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Physical Review Letters

Critical Dynamics of Model C Resolved

R. Folk, G. Moser

Published Jul 15, 2003• 25 citations
Publisher

Abstract

We analyze the field theoretic functions of the dynamical model C in two-loop order. Our results correct long-standing errors in these functions published by several authors. We discuss, in particular, the fixed points for the ratio w* of the two time scales involved, as well as their stability. The regions of the "phase diagram," whose axes are the spatial dimension d and number of order parameter components n, correspond to these fixed points; previous authors have found, in addition, an anomalous region in which the scaling properties were unclear. We show that such an anomalous region does not exist. There are only two regions: one with a finite fixed-point w* where the dynamical exponent z=2+alpha/nu, and another where w*=0 and z is equal to the model A value. We show how the one-loop result is recovered from the two-loop result in the limit epsilon=4-d going to zero.

DOI
10.1103/physrevlett.91.030601

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We analyze the field theoretic functions of the dynamical model C in two-loop order. Our results correct long-standing errors in these functions published by several authors. We discuss, in particular, the fixed points for the ratio w* of the two time scales involved, as well as their stability. The regions of the "phase diagram," whose axes are the spatial dimension d and number of order parameter components n, correspond to these fixed points; previous authors have found, in addition, an anomalous region in which the scaling properties were unclear. We show that such an anomalous region does not exist. There are only two regions: one with a finite fixed-point w* where the dynamical exponent z=2+alpha/nu, and another where w*=0 and z is equal to the model A value. We show how the one-loop result is recovered from the two-loop result in the limit epsilon=4-d going to zero.
Dynamical scaling functions above Tc for the characteristic frequencies and the dynamical correlation functions of the order parameter and the conserved density of model C are calculated in one loop order. By a proper exponentiation procedure these results can be extended in order to consider the changes in these functions using the fixed point values and exponents in two loop order. The dynamical amplitude ratio R of the characteristic frequencies is generalized to the critical region. Surprisingly the decay of the shape functions at large scaled frequency does not behave as expected from applying scaling arguments. The exponent upsilon of the decay does not change when going from the critical to the hydrodynamic region although the shape functions change. The value of upsilon for the order parameter is in agreement with its value in the critical region, whereas for the conserved density it is equal to 2, the value in the hydrodynamic region.
We review the progress made in dynamic bulk critical behaviour in equilibrium in the last 25 years since the review of Halperin and Hohenberg. We unify the presentation of the theoretical background by restricting ourselves to the field-theoretic renormalization group method. The main results obtained in the different universality classes are presented. This contains the critical dynamics near the gas–liquid transition in pure fluids (model H), the plait point and consolute point in mixtures (model H � ), the superfluid transition in 4 He (model F) and 4 He– 3 He mixtures (model F � ), the Curie point (model J) and Neel point (model G) in Heisenberg magnets and the superconducting transition. In comparison with experimental results, it became clear that in most cases one has to consider apart from the universal asymptotic critical behaviour also the non-universal effective behaviour. Either because it turned out to be inevitable due to a small dynamical transient exponent inhibiting the system to reach the asymptotics (e.g., at the superfluid transition) or because one is interested in the region further away from the phase transition like in pure fluids and mixtures at their gas–liquid or demixing transition. The calculation of the critical dynamics is adequate in most cases only in two-loop order. We review these results and present the solution to unreasonable features found for some models. Thus, we consider model C where relaxational and diffusive dynamics are coupled and the scaling properties and the limit to a purely relaxational model (model A) have not been understood. In general for models where the order parameter couples to other conserved densities time scale ratios between the kinetic coefficients of the order parameter and the conserved densities play an important role. Their fixed-point values and the approach to the fixed point are changed considerably in two-loop order compared to their values in one-loop order. These considerations are relevant for the explanation of the dynamical critical shape functions of systems such as superfluid helium (model F) and the isotropic antiferromagnet (model G). As far as possible, the comparison of results obtained by the renormalization group theory with numerical simulations has been made.
