is observed. The light source is a Ar

•Jan 1, 2007•0 citations
Single-mode microcavities filled with liquid crystals are predominantly nonlinear refractive optical elements. Pumped by lasers tuned above the filled cavity resonance frequency, we show that the phenomena of bistability, spatial pattern formation, and ``optical bullet holes'' appear even in a single-mode microcavity configuration. The solitons have an unexpected dark spatial profile and appear only beyond the bistability threshold.
When atoms scatter photons from a transverse laser into a high-finesse optical cavity, they form crystalline structures which maximize the intracavity light field and trap the atoms in the ordered array. Stable organization occurs when the laser field amplitude exceeds a certain threshold. For planar single-mode cavities there exist two equivalent possible atomic patterns, which determine the phase of the intracavity light field. Under these premises, we show that the effect of an additional laser pumping the cavity makes one pattern more favorable than the other and that it can dynamically force the system into a predetermined configuration. This is an instance of pattern formation and seeding in a nonlinear quantum-optical system.
We show experimentally optical bistability and the existence of bright and dark resonator solitons in the strong coupling regime between quantum-well excitons and the optical field in a semiconductor microcavity. The strong coupling results in a quasi-particle exciton-polariton, which gives access to positive and negative reactive and dissipative optical nonlinearities, as opposed to the usual room temperature semiconductor nonlinearities possessing essentially only one sign. The existence range and the properties of solitons can be varied widely by the detuning between polariton states and light frequency.
The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity.In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms.The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity.We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory.At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition.We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry.In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.
Optical bistability and bright and dark resonator solitons exist in semiconductor resonator at room temperature [C.O. Weis and Ye. Larionova, Rep. Prog. Phys. 70 (2007) 255-335], with the usual semiconductor nonlinearity. At low temperature in the strong coupling regime between quantum well excitons and the optical field in a semiconductor microcavity the nonlinearities are strong and based on “polariton nonlinearity”. The strong coupling results in a quasi-particle “exciton-polariton” which gives access to positive and negative reactive and dissipative optical nonlinearities, as opposed to the usual room temperature semiconductor nonlinearities possessing essentially only one sign. The type of nonlinearity and the properties of solitons can be varied widely by the detuning between the photon- and exciton resonances. We show for the first time experimentally the existence of patterns, bright and dark solitons based on polariton nonlinearity. 1. INTRODUCTION Bright and dark spatial solitons were shown to exist in such microresonators with and without population inversion [1-3]. At room temperature the nonlinearity which is at the origin of the soliton existence is the usual mixed absorptive/refractive semiconductor nonlinearity which can have transverse effects (e.g. self-focusing) and longitudinal effects such as nonlinear resonance, both ingredients for soliton stability. At low temperature (or at large exciton binding energies) the exciton, which merges with the absorption band at room temperature, is well separated spectrally from the absorption band so that the nonlinearity becomes that of a 2-level system. If the exciton resonance is strongly coupled with the field inside a resonator the exciton- and the photon resonances mix. At coincidence of the two resonance frequencies, the photon- and the exciton resonances hybridize in an avoided crossing and the two hybrid resonances are ascribed to a quasi-particle, the excitonpolariton. This quasi-particle has unusual optical properties. E.g. is the photon nonlinearity determined by exciton collisions. That the exciton-polariton system has interesting nonlinearities (e.g. induced absorption as opposed to the usual saturable absorption) has been shown previously [4]. It was realized that semiconductor microresonators in the strong field-exciton coupling regime might show optical bistability and first experimental proofs for bistability were given recently [5]. As optical bistability of a resonator is a precondition for the existence of spatial resonator solitons, the question arises whether semiconductor microresonators with polariton nonlinearity can support spatial resonator solitons, which, as a consequence of the large nonlinearity of the polaritons, could be expected to exist at rather small light intensities, as it is of importance for all applications. 2. EXPERIMENTAL ARRANGEMENT AND RESULTS The cooled resonator sample (4 K) is illuminated by light at the polariton resonance wavelengths, and the light reflected from the resonator is observed. The light source is a Ar