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Physics and Chemistry of Liquids

On the hydrodynamics of a superfluid with a three-particle “condensate”

Zygmunt M. Galasiewicz

Published Jan 1, 1977• 1 citation
Publisher

Abstract

Since 1974 there have been serious experimental and also theoretical pointers to the possibility that no Bose condensation occurs in superfluid He4. Evans presented a theoretical argument against a condesate, suggesting a “pairing” model of superfluid helium. As yet, experiment connot decide if the concept of a one-particle condensate can be replaced by the idea of a two-particle condensate. March and Galasiewicz have argued that, if there is no one-particle condensate in He4, a ground state wave function cannot be built from a product of pairs but must fundamentally include three-particle correlations at least. So the idea of a three (not two) particle condensate seems worth some attention. It is demonstrated here that assuming a three-particle condensate we can regain from microscopic theory the Landau hydrodynamic equation for the superfluid velocity.

DOI
10.1080/00319107708084146

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Since 1974 there have been serious experimental and also theoretical pointers to the possibility that no Bose condensation occurs in superfluid He4. Evans presented a theoretical argument against a condesate, suggesting a “pairing” model of superfluid helium. As yet, experiment connot decide if the concept of a one-particle condensate can be replaced by the idea of a two-particle condensate. March and Galasiewicz have argued that, if there is no one-particle condensate in He4, a ground state wave function cannot be built from a product of pairs but must fundamentally include three-particle correlations at least. So the idea of a three (not two) particle condensate seems worth some attention. It is demonstrated here that assuming a three-particle condensate we can regain from microscopic theory the Landau hydrodynamic equation for the superfluid velocity.
The paradoxes and disparities in the contemporary microscopic theory of superfluid helium (He–II) are discussed along with possible ways of resolving them by taking pair correlations of He4 atoms into consideration. It is shown that most paradoxes are associated with the commonly accepted initial assumption concerning the dominating role of single-particle Bose condensate (SPBC) in the quantum microstructure of the superfluid component ρs. The existence of intensive SPBC leads to a strong hybridization of the elementary excitation branches and to a common dispersion law for all boson branches, which is identified with the quasiparticle spectrum E(p) observed experimentally from slow neutron scattering in liquid helium. However, the stability of this spectrum during a transition through the λ-point and the large value of the gap in the vicinity of the “rotonic” minimum contradict both the Landau theoretical criterion of superfluidity and the small value of experimentally measured critical velocity. At the same time, a strong interaction between particles in the Bose liquid He4 strongly suppresses the SPBC which amounts to less than 1% of all He4 atoms and hence cannot be the main constituent of the superfluid component, unlike the case of a weakly nonideal Bose gas. Moreover, for a quite strong attraction between particles in a certain region of the momentum space, bound pairs of bosons can be formed in the superfluid Bose liquid, and a coherent pair condensate (CPC) analogous to the Cooper pair condensate in superconductors may appear. Such a strong CPC may completely suppress the weak SPBC. In this case, the one-particle spectrum ε(p) of elementary excitations does not hybridize with the collective (two-particle) spectrum and does not appear in the structure of the dynamic form factor S(p,ε), i.e., does not coincide with the spectrum measured from neutron scattering. The dispersion of one-particle spectrum is defined by the momentum dependence of the pair order parameter Ψ̃(p) and may have a minimum or a point of inflection at p≠0. This peculiarity in the one-particle spectrum of a Bose liquid with CPC but without SPBC vanishes together with Ψ̃(p) at the temperature Tc=Tλ of the phase transition from the superfluid to the normal state (unlike the rotonic minimum in the collective spectrum), while the corresponding critical velocity vc=min[ε(p)/p] vanishes at the λ-point in accordance with the Landau criterion and the experimental data. The assumption that the strong “Cooper-like” CPC is responsible for the quantum structure of the superfluid component ρs is confirmed indirectly by the successful application of the Justrow approximation (based on strong pair correlations) for describing the properties of liquid He4 and quantum liquid mixtures He3–4He on one hand, and by an anomalously large effective mass of He3 impurity atoms in He4, which is approximately equal to total mass of He3 and He4 atoms, thus pointing to the existence of helium atoms in superfluid liquid He–II. The value of the superfluid velocity circulation quantum in the Onsager–Feynman vortices in a Bose liquid with CPC but without SPBC is discussed as well as the critical velocities of superfluid He4 in ultrathin films and channels in which the creation and motion of quantum vortices are ruled out, and the quasiparticle spectrum undergoes dimensional quantization.
