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Chinese Physics B

Coherent control of negative refraction based on local-field enhancement and dynamically induced chirality

Nuo Ba, Gao Jin-Wei, Xing-Xia Tian, Wu Xi, Wu Jin-Hui

Published Jul 1, 2010• 2 citations
Publisher

Abstract

This paper studies the electromagnetic response of a coherently driven dense atomic ensemble to a weak probe. It finds that negative refraction with little absorption may be achieved in the presence of local-field enhanced interaction and dynamically induced chirality. The complex refractive index governing the probe refraction and absorption depends critically on the atomic density, the steady population distribution, the coherence dephasings, and the frequency detunings, and is also sensitive to the phase of the driving field because the photonic transition paths form a close loop. Thus, it can periodically tune the refractive index at a fixed frequency from negative to positive values and vice versa just by modulating the driving phase. Moreover, the optimal negative refraction is found to be near the probe magnetic resonance, which then requires the electric fields of the probe and the drive being on two-photon resonance due to the dipole synchronisation.

DOI
10.1088/1674-1056/19/7/074208

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•Dec 1, 2011•0 citations
This paper studies the electromagnetic response of a coherently driven dense atomic ensemble to a weak probe. It finds that negative refraction with little absorption may be achieved in the presence of local-field enhanced interaction and dynamically induced chirality. The complex refractive index governing the probe refraction and absorption depends critically on the atomic density, the steady population distribution, the coherence dephasings, and the frequency detunings, and is also sensitive to the phase of the driving field because the photonic transition paths form a close loop. Thus, it can periodically tune the refractive index at a fixed frequency from negative to positive values and vice versa just by modulating the driving phase. Moreover, the optimal negative refraction is found to be near the probe magnetic resonance, which then requires the electric fields of the probe and the drive being on two-photon resonance due to the dipole synchronisation.
This research focuses on a coherently driven four-level atomic medium with the aim of inducing a negative index of refraction while taking into consideration local field corrections as well as magnetoelectric cross coupling (i.e.,chirality) within the material's response functions. Two control fields are used to render the medium transparent for a probe field which simultaneously couples to an electric and a magnetic dipole transition, thus allowing one to test the permittivity and permeability of the material at the same time. Numerical simulations show that a negative index of refraction with low absorption can be obtained for a range of probe detunings while depending on number density and the ratio between the intensities of the control fields.
We show that negative refraction with minimal absorption can be obtained by means of quantum interference effects similar to electromagnetically induced transparency (EIT). Coupling a magnetic dipole transition coherently with an electric dipole transition leads to electromagnetically induced chirality, which can provide negative refraction without requiring negative permeability and also suppress absorption. This technique allows negative refraction in the optical regime at densities where the magnetic susceptibility is still small and with refraction/absorption ratios that are orders of magnitude larger than those achievable previously. Furthermore, the refractive index can be fine-tuned, which is essential for practical realization of subdiffraction-limit imaging. As with EIT, electromagnetically induced chirality should be applicable to a wide range of systems.
Abstract We investigate the electromagnetic chirality and negative refraction in a concentric nanoshell of a chiral metal sphere and a chiral atomic shell. The medium of the atomic shell with a four-level system is driven by a laser field and an incoherent pump field in a diamond configuration. We show that the electric and magnetic absorption spectra connecting through the chiral coefficients of the respective dipole moments of the two media, produce five and three lines spectral profiles. We explain that the spectral lines separated by dips are the manifestation of the classical (quantum) coherence effect of the wave field excitation in the medium of the metal sphere (atomic shell), and the interaction of the respective dipole moments at the interface of the two media. Furthermore, we show negative refraction with zero absorption without requiring permittivity (ϵ) and permeability (μ) simultaneously negative, where for all values of the incident wavelength, Re [μ] ≈ 1, representing a strong chiral electromagnetic behavior. Consequently, the negative refractive index enhances sufficiently beyond n = −1 for a wide range of parameters depending on the coupling parameters, chiral coefficients, and the radii ratio of the concentric metal-atomic nanoshell.
Enhancement and control of the index of refraction in a mixture of two three-level atomic species that form a pair of far-detuned $\ensuremath{\Lambda}$ schemes under two-photon resonance has been studied. We employ the density-matrix approach to properly take population relaxation into account and to describe the interaction of each $\ensuremath{\Lambda}$ system with the electromagnetic fields. Both $\ensuremath{\Lambda}$ systems are driven by a corresponding far-detuned coherent field at one atomic transition and are probed by the same weak field. In the dressed-state basis, it represents a superposition of effective two-level subsystems with the positions, widths, and amplitudes of the resonances controlled by the driving fields and allows for efficient control of the susceptibility of the total system; leading to refractive index (RI) enhancement with vanishing absorption in the absence of amplification. We analyze the experimental implementation of such a system in a cell of Rb atoms with a natural abundance of isotopes. An upper limit estimate of the RI enhancement is obtained.
We discuss the feasibility of negative refraction with reduced absorption in coherently driven atomic media. Coherent coupling of an electric and a magnetic dipole transition by laser fields induces magnetoelectric cross coupling and negative refraction at dipole densities which are considerably smaller than necessary to achieve a negative permeability. At the same time the absorption gets minimized due to destructive quantum interference and the ratio of negative refraction index to absorption becomes orders of magnitude larger than in systems without coherent cross coupling. The proposed scheme allows for a fine tuning of the refractive index. We derive a generalized expression for the impedance of a medium with magnetoelectric cross coupling and show that impedance matching to vacuum can easily be achieved. Finally we discuss the tensorial properties of the medium response and derive expressions for the dependence of the refractive index on the propagation direction.
The resonant absorption, emission, and scattering of light are the fundamental optical processes that have been used both to probe matter and to manipulate light itself. In the last decade there has been essential progress in coherent control of both linear and nonlinear optical responses based on resonant excitation of atomic coherence in multilevel quantum systems. Some interesting and useful phenomena, resulting from coherent control of absorption and the group index, such as electromagnetically induced transparency, lasing without inversion, and ultra-slow group velocity of light have been widely studied. This work is focused on coherent control of refractive index and resonant fluorescence in multilevel medium. \n \nWe suggest two promising schemes for resonant enhancement of the refractive index with eliminated absorption and propose their implementation in transition element doped crystals with excited state absorption and in a cell of Rb atoms at natural abundance. We show how to use one of these schemes for spatial variation of the refractive index via its periodic resonant increase/decrease, remarkably keeping at the same time zero absorption/gain. It opens the way to production of transparent photonic structures (such as distributed Bragg reflectors, holey fibers, or photonic crystals) in a homogeneous resonant atomic media such as dielectrics with homogeneously distributed impurities, atomic, or molecular gases. These optically produced photonic structures could easily be controlled (including switching on/off, changing amplitude and period of modulation) and would be highly selective in frequency, naturally limited by the width of the optical resonance. \n \nWe also derive the optical fluorescence spectra of a three-level medium driven by two coherent fields at the adjacent transitions in a general case when all three transitions are allowed. We show that coherent driving can efficiently control the distribution of intensities between the fluorescent channels. In particular, the total intensity of fluorescence at the transition which is not driven by the optical fields may essentially exceed the fluorescence intensity at the driven transitions under the condition of two-photon resonance. This counter-intuitive effect is due to depletion of the intermediate state via atomic interference.