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IEEE Journal of Quantum Electronics

Gain nonlinearity in inhomogeneously broadened laser media

V R Belan, V V Grigor'yants, M. L. Gurari, M. E. Zhabotinski, N. Otradinskaja

Published Jun 1, 1969• 0 citations
Publisher
DOI
10.1109/jqe.1969.1081970

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This chapter begins with a heuristic derivation of atomic population rate equations which include changes to level populations due to stimulated transitions as well as level relaxations and pump. These equations are used to study the saturation of population inversion with increasing light intensity and its dependence on the type of gain medium (three-level gain media vs. four-level gain media), lineshape and nature of line broadening (homogeneous vs inhomogeneous broadening). How saturation affects lineshape and thus gain and absorption giving rise to phenomena like power broadening and spectral hole burning is also discussed. The chapter summarizes the equations of motion for atomic polarization, inversion and the cavity field describing their nonlinear dynamical coupling. These equations, known as the Maxwell-Bloch equations, provide a complete description of atom-field interaction in a laser. Approximations of these equations, including the rate equation approximation, to deal with different laser classes are briefly described. These will be used in the next few chapters to explore and understand the rich and varied behavior of lasers. The chapter ends with a summary of select gain media for different types of commonly used lasers.
Coherent amplification of short-pulse XeCl lasers is studied theoretically by using multilevel Maxwell–Bloch equations in which the vibrational–rotational structures of a XeCl gain spectrum are included. The model used considers 100 transitions each in the P and R branches for six different vibrational transitions of XeCl(B, υ = 0) → XeCl(X, υ′ = 0–5). Coherence components between sublevels in the B and X states are also properly calculated. The model can successfully predict coherent effects such as a quantum beat caused by the spectrum overlap of the several vibrational–rotational transitions involved in a short-pulse laser spectrum. During amplification, laser pulses experience some nonlinear effects caused by the complex gain spectrum structure and by the coherent interactions; thus a considerable change in the laser pulse shape and a substantial reduction in the duration of the amplified laser pulse are predicted. The Frantz–Nodvik equation in the rate-equation limit and even single-level Maxwell–Bloch equations are not applicable for short-pulse propagation analyses in inhomogeneously broadened gain media.