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Review of Scientific Instruments

Pulsed source of metal atoms and their compounds

Dmitri A. Chestakov, Anna M. Zawadzka, David H. Parker, Konstantin V. Vidma, Alexey V. Baklanov, Sergei A. Kochubei

Published Jan 7, 2005• 2 citations
Publisher

Abstract

A pulsed source for production of metal atoms and their oxide compounds in a supersonic expansion is described. The design utilizes a simple pulsed valve and produces a concentration of 106–107atomspercm−3 of the desired metal atoms in a molecular beam. Depending on the carrier gas used, metal compounds at similar concentration levels can also be produced.

DOI
10.1063/1.1841952

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A pulsed source for production of metal atoms and their oxide compounds in a supersonic expansion is described. The design utilizes a simple pulsed valve and produces a concentration of 106–107atomspercm−3 of the desired metal atoms in a molecular beam. Depending on the carrier gas used, metal compounds at similar concentration levels can also be produced.
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This dissertation describes a general approach of generating a high flux of cold atoms that can be confined in a magneto-optical trap. As an alternative to the state-of-the-art laser cooling method, this approach widens our ability to cool and control atoms without relying on a specific atomic transition and availability of laser. In this dissertation I will discuss the design, construction of the experiment and characterization of a pulsed cold atom source in detail. This work is based on a new paradigm: entrainment of atoms in the carrier gas of a supersonic beam, followed by the magnetic deceleration and trapping. Our methodology is based on the supersonic beam created by the expansion of a dense carrier gas from a pulsed release of gas through a small aperture. Cold noble gas emerging from this pulsed high pressure supersonic nozzle acts as a carrier, into which atoms of interest are then entrained. In our studies with the lithium atoms, up to 10¹¹ atoms per pulse could be entrained into a supersonic beam of helium at a translation temperature of below 100 mK. The supersonic valve is typically operated at a rate of below 1 Hz in the experiment. A much larger flux can be achieved at a higher repetition rate. These atoms are moving at a speed of 500 ms⁻¹ and need to be decelerated almost to a complete stop, in order to be trapped and cooled to quantum degeneracy. A 2.5-meter long moving-trap magnetic decelerator with 480 coil pairs was built and characterized. Atoms moving at a speed around 500 ms⁻¹ were trapped and decelerated to various final velocities ranging from 400 ms⁻¹ to 50 ms⁻¹, at a resulting temperature of 30 mK and a flux of 10⁸ ~ 10⁹ atoms per pulse. This whole process takes place within only 10 ms, at a repetition rate of 100 Hz 10¹⁰ ~ 10¹¹ atoms can be delivered per second. This approach is very general compared to the laser cooling, since most atoms in the periodic table have a magnetic moment in their ground state or can be optically pumped to a long-lived para-magnetic metastable state. In this dissertation, I show the working principle of each component of our experiment and characterize the atom beam at multiple stages. I describe in detail the construction and optimization of our magnetic decelerator, and demonstrate the control and monitoring system with the experiment results. Also implemented in this work is a flexible laser system that is composed of a reference diode laser and two tapered amplifiers to control and probe the internal states of atoms, as well as provide the trapping force. I also explore the optical molasses and chirped cooling techniques which help load the atoms into a magneto-optical trap. The successful demonstration of this method of creating a cold atom source leads us to believe that the magnetically decelerated supersonic atoms will play an important role in the area of cold atom physics
A molecular beam source for high-energy metastable atoms, utilizing a corona discharge, is described. It was designed for scattering experiments where accurate alignment of beam components is required. The metastable atoms produced in this source have kinetic energies from 5 to 74 eV dependent on the species and sufficient velocity selection to reveal structure in the differential cross sections. These high-energy metastables were previously reported as photons. When the molecular beam source was operated at 200–300 Torr, a supersonic beam of metastables was produced. An optimization of operating conditions produced a supersonic beam flux two orders of magnitude greater than previously reported.
Abstract An intense source of cold hydrogen atoms in a supersonic beam is presented. H and D atoms are produced from pure samples of H2 and D2 using a barrier discharge near the orifice of a cryogenic pulsed valve. The atoms are entrained in the supersonic expansion of the precursor molecules and cool down to translational temperatures as low as ∼ 15 mK. The H-atom density at a distance of 1.2 m from the valve orifice is estimated to be around 108 cm−3. The mean velocity of the supersonic beam containing the H (D) atoms can be adjusted between 2600 and 1200 m s−1 (between 1850 and 820 m s−1). The barrier discharge also produces H n + and D n + ions with n ranging from 2 to 8, which can be deflected off the beam by electric fields. The use of this H-atom source in spectroscopic measurements is demonstrated by an investigation of the Stark effect in the 1s–2s two-photon transition of H and D. A near-Fourier-transform-limited pulsed laser generating pulses of UV radiation of adjustable pulse length between 10 and 200 ns near 243 nm is used to record spectra with full resolution of the hyperfine structure in the s states, providing a textbook example of the Stark effect in the simplest set of near-degenerate states of one-electron atoms.