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Physics Letters A

Spin correlations and Haldane gap in the S = 2 antiferromagnetic Heisenberg chain

Shoji Yamamoto

Published Apr 1, 1996• 29 citations
Publisher
DOI
10.1016/0375-9601(96)00106-5

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Haldane gap in S = 2 XXZ quantum antiferromagnet

Charudatt Kadolkar, Neena Goveas, Dipan K. Ghosh +1 more

Journal of Magnetism and Magnetic Materials•Jan 1, 1998•1 citation
Using the valence-bond-solid (VBS) approach and the Schwinger-boson mean-field approximation, we study the dependence of the Haldane gap of a spin-1 linear-chain Heisenberg antiferromagnet on impurity doping with different spins. The impurity spins affect the singlet pairing order parameter \ensuremath{\Delta} and the constraint factor \ensuremath{\lambda}. As a result, the Haldane gap is reduced by a factor \ensuremath{\sim}ni2/3{\mathit{n}}_{\mathit{i}}^{2/3}ni2/3​, with ni{\mathit{n}}_{\mathit{i}}ni​ as the impurity concentration, and eventually collapses at ni{\mathit{n}}_{\mathit{i}}ni​\ensuremath{\sim}1/\ensuremath{\xi} with \ensuremath{\xi} as the VBS correlation length. This theoretical prediction can be verified by neutron-scattering experiments.
The ground-state properties of the spin-1/2 Heisenberg chain, which has two exchange couplings (J>J') alternatingly, are studied. This model interpolates the spin-1 antiferromagnetic Heisenberg chain (AFHC) (J'\ensuremath{\rightarrow}-\ensuremath{\infty}, J>0), the dimerized spin-1/2 AFHC (J'\ensuremath{\simeq}J>0), and the uniform spin-1/2 AFHC (J'=J>0) continuously. The string order introduced by den Nijs--Rommelse and Tasaki changes continuously through the Haldane phase and the dimer phase to vanish at J=J'. It is at a maximum for J'=0. This implies that the string order is related to the local singlet correlation in terms of the spin-1/2 model. The lowest excitation can be regarded as the renormalized triplet wave. The reversal of the anisotropy effect on the excitation spectrum of the spin-1 AFHC is also explained in a intuitive way based on this picture.
The properties of the spin-1/2 double chain Heisenberg antiferromagnet are studied by means of the numerical diagonalization and the projector Monte Carlo simulation. The model consists of the two spin 1/2 antiferromagnetic quantum Heisenberg chains coupled with each other via the ferromagnetic interchain coupling J ′ . It is shown that the first excited state has a gap for large enough J ′ . This gap continues to the Haldane gap in the limit J ′ →∞, where spins on the different chains form triplets on each site. On the other hand, the gap decreases rapidly between J ′ =1.0 and 0.6 and is undetectable for J ′ <0.6 within the present accuracy.