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Physical Review

Liquid Helium II: Bose-Einstein Condensation and Two-Fluid Model

Paul R. Zilsel

Published Dec 1, 1953• 12 citations
Publisher

Abstract

The Bose-Einstein condensation mechanism is shown to be capable of accounting for the existence of separate hydrodynamic velocity fields for the normal and the superfluid, provided suitable assumptions are made with regard to the single-particle energy spectrum. We consider the effect on the microcanonical gas distribution of imposing a nonzero value of the total momentum P. For an ordinary gas the effect is trivial, the whole distribution being merely shifted in momentum space. However, in the case of a degenerate Bose gas whose single-particle energy spectrum has a sharp minimum (gap or cusp), only the excited part of the gas (normal fluid) participates in the imposed motion, the condensate (superfluid) remaining "frozen" in momentum space. This rigidity of the condensate in momentum space plays the same role as the rigidity of the superelectrons on imposition of a magnetic field in the London theory of superconductivity. P acts as an additional thermodynamic variable, states with P \ensuremath{\ne} 0 being macroscopically metastable and corresponding to the existence of a relative velocity between normal and superfluid. The basic hydrodynamic assumption of the two-fluid model is thus reduced to an assumption concerning the form of an effective single-particle energy spectrum, and the parallelism between the theories of superconductivity and superfluidity is clearly exhibited. The present theory permits, in particular, the introduction of the mathematical form of Landau's phonon and "roton" spectra within the framework of the Bose-Einstein condensation picture. The statistical-thermodynamic formulas are derived and are shown to lead to characteristic two-fluid equations derived previously from a variational principle.

DOI
10.1103/physrev.92.1106

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The paradoxes and disparities in the contemporary microscopic theory of superfluid helium (He–II) are discussed along with possible ways of resolving them by taking pair correlations of He4 atoms into consideration. It is shown that most paradoxes are associated with the commonly accepted initial assumption concerning the dominating role of single-particle Bose condensate (SPBC) in the quantum microstructure of the superfluid component ρs. The existence of intensive SPBC leads to a strong hybridization of the elementary excitation branches and to a common dispersion law for all boson branches, which is identified with the quasiparticle spectrum E(p) observed experimentally from slow neutron scattering in liquid helium. However, the stability of this spectrum during a transition through the λ-point and the large value of the gap in the vicinity of the “rotonic” minimum contradict both the Landau theoretical criterion of superfluidity and the small value of experimentally measured critical velocity. At the same time, a strong interaction between particles in the Bose liquid He4 strongly suppresses the SPBC which amounts to less than 1% of all He4 atoms and hence cannot be the main constituent of the superfluid component, unlike the case of a weakly nonideal Bose gas. Moreover, for a quite strong attraction between particles in a certain region of the momentum space, bound pairs of bosons can be formed in the superfluid Bose liquid, and a coherent pair condensate (CPC) analogous to the Cooper pair condensate in superconductors may appear. Such a strong CPC may completely suppress the weak SPBC. In this case, the one-particle spectrum ε(p) of elementary excitations does not hybridize with the collective (two-particle) spectrum and does not appear in the structure of the dynamic form factor S(p,ε), i.e., does not coincide with the spectrum measured from neutron scattering. The dispersion of one-particle spectrum is defined by the momentum dependence of the pair order parameter Ψ̃(p) and may have a minimum or a point of inflection at p≠0. This peculiarity in the one-particle spectrum of a Bose liquid with CPC but without SPBC vanishes together with Ψ̃(p) at the temperature Tc=Tλ of the phase transition from the superfluid to the normal state (unlike the rotonic minimum in the collective spectrum), while the corresponding critical velocity vc=min[ε(p)/p] vanishes at the λ-point in accordance with the Landau criterion and the experimental data. The assumption that the strong “Cooper-like” CPC is responsible for the quantum structure of the superfluid component ρs is confirmed indirectly by the successful application of the Justrow approximation (based on strong pair correlations) for describing the properties of liquid He4 and quantum liquid mixtures He3–4He on one hand, and by an anomalously large effective mass of He3 impurity atoms in He4, which is approximately equal to total mass of He3 and He4 atoms, thus pointing to the existence of helium atoms in superfluid liquid He–II. The value of the superfluid velocity circulation quantum in the Onsager–Feynman vortices in a Bose liquid with CPC but without SPBC is discussed as well as the critical velocities of superfluid He4 in ultrathin films and channels in which the creation and motion of quantum vortices are ruled out, and the quasiparticle spectrum undergoes dimensional quantization.

