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Physical Review A

Cavity-perturbed strong-field resonance fluorescence

A. Lezama, Yifu Zhu, S. Morin, THOMAS W. MOSSBERG

Published Mar 1, 1989• 26 citations
Publisher

Abstract

The spectrum of light emitted out the sides of a confocal mode-degenerate optical cavity by Ba atoms driven by a strong, resonant, excitation field has been studied. The cavity is found to induce asymmetries in the classic three-peaked Mollow spectrum. These asymmetries are explained primarily in terms of a spectral structure introduced into the electromagnetic vacuum reservoir by the cavity.

DOI
10.1103/physreva.39.2754

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Effect of optical gain on the fluorescence of two-level atoms into the modes of an optical cavity

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The emission of strongly driven two-level-like Ba atoms into the modes of an optical cavity has been studied as a function of cavity tuning and Ba density. At low densities, the cavity-mode emission viewed as a function of cavity tuning is identical in form to the three-peaked Mollow emission spectrum. At high densities, however, the cavity-mode emission is strongly amplified (attenuated) when the cavity is tuned to the frequency of one (the other) Mollow sideband. It is predicted that modest increases in Ba density will cause lasing to occur in this system.

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Spectra of the atomic resonance fluorescence and of the cavity-transmitted light in a driven Jaynes-Cummings system are studied theoretically, where the cavity is driven by a classical field of arbitrary strength. In the regime of strong atom-cavity coupling, anomalous resonance peaks occur at $\ifmmode\pm\else\textpm\fi{}\sqrt{n}{g}^{\ensuremath{'}} (n=2,3,\dots{}),$ with the modified vacuum Rabi frequency ${g}^{\ensuremath{'}},$ both in the atomic fluorescence and the cavity transmission. These peaks as well as the observed shift of the vacuum Rabi splitting are explained in terms of the quasienergy levels induced dynamically by the strong driving field. For a stronger driving field, it is shown that the spectrum of the cavity transmission deviates from that of the atomic fluorescence. In the presence of significant damping, the spectrum of the cavity transmission approaches a singlet structure in the strong driving-field limit, and it is found additionally that a bimodal photon-number distribution, which results in a unique quintuplet spectrum of the atomic fluorescence, does not show up in the cavity transmission.

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Summary form only given. The problem of an atom driven by a strong laser was first investigated theoretically in 1969 by B.R. Mollow. He discovered that the resonance fluorescence spectrum has a three-peaked structure with the central peak being more pronounced than the two side peaks. The common Mollow triplet fluorescence pattern can be altered in many ways, by making adjustments to the system. The system can be placed in a squeezed vacuum, the atom can be placed in a cavity, or a bichromatic field can be used instead of a monochromatic laser. These alterations all have an effect on the resulting resonance fluorescence and probe absorption spectra. Other interesting modifications occur when the atom interacts with a stochastic field as well as a laser. The previous approaches were numerical. Here we also obtain analytic solutions (in certain limits) which provide additional insight.

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The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.

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Nature Photonics•Jan 10, 2024•26 citations
The spectrum of light emitted out the sides of a confocal mode-degenerate optical cavity by Ba atoms driven by a strong, resonant, excitation field has been studied. The cavity is found to induce asymmetries in the classic three-peaked Mollow spectrum. These asymmetries are explained primarily in terms of a spectral structure introduced into the electromagnetic vacuum reservoir by the cavity.
The emission of strongly driven two-level-like Ba atoms into the modes of an optical cavity has been studied as a function of cavity tuning and Ba density. At low densities, the cavity-mode emission viewed as a function of cavity tuning is identical in form to the three-peaked Mollow emission spectrum. At high densities, however, the cavity-mode emission is strongly amplified (attenuated) when the cavity is tuned to the frequency of one (the other) Mollow sideband. It is predicted that modest increases in Ba density will cause lasing to occur in this system.
Spectra of the atomic resonance fluorescence and of the cavity-transmitted light in a driven Jaynes-Cummings system are studied theoretically, where the cavity is driven by a classical field of arbitrary strength. In the regime of strong atom-cavity coupling, anomalous resonance peaks occur at $\ifmmode\pm\else\textpm\fi{}\sqrt{n}{g}^{\ensuremath{'}} (n=2,3,\dots{}),$ with the modified vacuum Rabi frequency ${g}^{\ensuremath{'}},$ both in the atomic fluorescence and the cavity transmission. These peaks as well as the observed shift of the vacuum Rabi splitting are explained in terms of the quasienergy levels induced dynamically by the strong driving field. For a stronger driving field, it is shown that the spectrum of the cavity transmission deviates from that of the atomic fluorescence. In the presence of significant damping, the spectrum of the cavity transmission approaches a singlet structure in the strong driving-field limit, and it is found additionally that a bimodal photon-number distribution, which results in a unique quintuplet spectrum of the atomic fluorescence, does not show up in the cavity transmission.
Summary form only given. The problem of an atom driven by a strong laser was first investigated theoretically in 1969 by B.R. Mollow. He discovered that the resonance fluorescence spectrum has a three-peaked structure with the central peak being more pronounced than the two side peaks. The common Mollow triplet fluorescence pattern can be altered in many ways, by making adjustments to the system. The system can be placed in a squeezed vacuum, the atom can be placed in a cavity, or a bichromatic field can be used instead of a monochromatic laser. These alterations all have an effect on the resulting resonance fluorescence and probe absorption spectra. Other interesting modifications occur when the atom interacts with a stochastic field as well as a laser. The previous approaches were numerical. Here we also obtain analytic solutions (in certain limits) which provide additional insight.
The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.
We calculate the steady-state spectrum of resonance fluorescence from a two-level atom coupled to a single cavity mode and driven by a strong, in general off-resonance, external field. In the strong-coupling limit, each Mollow triplet component is split into a multiplet, whose detailed structure depends on the atom–cavity coupling, the cavity and spontaneous emission decay constants, and the photon-number distribution of the cavity mode. The dressed states for this system are identified, and the spectral features are interpreted in terms of transitions among these dressed states. In particular, we find that the central component of the central multiplet can have a strongly subnatural linewidth.
Abstract The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.