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Nanotechnology

Spin-polarized pumping in a double quantum dot

E. Cota, Ramón Aguado, C. E. Creffield, Gloria Platero

Published Jan 10, 2003• 31 citations
Publisher

Abstract

We study the pumping of spin-polarized electrons in a double quantum dot system with up to two electrons per dot, via an applied AC field and a constant magnetic field. The behaviour of the current through the double-dot system is studied as a function of the AC field and coupling to the leads, using a Markov master equation approach for the time evolution of the reduced density matrix. For up to two electrons in the system, we find that the formation of a spin-triplet state blocks the current through the device, and analyse possible solutions. When we incorporate three-and four-particle states, with up to two opposite spin electrons per dot, we find a regime where the pumping of spin-polarized electrons is realized through double occupancy states in each dot. This property is robust against spin-relaxation and decoherence processes which are taken into account phenomenologically. Finally we study the effects of applying a pulsed AC field and the possibility of the resolution of Rabi oscillations.

DOI
10.1088/0957-4484/14/2/310

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We study the pumping of spin-polarized electrons in a double quantum dot system with up to two electrons per dot, via an applied AC field and a constant magnetic field. The behaviour of the current through the double-dot system is studied as a function of the AC field and coupling to the leads, using a Markov master equation approach for the time evolution of the reduced density matrix. For up to two electrons in the system, we find that the formation of a spin-triplet state blocks the current through the device, and analyse possible solutions. When we incorporate three-and four-particle states, with up to two opposite spin electrons per dot, we find a regime where the pumping of spin-polarized electrons is realized through double occupancy states in each dot. This property is robust against spin-relaxation and decoherence processes which are taken into account phenomenologically. Finally we study the effects of applying a pulsed AC field and the possibility of the resolution of Rabi oscillations.
We analyze the charge and spin dynamics in a DC biased double quantum dot driven by crossed DC and AC magnetic fields. In this configuration, spatial delocalization due to inter-dot tunnel competes with intra-dot spin rotations induced by the time dependent magnetic field, giving rise to a complicated time dependent behavior of the tunnelling current. When the Zeeman splitting has the same value in both dots and spin flip is negligible, the electrons remain in the triplet subspace (dark subspace) performing coherent spin rotations and the current does not flow. This electronic trapping is removed either by finite spin relaxation or when the Zeeman splitting is different in each quantum dot. In the first case, our results show that measuring the current will allow to get information on the spin relaxation time. In the last case, we will show that applying a resonant bichromatic magnetic field, the electrons become trapped in a coherent superposition of states and electronic transport is blocked. Then, manipulating AC magnetic fields, electrons are driven to perform coherent spin rotations which can be unambiguously detected by direct measurement of the tunneling current.
We analyze coherent spin rotations in a dc biased double quantum dot driven by crossed dc and ac magnetic fields. In this configuration, spatial delocalization due to interdot tunneling competes with intradot spin rotations induced by the time dependent magnetic field, giving rise to a complicated time dependent behavior of the tunneling current. When the Zeeman splitting has the same value in both dots and spin flip is negligible, the electrons remain in the triplet subspace performing coherent spin rotations and current does not flow. This electronic trapping is removed either by finite spin relaxation or when the Zeeman splitting is different in each quantum dot. In the last case, we will show that by applying a resonant bichromatic magnetic field, the electrons become trapped in a coherent superposition of states and electronic transport is blocked. Then, manipulating ac magnetic fields allows one to drive electrons to perform coherent spin rotations which can be unambiguously detected by direct measurement of the tunneling current.