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Landau's theory of superfluidity

Allan Griffin, Tetsuro Nikuni, E. Zaremba

In this chapter, we review the famous Landau theory of superfluidity at finite temperatures. This theory is based on coupled hydrodynamic equations for the superfluid and normal fluid components. Landau's two-fluid description is only valid when collisions among the thermal excitations making up the normal fluid are strong enough to produce local hydrodynamic equilibrium. These two-fluid equations were originally developed for liquid. He but are thought to be generic in form, describing the collision-dominated hydrodynamic region of all Bose superfluids. In this chapter, we will consider the solutions of the two-fluid equations mainly for a uniform superfluid. We discuss the existence of second sound (involving the out-of-phase motion of the superfluid and normal fluid components) as a characteristic feature of a Bose superfluid at finite temperatures. This chapter gives background material needed for Chapters 15–19. In Chapter 15, we will show that, in the appropriate limit, the Landau two-fluid equations can be derived from the ZNG coupled equations given in Chapter 3 for a trapped dilute Bose-condensed gas. In Chapters 17–19, we extend this discussion and derive the Landau–Khalatnikov two-fluid equations, which include hydrodynamic damping associated with various transport coefficients. Useful reviews of the two-fluid equations in the context of dilute spatially uniform Bose-condensed gases are given by Pethick and Smith (2008, Chapter 10) and Pitaevskii and Stringari (2003, Chapter 6). History of two-fluid equations The original discovery of superfluidity in liquid He was dramatically announced with the publication of the famous back-to-back papers of Kapitza (1938) in Moscow and Allen and Misener (1938) in Cambridge. These and subsequent experiments in the next few years showed that superfluid He could exhibit very bizarre hydrodynamic behaviour compared to classical liquids.