The basic assumption of this paper is that in the presence of Bose-Einstein condensation (BEC) in liquid 4He^{4}\mathrm{He}4He, the wave functions of occupied many particle states are the superposition of two components; a phase coherent component, proportional to the ground state wave function and a phase incoherent component. It is shown that this assumption satisfies necessary conditions imposed by the presence of BEC and that the wave functions of the ideal Bose gas and wave functions of the Bijl-Feynman type are of this form. It is shown that this single assumption provides simple microscopic explanations of essentially all the exotic properties of helium II; why BEC implies two fluid behavior, how the superfluid and condensate fractions are linked, how Landau theory is linked to the presence of BEC, why the superfluid exhibits flow without viscosity and macroscopic quantum effects while the normal fluid does not, how the anomalous expansion and loss of spatial order, observed in helium II as it is cooled, is linked to BEC, and how the presence of sharp peaks observed in the dynamic structure factor are linked with BEC. The theory provides predictions that are in quantitative agreement with a wide range of presently unexplained experimental data on helium II.
A well-known paradox in the theory of superfluidity is studied: superfluidity is linked to Bose condensation, but the superfluid density is always greater than the density of the Bose condensate. Based on the model of a weakly nonideal Bose gas, it is demonstrated that supercondensate particles, forming pairs which are correlated in momentum space—the two-particle condensate—make the missing contribution to the superfluid density. It is shown that in the case of slow spatial variations of superfluid flows it is possible to introduce a macroscopic wave function describing the entire superfluid component and not only the single-particle condensate. The characteristic features of weak superfluidity in Bose systems are studied and it is shown that the tunneling effect is a sensitive tool for studying the structure of the superfluid component. It is hypothesized that the superfluid component of real He II consists of the sum of one-, two-, three-, and many-particle condensates.
The Bose-Einstein condensation mechanism is shown to be capable of accounting for the existence of separate hydrodynamic velocity fields for the normal and the superfluid, provided suitable assumptions are made with regard to the single-particle energy spectrum. We consider the effect on the microcanonical gas distribution of imposing a nonzero value of the total momentum P. For an ordinary gas the effect is trivial, the whole distribution being merely shifted in momentum space. However, in the case of a degenerate Bose gas whose single-particle energy spectrum has a sharp minimum (gap or cusp), only the excited part of the gas (normal fluid) participates in the imposed motion, the condensate (superfluid) remaining "frozen" in momentum space. This rigidity of the condensate in momentum space plays the same role as the rigidity of the superelectrons on imposition of a magnetic field in the London theory of superconductivity. P acts as an additional thermodynamic variable, states with P \ensuremath{\ne} 0 being macroscopically metastable and corresponding to the existence of a relative velocity between normal and superfluid. The basic hydrodynamic assumption of the two-fluid model is thus reduced to an assumption concerning the form of an effective single-particle energy spectrum, and the parallelism between the theories of superconductivity and superfluidity is clearly exhibited. The present theory permits, in particular, the introduction of the mathematical form of Landau's phonon and "roton" spectra within the framework of the Bose-Einstein condensation picture. The statistical-thermodynamic formulas are derived and are shown to lead to characteristic two-fluid equations derived previously from a variational principle.
Abstract Chapter 2 describes the basic knowledge of Bose-condensed systems in order to study the quantum hydrodynamics for both the superfluid helium and the atomic-gas BECs in the following sections. Starting from the field theoretical formulation, we will first give a self-contained explanation of the derivation of the most fundamental GP equation for weakly interacting Bose gases at zero temperature. We will also highlight the theoretical treatment for incorporating the concept of elementary excitations to describe low-energy excitations of Bose systems, the definition of normal and superfluid components, and eventually the celebrated model of two-fluid hydrodynamics. Finally, the microscopic structure and dynamics of topological excitations obtained from the GP equation are discussed by exemplifying solitons, vortex lines, and vortex rings.