We report on our recent progress in applying semiconductor quantum dots for spin-based quantum computation, as proposed by Loss and DiVincenzo (1998 Phys. Rev. A 57 120). For the purpose of single-electron spin resonance, we study different types of single quantum dot devices that are designed for the generation of a local ac magnetic field in the vicinity of the dot. We observe photon-assisted tunnelling as well as pumping due to the ac voltage induced by the ac current driven through a wire in the vicinity of the dot, but no evidence for ESR so far. Analogue concepts for a double quantum dot and the hydrogen molecule are discussed in detail. Our experimental results in laterally coupled vertical double quantum dot device show that the Heitler–London model forms a good approximation of the two-electron wavefunction. The exchange coupling constant J is estimated. The relevance of this system for two-qubit gates, in particular the SWAP operation, is discussed. Density functional calculations reveal the importance of the gate electrode geometry in lateral quantum dots for the tunability of J in realistic two-qubit gates.
The spin dynamics in two electron double quantum dots embedded in a two-dimensional electron gas at the interface between SrTiO3{\mathrm{Sr}\mathrm{Ti}\mathrm{O}}_{3}SrTiO3​ and LaAlO3{\mathrm{La}\mathrm{Al}\mathrm{O}}_{3}LaAlO3​ is studied by an exact numerical solution of the time-dependent Schr\"odinger equation in the context of the electric-dipole-spin-resonance experiment. On the basis of the three-band model of 3d3d3d electrons localized at Ti\mathrm{Ti}Ti ions on the square lattice, we analyze in detail the singlet-triplet transition induced by the ac electric field, in the magnetic field range close to the avoided crossing that appears as a result of the spin-orbit coupling. For symmetric double quantum dots the single-photon spin-flip transition is prohibited due to the parity symmetry, and the transition can occur only by the higher-order two-photon processes. For a weakly asymmetric system, when the first-order singlet-triplet transitions are released due to the parity symmetry breaking, the spin-flip transition has a character of the Rabi oscillations for a low electric field amplitude. As the amplitude is increased, the frequency of the transition is blueshifted (redshifted) for the magnetic field below (above) the single-triplet avoided crossing. For a sufficiently high magnetic field and high ac-field amplitude, the electric field drives the system across the avoided crossing, inducing the spin flip by the Landau-Zener-Stueckelberg-Majorana effect. Finally, the optimization of the geometrical parameters of the system with respect to the time of spin flip of its fidelity is also presented.
In moderately strong magnetic fields, the difference in Land\'e ggg factors in each of the dots of a two-electron double quantum dot (DQD) may induce oscillations between singlet and triplet states of an entangled pair and lead to a nonequilibrium electron spin polarization in the system. The calculated bipolar polarization reflects the strong spin correlation in the spatially separated pair of electrons that occupy almost degenerate states in a coupled DQD. We will show that this polarization may partially survive the rapid inhomogeneous decoherence caused by random nuclear magnetic fields.
Electrical spin manipulation in double SrTiO3_33​/LaAlO3_33​ quantum dots
The spin dynamics in two electron double quantum dots embedded in two dimensional electron gas at the interface between SrTiO3_33​ and LaAlO3_33​ is studied by an exact numerical solution of the time-dependent Schrödinger equation, in the context of the electric dipole spin resonance experiment. Based on the three band model of 3d3d3d-electrons localized at Ti ions on the square lattice we analyze in details the singlet-triplet transition induced by the AC electric field, in the magnetic field range close to the avoided crossing which appears as a result of the spin-orbit coupling. Our calculations show that for symmetric double quantum dots the single photon spin-flip transitions is prohibited due to the parity symmetry and the transition can occur only by the higher order two-photon processes. For a weakly asymmetric system, when the first order singlet-triplet transitions are released due to the parity symmetry breaking, the spin-flip transition has a character of the Rabi oscillations for a low electric field amplitude. As the amplitude is increased the frequency of the transition is blueshifted (redshifted) for the magnetic field below (above) the single-triplet avoided crossing. Interestingly, for a sufficiently high magnetic field and high AC field amplitude the electric field drives the system across the avoided crossing inducing the spin-flip by the Landau-Zener-Stueckelberg-Majorana transitions with 100\% spin flip probability for a slow sweep. Finally, the optimization of the geometrical parameters of the system with respect to the time of spin-flip of its fidelity is also presented.