A set of quantum equations describing the superfluorescent emission by two groups of sources having different resonance frequencies is presented. Numerical solutions are derived which in particular show significant differences between the quantum and the semiclassical results.
Superfluorescence is treated in the Markovian master-equation approach. We show that we have to consider the complex coupling between any pair of atoms in order to reproduce superfluorescence signals with ringings as exhibited by experiments. We compare numerical results of our model with those obtained by a semiclassical approach of superfluorescence. The quantum treatment is found to be in agreement with the semiclassical approach only if the semiclassical tipping angle is taken equal to the square root of the number of radiating particles.
The "superfluorescence equations" deduced in a previous paper are generalized to the case of finite temperature and translated into the atomic coherent-state representation of Arecchi et al. We get three coupled partial differential equations involving the quasiprobability distribution $Q(\ensuremath{\theta},t)$ of the atomic system and two suitable functions $\mathcal{F}(\ensuremath{\theta},t)$ and $\mathfrak{M}(\ensuremath{\theta},t)$ describing the stimulated processes which are relevant in oscillatory superfluorescence. Neglecting $\mathcal{F}(\ensuremath{\theta},t)$ and $\mathfrak{M}(\ensuremath{\theta},t)$, the equation for $Q(\ensuremath{\theta},t)$ reduces to the Fokker-Planck equation of Narducci et al. corrected by the contribution of thermal noise. The stationary solution is given by the unperturbed canonical state, which is shown to be the exact stationary solution of the single-mode model from which the superfluorescence equations have been deduced. These equations prescribe that $\mathfrak{M}(\ensuremath{\theta},t)$ always remain equal and opposite to $\mathcal{F}(\ensuremath{\theta},t)$, so that the superfluorescence equations reduce automatically to two equations. Eliminating $\mathcal{F}(\ensuremath{\theta},t)$ between the two remaining equations, one obtains a non-Markovian equation for $Q(\ensuremath{\theta},t)$ with derivatives of all orders in $\ensuremath{\theta}$. In the case of pure superfluorescence or super-radiance, such an equation reduces to a Markovian Fokker-Planck equation with derivatives of first and second order in $\ensuremath{\theta}$ which exhibits an interesting fourth-order contribution in the diffusion term. In fact, if one excludes a very small region around the north pole of the Bloch sphere, this term is much larger than the second-order contribution in the diffusion term of the equation of Narducci et al. In the case of oscillatory superfluorescence, the presence of memory effects enhances fluctuations, thus forbidding the existence of "classical" time evolutions.
An approach to modeling the dynamics of x-ray amplified spontaneous emission and superfluorescence, the phenomenon of collective x-ray emission initiated by intense pulses of x-ray free-electron lasers, is developed based on stochastic partial differential equations. The equations are derived from first principles, and the relevant approximations, derivation steps, and extensions specific to stimulated x-ray emission are presented. The resulting equations take the form of three-dimensional generalized Maxwell-Bloch equations augmented with noise terms for both field and atomic variables. The derived noise terms possess specific correlation properties that enable the correct reconstruction of spontaneous emission. Consequently, the developed theoretical formalism is universally suitable for describing all stages of stimulated x-ray emission: spontaneous emission, amplified spontaneous emission, and superfluorescence. We present numerical examples that illustrate various properties of the emitted field, including spatiotemporal coherence and spectral-angular and polarization characteristics. We anticipate that the proposed theoretical framework will establish a robust foundation for interpreting measurements in stimulated x-ray emission spectroscopy, modeling x-ray laser oscillators, and describing other experiments leveraging x-ray superfluorescence.