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Soviet Journal of Quantum Electronics

Self-reversal of the wavefront of high-power radiation in a light-induced four-wave interaction in a resonant medium

Pavel A Apanasevich, Anatolii A Afanas'ev, S. Ya. Kilin

Published Apr 30, 1985• 1 citation
Publisher

Abstract

A wavefront reversal system is proposed for high-power optical radiation. This system is based on a resonant four-wave interaction without recourse to external pump waves. Stimulated scattering of the wave being reversed in a resonant medium placed inside a resonator creates two opposite pump waves and a parametric interaction between them generates reversed radiation. The efficiency of such self-reversal is comparable with the efficiency of conventional wavefront reversal as a result of a four-wave interaction in nonresonant media with a phase nonlinearity and it may reach 10 −3 .

DOI
10.1070/qe1985v015n04abeh007000

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A wavefront reversal system is proposed for high-power optical radiation. This system is based on a resonant four-wave interaction without recourse to external pump waves. Stimulated scattering of the wave being reversed in a resonant medium placed inside a resonator creates two opposite pump waves and a parametric interaction between them generates reversed radiation. The efficiency of such self-reversal is comparable with the efficiency of conventional wavefront reversal as a result of a four-wave interaction in nonresonant media with a phase nonlinearity and it may reach 10 −3 .
An investigation is made of wavefront reversal of optical radiation in a nondegenerate four-wave interaction in a resonant medium. It is shown that for a pump intensity comparable with the saturation intensity of the absorption line of the resonant medium, the reversed wave spectrum has two side peaks positioned symmetrically relative to the central peak which corresponds to a degenerate interaction. These side peaks are attributable to regions of negative absorption (amplification) of weak radiation by the resonant medium situated in a high-power field of opposite pump waves. The dependences of the magnitudes and positions of these peaks on the pump intensity can be used to control the spectral and energy characteristics of the reflected radiation. The conditions for self-excitation of a reversing system based on resonant four-wave interaction are determined. In particular, the ranges of the pump intensity and the optical density of the resonant medium in which self-excitation of the reversing system may occur, are determined for a degenerate interaction.
Equations describing a transient degenerate four-wave interaction in a resonant medium are derived and solved numerically. The approximation of a "following" nonlinear polarization state is used to determine the range of values of the parameters of the medium and the radiation field in which the efficiency of a transient four-wave interaction is higher than that of the steady-state process. It is found that amplification of weak radiation as a result of transient energy exchange can only be achieved in the four-wave interaction for different pump wave intensities.
A theoretical analysis is made of wavefront reversal which is not sensitive to the optical quality of the nonlinear wavefront-reversing medium when complex-conjugate reference waves are formed spontaneously. An investigation is made of the linear and nonlinear stages of reversed wave generation in various nonlinear media using feedback in degenerate and nondegenerate four-wave interaction. It is shown that in nonamplifying nonlinear media this method can only be achieved by additional amplification of the radiation reflected from the nonlinear medium.
A system for phase conjugation of Stokes radiation by a four-wave interaction involving intracavity stimulated Raman scattering (STRS) in a Raman-active medium with a nonresonant nonlinearity. This method can be used in construction of high-power sources of highly directional Stokes radiation on the basis of round-trip STRS amplifiers coupled to a phase-conjugating element. It is shown that an STRS converter utilizing organic liquids and subjected to laser pumping of less than 100 MW/cm2 intensity inside a resonator can ensure a highly efficient phase conjugation with a peak reflection coefficient in excess of unity. Depending on the ratio of the Raman and nonresonant susceptibilities of a medium, there is an optimal value of the coefficient representing the degree of conversion of laser pump radiation into STRS radiation, which ensures the maximum phase conjugation efficiency.