Cambridge University Press eBooks•Feb 19, 2009•1 citation
The Bose-Einstein condensation mechanism is shown to be capable of accounting for the existence of separate hydrodynamic velocity fields for the normal and the superfluid, provided suitable assumptions are made with regard to the single-particle energy spectrum. We consider the effect on the microcanonical gas distribution of imposing a nonzero value of the total momentum P. For an ordinary gas the effect is trivial, the whole distribution being merely shifted in momentum space. However, in the case of a degenerate Bose gas whose single-particle energy spectrum has a sharp minimum (gap or cusp), only the excited part of the gas (normal fluid) participates in the imposed motion, the condensate (superfluid) remaining "frozen" in momentum space. This rigidity of the condensate in momentum space plays the same role as the rigidity of the superelectrons on imposition of a magnetic field in the London theory of superconductivity. P acts as an additional thermodynamic variable, states with P \ensuremath{\ne} 0 being macroscopically metastable and corresponding to the existence of a relative velocity between normal and superfluid. The basic hydrodynamic assumption of the two-fluid model is thus reduced to an assumption concerning the form of an effective single-particle energy spectrum, and the parallelism between the theories of superconductivity and superfluidity is clearly exhibited. The present theory permits, in particular, the introduction of the mathematical form of Landau's phonon and "roton" spectra within the framework of the Bose-Einstein condensation picture. The statistical-thermodynamic formulas are derived and are shown to lead to characteristic two-fluid equations derived previously from a variational principle.
The basic assumption of this paper is that in the presence of Bose-Einstein condensation (BEC) in liquid 4He^{4}\mathrm{He}4He, the wave functions of occupied many particle states are the superposition of two components; a phase coherent component, proportional to the ground state wave function and a phase incoherent component. It is shown that this assumption satisfies necessary conditions imposed by the presence of BEC and that the wave functions of the ideal Bose gas and wave functions of the Bijl-Feynman type are of this form. It is shown that this single assumption provides simple microscopic explanations of essentially all the exotic properties of helium II; why BEC implies two fluid behavior, how the superfluid and condensate fractions are linked, how Landau theory is linked to the presence of BEC, why the superfluid exhibits flow without viscosity and macroscopic quantum effects while the normal fluid does not, how the anomalous expansion and loss of spatial order, observed in helium II as it is cooled, is linked to BEC, and how the presence of sharp peaks observed in the dynamic structure factor are linked with BEC. The theory provides predictions that are in quantitative agreement with a wide range of presently unexplained experimental data on helium II.
The paradoxes and disparities in the contemporary microscopic theory of superfluid helium (He–II) are discussed along with possible ways of resolving them by taking pair correlations of He4 atoms into consideration. It is shown that most paradoxes are associated with the commonly accepted initial assumption concerning the dominating role of single-particle Bose condensate (SPBC) in the quantum microstructure of the superfluid component ρs. The existence of intensive SPBC leads to a strong hybridization of the elementary excitation branches and to a common dispersion law for all boson branches, which is identified with the quasiparticle spectrum E(p) observed experimentally from slow neutron scattering in liquid helium. However, the stability of this spectrum during a transition through the λ-point and the large value of the gap in the vicinity of the “rotonic” minimum contradict both the Landau theoretical criterion of superfluidity and the small value of experimentally measured critical velocity. At the same time, a strong interaction between particles in the Bose liquid He4 strongly suppresses the SPBC which amounts to less than 1% of all He4 atoms and hence cannot be the main constituent of the superfluid component, unlike the case of a weakly nonideal Bose gas. Moreover, for a quite strong attraction between particles in a certain region of the momentum space, bound pairs of bosons can be formed in the superfluid Bose liquid, and a coherent pair condensate (CPC) analogous to the Cooper pair condensate in superconductors may appear. Such a strong CPC may completely suppress the weak SPBC. In this case, the one-particle spectrum ε(p) of elementary excitations does not hybridize with the collective (two-particle) spectrum and does not appear in the structure of the dynamic form factor S(p,ε), i.e., does not coincide with the spectrum measured from neutron scattering. The dispersion of one-particle spectrum is defined by the momentum dependence of the pair order parameter Ψ̃(p) and may have a minimum or a point of inflection at p≠0. This peculiarity in the one-particle spectrum of a Bose liquid with CPC but without SPBC vanishes together with Ψ̃(p) at the temperature Tc=Tλ of the phase transition from the superfluid to the normal state (unlike the rotonic minimum in the collective spectrum), while the corresponding critical velocity vc=min[ε(p)/p] vanishes at the λ-point in accordance with the Landau criterion and the experimental data. The assumption that the strong “Cooper-like” CPC is responsible for the quantum structure of the superfluid component ρs is confirmed indirectly by the successful application of the Justrow approximation (based on strong pair correlations) for describing the properties of liquid He4 and quantum liquid mixtures He3–4He on one hand, and by an anomalously large effective mass of He3 impurity atoms in He4, which is approximately equal to total mass of He3 and He4 atoms, thus pointing to the existence of helium atoms in superfluid liquid He–II. The value of the superfluid velocity circulation quantum in the Onsager–Feynman vortices in a Bose liquid with CPC but without SPBC is discussed as well as the critical velocities of superfluid He4 in ultrathin films and channels in which the creation and motion of quantum vortices are ruled out, and the quasiparticle spectrum undergoes dimensional quantization.
