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Journal of Modern Optics

Quantum dynamics of two quantum dots in the vicinity of a photonic band edge: role of structured reservoirs and phonons

C. Roy

Published Apr 10, 2010• 0 citations
Publisher

Abstract

We study the population and disentanglement dynamics of two identical quantum dots placed inside the structured electromagnetic reservoir of a photonic crystal and coupled to an independent bath of thermal phonons. A formalism based on the method of generalized-Laplace transforms is developed to study the population and disentanglement dynamics. The effect of resonant dipole dipole interaction between the two quantum dots on the population dynamics in the presence of phonons and shows that the two two-level atoms can have a residual population at long times in the structured reservoir of a photonic crystal due to the formation of a photon-atom bound state. The disentanglement dynamics of the two quantum dots (assumed to be initially entangled) is studied using concurrence as a measure and is computed from the reduced two two-level system density matrix using the method of generalized-Laplace transforms. We show that partial disentanglement results from the interaction of the two quantum dots with the electromagnetic and phonon reservoirs. However, substantial entanglement is preserved in the fractionalized steady state formed if the transition frequency of two the quantum dots lies in the vicinity of the photonic band edge. We also discuss in detail the role of acoustic phonons on the population and disentanglement dynamics and the long time residual entanglement.

DOI
10.1080/09500341003789918

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We study the population and disentanglement dynamics of two identical quantum dots placed inside the structured electromagnetic reservoir of a photonic crystal and coupled to an independent bath of thermal phonons. A formalism based on the method of generalized-Laplace transforms is developed to study the population and disentanglement dynamics. The effect of resonant dipole dipole interaction between the two quantum dots on the population dynamics in the presence of phonons and shows that the two two-level atoms can have a residual population at long times in the structured reservoir of a photonic crystal due to the formation of a photon-atom bound state. The disentanglement dynamics of the two quantum dots (assumed to be initially entangled) is studied using concurrence as a measure and is computed from the reduced two two-level system density matrix using the method of generalized-Laplace transforms. We show that partial disentanglement results from the interaction of the two quantum dots with the electromagnetic and phonon reservoirs. However, substantial entanglement is preserved in the fractionalized steady state formed if the transition frequency of two the quantum dots lies in the vicinity of the photonic band edge. We also discuss in detail the role of acoustic phonons on the population and disentanglement dynamics and the long time residual entanglement.
In this thesis we study the role of nonradiative degrees of freedom on quantum optical properties of mesoscopic quantum dots placed in the structured electromagnetic reservoir of a photonic crystal. We derive a quantum theory of the role of acoustic and optical phonons in modifying the optical absorption lineshape, polarization dynamics, and population dynamics of a two-level atom (quantum dot) in the ``colored" electromagnetic vacuum of a photonic band gap (PBG) material. This is based on a microscopic Hamiltonian describing both radiative and vibrational processes quantum mechanically. Phonon sidebands in an ordinary electromagnetic reservoir are recaptured in a simple model of optical phonons using a mean-field factorization of the atomic and lattice displacement operators. Our formalism is then used to treat the non-Markovian dynamics of the same system within the structured electromagnetic density of states of a photonic crystal. We elucidate the extent to which phonon-assisted decay limits the lifetime of a single photon-atom bound state and derive the modified spontaneous emission dynamics due to coupling to various phonon baths. We demonstrate that coherent interaction with undamped phonons can lead to enhanced lifetime of a photon-atom bound state in a PBG by (i) dephasing and reducing the transition electric dipole moment of the atom and (ii) reducing the quantum mechanical overlap of the state vectors of the excited and ground state (polaronic shift). This results in reduction of the steady-state atomic polarization but an increase in the fractionalized upper state population in the photon-atom bound state. We demonstrate, on the other hand, that the lifetime of the photon-atom bound state in a PBG is limited by the lifetime of phonons due to lattice anharmonicities (break-up of phonons into lower energy phonons) and purely nonradiative decay. We demonstrate how these additional damping effects limit the extent of the polaronic (Franck-Condon) shift of the atomic excited state. We also derive the modified polarization decay and dephasing rates in the presence of such damping. This leads to a microscopic, quantum theory of the optical absorption lineshapes. Our model and formalism provide a starting point for describing dephasing and relaxation in the presence of external coherent fields and multiple quantum dot interactions in electromagnetic reservoirs with radiative memory effects.