The renormalization-group equations for critical behavior in $4\ensuremath{-}\ensuremath{\epsilon}$ dimensions are generalized to the discussion of dynamic exponents at T=TcT={T}_{c}T=Tc​ and then applied to a situation recently considered by Hohenberg, Halperin, and Ma (HHM); namely, one in which an nnn-component primary field $\ensuremath{\psi}$ is coupled to a secondary field $\ensuremath{\phi}$ via a ${\ensuremath{\lambda}}_{0}(\ensuremath{\psi}\ensuremath{\psi})\ensuremath{\phi}$ coupling. In this work their analysis of relaxational fields is explicitly considered at order ${\ensuremath{\epsilon}}^{2}$. For n<4n<4n<4, we find the dynamic exponents differ in one case at $O({\ensuremath{\epsilon}}^{2})$ from that given by HHM. In contrast to HHM, the dynamic scaling postulate is also preserved by the second-order fixed points in all instances and detailed analysis is given. The fixed-point values of RRR, a dimensionless ratio of relaxation rates for the $\ensuremath{\phi}$ and $\ensuremath{\psi}$ fields, in certain cases, is found to go as ${R}^{*}\ensuremath{\sim}\frac{1}{\ensuremath{\epsilon}}$ which is a new result. This large value where it occurs is found essential to understanding dynamic scaling. Analysis of the case of a propagating conserved $\ensuremath{\phi}$ field also is given. It is found that its dynamic critical properties can be characterized by its damping term alone.
This article concludes a series of papers [Folk, Holovatch, and Moser, Phys. Rev. E 78, 041124 (2008); 78, 041125 (2008); 79, 031109 (2009)] where the tools of the field theoretical renormalization group were employed to explain and quantitatively describe different types of static and dynamic behavior in the vicinity of multicritical points. Here we give the complete two-loop calculation and analysis of the dynamic renormalization-group flow equations at the multicritical point in anisotropic antiferromagnets in an external magnetic field. We find that the time scales of the order parameters characterizing the parallel and perpendicular ordering with respect to the external field scale in the same way. This holds independent whether the Heisenberg fixed point or the biconical fixed point in statics is the stable one. The nonasymptotic analysis of the dynamic flow equations shows that due to cancellation effects the critical behavior is described, in distances from the critical point accessible to experiments, by the critical behavior qualitatively found in one-loop order. Although one may conclude from the effective dynamic exponents (taking almost their one-loop values) that weak scaling for the order parameter components is valid, the flow of the time-scale ratios is quite different, and they do not reach their asymptotic values.
We calculate the relaxational dynamical critical behavior of systems of O(n_{ parallel}) plus sign in circleO(n_{ perpendicular}) symmetry including conservation of magnetization by renormalization group theory within the minimal subtraction scheme in two-loop order. Within the stability region of the Heisenberg fixed point and the biconical fixed point, strong dynamical scaling holds, with the asymptotic dynamical critical exponent z=2varphinu-1 , where varphi is the crossover exponent and nu the exponent of the correlation length. The critical dynamics at n_{ parallel}=1 and n_{ perpendicular}=2 is governed by a small dynamical transient exponent leading to nonuniversal nonasymptotic dynamical behavior. This may be seen, e.g., in the temperature dependence of the magnetic transport coefficients.
The renormalization-group recursion relations are solved for the effective Hamiltonians relative to phase transitions with four-component order parameters. For this value of n there are 22 types of Hamiltonians which can be classified into two categories according to the action of their normalizer GN{G}_{N}GN​ on the corresponding parameter space (GN{G}_{N}GN​ is the symmetry group leaving globally invariant this space). In the first case, GN{G}_{N}GN​ generates a finite number of isolated fixed points whose characteristics can be deduced from the detailed investigation of five Hamiltonians only.In the second category, for which GN{G}_{N}GN​ is a continuous group, there are, in addition to isolated fixed points, continuous manifolds of physically equivalent fixed points (the dimension of the manifolds is either one or three). In the search for a stable fixed point, the continuous manifolds can be ignored, while the isolated points are related to the five former Hamiltonians. For n=4, it is necessary to solve the recursion relations to two-loop order. The only possible stable ones among the fixed points then arise from a splitting of points which coincide, to one-loop order, with the isotropic fixed point. Extending, to two-loop order, a result recently established to the preceding order, we show that if a stable fixed point exists, it is unique. For n=4, the stable fixed point has one of three possible symmetries : di-icosahedral, hypercubic, or dicylindrical.Despite this anisotropy of the critical fluctuations, the exponents associated with any of the stable fixed points are identical to order ${\ensuremath{\epsilon}}^{2}$ to the ``isotropic'' exponents corresponding to n=4. The cubic point is destabilized by any operator of symmetry lower than cubic. The dicylindrical one remains stable with respect to certain anisotropies of lower symmetry. We examine the available experimental data in light of the preceding theoretical results concerning the critical behavior and the thermodynamic order of the transitions. On the other hand, we establish two general symmetry conditions relative to the stable fixed points determined by the renormalization-group equations. The first one specifies group theoretically, for each value of n, the possible symmetries Gi∗{G}_{i}^{\mathrm{*}}Gi∗​ of the stable fixed points. The second one formulates a necessary condition for the occurrence of an anisotropic stable fixed point: The normalizer GN{G}_{N}GN​ of the considered parameter space must fulfill the condition GN{G}_{N}GN​\ensuremath{\subset}@;BGi∗{\mathrm{BG}}_{i}^{\mathrm{*}}BGi∗​ for one, at least, of the former Gi∗{G}_{i}^{\mathrm{*}}Gi∗​ groups. These rules are shown to be very restrictive for n=4: On the basis of symmetry the lack of a stable fixed point can be asserted for 10 Hamiltonians out of 22, without solving the fixed-point equations.