One considers the superfluid (SF) state of a Bose liquid with a strong repulsion between bosons, in which at T=0, along with a weak single-particle Bose-Einstein condensate (BEC), there exists an intensive pair coherent condensate (PCC), analogous to the Cooper condensate in a Fermi liquid with an attraction between the fermions. Such a PCC emerges in a system of bosons due to an oscillating sign-changing momentum dependence of the Fourier component of the pair interaction potential, which is characteristic of a certain family of repulsion potentials. In such cases, the Fourier component is negative in some domain of nonzero momentum transfer, which corresponds to an effective attraction. The collective effects of renormalization (``screening'') of the initial interaction lead to a suppression of the repulsion and an enhancement of the effective attraction. It is the ratio of the BEC density to the full density of the liquid n0/n≪1n_0/n\ll 1n0​/n≪1 that is used as a small parameter---unlike in the Bogolyubov theory for a quasi-ideal Bose gas, in which the small parameter is the ratio of the number of supracondensate excitations to the number of particles in an intensive BEC, (n−n0)/n0≪1(n-n_0)/n_0\ll 1(n−n0​)/n0​≪1. A closed system of nonlinear integral equations for the normal and anomalous self-energy parts is obtained, in the framework of a renormalized perturbation theory built on combined hydrodynamic and field variables. In the framework of the hard-spheres model, a spectrum of quasiparticles is obtained, which is in good accordance with the experimental spectrum of elementary excitations in superfluid 4^44He. The question of applicability of the Landau criterion in the absence of quantum vortices is discussed.
The equations of motion for the reduced density matrices of an interacting Bose system are treated using the concept of off-diagonal long-range order. The equations are decoupled on the one-particle level. With this approximation, the hydrodynamic equations for the densities and the velocities of the condensate and the depletion are derived. The interaction between the two fluid components depends on density variations and on the relative velocity. The latter interaction terms appear as kinetic pressure terms and a Magnus force term. Via the equation for the total momentum, a connection between the velocities of the condensate and the depletion, and the velocities in Landau's two-fluid model is derived. The excitation spectrum of the system is investigated in the phonon region. A comparison of the resulting velocities for the first and second sound with the experimentally determined ones shows that the functional dependence of the condensate density on temperature is similar to that of the superfluid component.
The theory of the condensate of a weakly interacting Bose gas is developed. The condensate is described by a wavefunction ψ(x, t) normalized to the number of particles. It obeys a nonlinear self-consistent field equation. The solution in the presence of a rigid wall with the boundary condition of vanishing wavefunction involves a de Broglie length. This length depends on the mean potential energy per particle. The self-consistent field term keeps the density uniform except in localized spatial regions. In the hydrodynamical version, a key role is played by the quantum potential. A theory of quantized vortices and of general potential flows follows immediately. In contrast to classical hydrodynamics, the cores of vortices are completely determined by the de Broglie length and all energies are finite. Nonstationary disturbances of the condensate correspond to phonons, rotons, vortex waves etc. They can exchange momentum with rigid boundaries. This is compatible with the vanishing of the wavefunction at a boundary. This condition fully determines the dynamics of the system. These points are illustrated by considering the motion of a foreign ion in a Bose gas, a rotating container of fluid, and the Landau criterion for superfluidity.
In this chapter, we review the famous Landau theory of superfluidity at finite temperatures. This theory is based on coupled hydrodynamic equations for the superfluid and normal fluid components. Landau's two-fluid description is only valid when collisions among the thermal excitations making up the normal fluid are strong enough to produce local hydrodynamic equilibrium. These two-fluid equations were originally developed for liquid. He but are thought to be generic in form, describing the collision-dominated hydrodynamic region of all Bose superfluids. In this chapter, we will consider the solutions of the two-fluid equations mainly for a uniform superfluid. We discuss the existence of second sound (involving the out-of-phase motion of the superfluid and normal fluid components) as a characteristic feature of a Bose superfluid at finite temperatures. This chapter gives background material needed for Chapters 15–19. In Chapter 15, we will show that, in the appropriate limit, the Landau two-fluid equations can be derived from the ZNG coupled equations given in Chapter 3 for a trapped dilute Bose-condensed gas. In Chapters 17–19, we extend this discussion and derive the Landau–Khalatnikov two-fluid equations, which include hydrodynamic damping associated with various transport coefficients. Useful reviews of the two-fluid equations in the context of dilute spatially uniform Bose-condensed gases are given by Pethick and Smith (2008, Chapter 10) and Pitaevskii and Stringari (2003, Chapter 6). History of two-fluid equations The original discovery of superfluidity in liquid He was dramatically announced with the publication of the famous back-to-back papers of Kapitza (1938) in Moscow and Allen and Misener (1938) in Cambridge. These and subsequent experiments in the next few years showed that superfluid He could exhibit very bizarre hydrodynamic behaviour compared to classical liquids.