We derive a quantum theory of the role of acoustic and optical phonons in modifying the optical absorption line shape, polarization dynamics, and population dynamics of a two-level atom (quantum dot) in the ``colored'' electromagnetic vacuum of a photonic band-gap (PBG) material. This is based on a microscopic Hamiltonian describing both radiative and vibrational processes quantum mechanically. We elucidate the extent to which phonon-assisted decay limits the lifetime of a single photon-atom bound state and derive the modified spontaneous emission dynamics due to coupling to various phonon baths. We demonstrate that coherent interaction with undamped phonons can lead to an enhanced lifetime of a photon-atom bound state in a PBG. This results in reduction of the steady-state atomic polarization but an increase in the fractionalized upper state population in the photon-atom bound state. We demonstrate, on the other hand, that the lifetime of the photon-atom bound state in a PBG is limited by the lifetime of phonons due to lattice anharmonicities (breakup of phonons into lower energy phonons) and purely nonradiative decay. We also derive the modified polarization decay and dephasing rates in the presence of such damping. This leads to a microscopic, quantum theory of the optical absorption line shapes. Our model and formalism provide a starting point for describing dephasing and relaxation in the presence of external coherent fields and multiple quantum dot interactions in electromagnetic reservoirs with radiative memory effects.
The entanglement dynamics of a laser-pumped two-level quantum dot pair is investigated in the steady state. The closely spaced two-level emitters, embedded in a semiconductor substrate, interact with both the environmental vacuum modes of the electromagnetic field reservoir as well as with the lattice vibrational phonon thermostat. We have found that the entanglement among the pair’s components is substantially enhanced due to the presence of the phonon subsystem. The reason is phonon-induced decay among the symmetrical and antisymmetrical two-qubit collective states and, consequently, the population of the latter one. This also means that through thermal phonon bath engineering one can access the subradiant two-particle cooperative state.
We study how the environment of photonic band gap (PBG) materials affects entanglement dynamics of qubits. Entanglement between the single qubit and the PBG environment is investigated through the von Neumann entropy while that for two initially entangled qubits in this PBG reservoir is through concurrence. Dynamics of these measurements are solved in use of the fractional calculus which has been shown appropriate for the systems with non-Markovian dynamics. Entropy dynamics of the single qubit system reveals that the coupling with the PBG reservoir prevents decoherence of the qubit through the steady entropy with non-zero value. The effect of PBG reservoir on the concurrence of the two-qubit system leads to the long-time entanglement preservation. The concurrence dynamics shows that unphysical entanglement trapping does not exist in the system with the qubit frequency lying outside the PBG region. Long-time memory effect of the PBG reservoir occurs only for the qubit frequency in the PBG region. Entanglement mechanisms resulting from this long-time memory effect are discussed.
We study the dynamics of the N-photon entanglement, E(N)(t), for the two-mode Jaynes-Cummings model in the case of a small number N of photons coupled to a single quantum dot inside a cavity, such as a microdisk cavity or a photonic crystal cavity. The quantum dot transitions associated with the photons with different polarizations are assumed to be independent of each other and, hence, the time evolutions of the ' + '- and ' - '-polarized photons are formally separable. However, due to the indistinguishability of the photons, such an interaction still leads to the entanglement of initially disentangled photon states, owing to the nonlinear dependence of the characteristic frequencies on the photon population numbers. The time dependence of the entanglement is the result of superimposing oscillations with incommensurate frequencies. Therefore, E(N)(t) is a quasi-periodic function of time with a complex profile strongly dependent on the number of photons.
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