We calculate the far-field intensity pattern of superradiant emission from an optically thin ensemble of atomic oscillators excited by a spatially nonuniform laser pulse of large Rabi area. As the excitation intensity is increased, the superradiant field develops ring structure and expands due to self-diffraction. This effect is made manifest by a two-pulse photon echo experiment where the second pulse is spatially much broader than the first and has a small Rabi area. As a function of the intensity of the first excitation pulse, we measure the on-axis and off-axis echo intensity and find, in agreement with our calculations, that the two behave differently. We also show that for a random, sufficiently smooth excitation profile, the total power of cooperative emission is proportional to the integral, over the excited volume, of the induced dipole moment squared.
A theoretical model for superradiant damping effect in inhomogeneously broadened media and its application to photon-echo problems are discussed. Only optically thin systems are considered, and all nonradiative relaxation mechanisms are neglected. Numerical calculations are performed for a very wide square inhomogeneous line shape and square applied pulses. It is shown that excitation of the system becomes increasingly difficult as the superradiant lifetime ${\ensuremath{\tau}}_{s}$ becomes comparable with
T2∗. The energy reradiated after the end of the exciting pulse is considerable for ${\ensuremath{\tau}}_{s}\ensuremath{\approx}{T}_{2}^{*}$ and for some applied pulse areas. Two-pulse sequences produce multiple echoes as the microscopic polarizations spontaneously rephase. The first-echo amplitude maximum is found to occur for first-applied-pulse areas increasingly above $\frac{1}{2}\ensuremath{\pi}$ as ${\ensuremath{\tau}}_{s}$ decreases. For a given first-pulse area, the echo intensities increase initially as ${\ensuremath{\tau}}_{s}$ decreases (negligible damping) and finally decrease and vanish (important damping). The ratio of the second- to first-echo amplitudes is found to be proportional to $\frac{{T}_{2}^{*}}{{\ensuremath{\tau}}_{s}}$ for small superradiance levels and to decrease when ${\ensuremath{\tau}}_{s}$ approaches
T2∗. An approximate estimate of this ratio is derived for the region of linearity in $\frac{{T}_{2}^{*}}{{\ensuremath{\tau}}_{s}}$.
A collection of
N Rydberg atoms and a resonant millimeter-wave cavity are shown to exchange energy back and forth at a rate $2(\frac{d}{\ensuremath{\hbar}}){\mathcal{E}}_{0}\sqrt{N}$, where
d is the electric dipole matrix element of the atomic transition and
E0 the "field per photon" in the cavity. This experiment is a demonstration of self-induced Rabi oscillations in a two-level atom system coupled to a single electromagnetic field mode and can also be considered as a very simple illustration of "ringings" in superradiant emission.
A theoretical model for the propagation of coherent light pulses in resonant media where a large number of atoms cooperate in spontaneous emission (superradiance) is discussed. The medium is supposedly free of inhomogeneous broadening, and no lossy relaxation mechanisms are taken into account. The conditions for the emission of all spontaneous radiation in the direction of pulse propagation are described. A semi-classical model is used and, at each point in the medium, the propagation field and the spontaneous damping field are considered separately. The equation governing the evolution of a superradiant system in the presence of an applied pulse is derived. A mechanism of energy transfer from the traveling pulse to the medium is described which includes superradiant spontaneous emission effects. As a result of the neglect of all lossy relaxation processes, all energy stored in the medium is eventually returned to the pulse by coherent spontaneous emission. Therefore, in this theory, all pulses travel through the medium without energy loss. Numerical results for square input pulses are discussed which show two possible types of propagation behavior: (a) Low input intensities produce a negative tail to the input (positive) pulse and sharpening of the tail with the advance in the medium; (b) higher input intensities produce, after sufficient penetration, a steady-state pulse envelope somewhat similar to the $2\ensuremath{\pi}$ pulses of self-induced transparency. The steady-state solutions of the equations of motion are found numerically and the pulse shapes are computed for different degrees of superradiance. In the limit of strong superradiance, very asymmetric pulse envelopes of large area are found. For negligible superradiance, approximately $2\ensuremath{\pi}$ hyperbolic-secant pulses are obtained. The effects of inhomogeneous broadening are briefly considered, and the consequences of important superradiant damping in photon-echo experiments are qualitatively discussed.
We report the experimental observation of a superradiant emission emanating from an elongated dense ensemble of laser cooled two-level atoms, with a radial extent smaller than the transition wavelength. In the presence of a strong driving laser, we observe that the system is superradiant along its symmmetry axis. This occurs even though the driving laser is orthogonal to the superradiance direction. This superradiance modifies the spontaneous emission, and, resultantly, the Rabi oscillations. We also investigate Dicke superradiance in the emission of an almost fully inverted system as a function of the atom number. The experimental results are in qualitative agreement with ab-initio, beyond-mean-field calculations.
Summary form only given. The radiative behavior of an ensemble of correlated atoms can be dramatically different from that of a single atom. Correlation, for example, can give rise to sub- or superradiant emission. Experimental studies of the fascinating correlative effects expected have been severely constrained by difficulties in creating suitably correlated media and by propagation effects that perturb correlation during emission. We have found that optical cavities of moderate reflectivity and very short ring-down time can be employed to "accelerate" the superradiant process and bring it to dominance in media sufficiently dilute so that propagation effects both in excitation and emission are absent. For the first time, it is possible to observe strong optical superradiance under the pure and simple conditions that were originally envisioned. Note that superradiance here does not refer to the emission of initially inverted atomic samples (i.e. superfluorescence), but to cooperative emission from samples of atoms prepared in correlated superposition states. Moreover, the cavity accelerated superradiant system is found to display heretofore unknown nonlinear behavior in terms of its effect on the "area" of injected optical pulses.
In order to study the cooperative emission of radiation from an extended system of
N two-level atoms, we use the master-equation approach within the Born and Markov approximations. All the properties of the emission of radiation can be deduced from the diagonalization of the coupling matrix $\ensuremath{\Gamma}$, where an element ${\ensuremath{\Gamma}}_{\mathrm{jk}}$ gives the coupling between the atoms labeled
j and
k via the electromagnetic field. We choose a pencil-shaped volume and study analytically the coupling matrix in the limit for small and large Fresnel numbers. For Fresnel numbers of order unity numerical methods are used. Thus we prove that, for the pencil-shaped geometry, any elaborated model must take into account the interaction of the atoms with the infinity of electromagnetic field modes lying inside two small solid angles about the axis of the largest linear dimension, which we label the
z axis. In other words, the intensity of radiation emitted by any atom of the system depends on its position with respect to the others and this "propagation effect" cannot be neglected when interpreting superradiance experiments. For small Fresnel numbers the
z dependence predominates, in the opposite case the (
x,y) dependence does, while for Fresnel numbers of order unity the dependence of all three components must be taken into account. Preliminary calculations are given for which only the
z dependence is considered; for Fresnel numbers of magnitude of order unity or smaller, the effect of propagation along the
z axis displays large delays for the appearance of superradiance with respect to the time at which the superradiant pulse is maximum when the "propagation effects" are neglected (one-mode model).