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Physical Review A

Measurements of mode-splitting self-pulsing in a single-mode, Fabry-Perot laser

Mari W. Maeda, N. B. Abraham

Published Dec 1, 1982• 51 citations
Publisher

Abstract

Self-pulsing of a single-mode laser has been studied with the use of the inhomogeneously broadened 3.51-\ensuremath{\mu}m transition in xenon. Time-averaged intensity power spectra, average power output, and real-time observations of intensity fluctuations have been recorded for various detunings of the Fabry-Perot cavity. Two forms of self-pulsing have been observed, both of which can be explained in terms of the phase locking of several frequencies which simultaneously exist in the same spatial mode, made possible by the rapid variations of the index of refraction in the high-gain medium. One form of such mode splitting occurs in the wings of the atomic response due to the variations in the inhomogeneously broadened anomalous dispersion. The second form can occur anywhere in the tuning range of the laser as it is caused by distortions induced in the dispersion by the hole-burning effects of the oscillating mode. The pulsation frequency of this induced mode splitting varies with cavity tuning, shows a dip at the atomic line center, and may be absent for detuning of one or two homogeneous linewidths away from center. The instabilities have shown subharmonic bifurcations of the pulsation frequencies. Both high-$Q$ pulsation frequencies and broad bands of frequencies in the power spectra have been observed for various operating conditions.

DOI
10.1103/physreva.26.3395

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Self-pulsing of a single-mode laser has been studied with the use of the inhomogeneously broadened 3.51-\ensuremath{\mu}m transition in xenon. Time-averaged intensity power spectra, average power output, and real-time observations of intensity fluctuations have been recorded for various detunings of the Fabry-Perot cavity. Two forms of self-pulsing have been observed, both of which can be explained in terms of the phase locking of several frequencies which simultaneously exist in the same spatial mode, made possible by the rapid variations of the index of refraction in the high-gain medium. One form of such mode splitting occurs in the wings of the atomic response due to the variations in the inhomogeneously broadened anomalous dispersion. The second form can occur anywhere in the tuning range of the laser as it is caused by distortions induced in the dispersion by the hole-burning effects of the oscillating mode. The pulsation frequency of this induced mode splitting varies with cavity tuning, shows a dip at the atomic line center, and may be absent for detuning of one or two homogeneous linewidths away from center. The instabilities have shown subharmonic bifurcations of the pulsation frequencies. Both high-QQQ pulsation frequencies and broad bands of frequencies in the power spectra have been observed for various operating conditions.
We use the semiclassical strong-signal theory of the laser to predict and explain the onset of side-mode buildup in lasers with one oscillating mode. Two general categories are considered: one for which the side modes and the oscillating mode all have the same wavelength and the other for which they have different wavelengths. The treatments include an arbitrary amount of inhomogeneous broadening. Our approach unifies the treatments of the side-mode instabilities presented earlier and extends them to handle standing waves in addition to the previously treated running waves. We write the field and the population matrix elements as Fourier series in the adjacent-mode beat frequency. This approach has been used extensively in both multimode laser theory and saturation spectroscopy. This technique coincides with linear stability analyses used by others, provided that our beat frequency includes a contribution that is proportional to the complex side-mode gain. We give a solution that allows for detuned operation along with its simpler, centrally tuned special case. The connection with saturation spectroscopy clearly reveals that the side-mode instabilities require side-mode gain. For the single-wavelength case, nonlinear anomalous dispersion is also required. The side-mode gain and dispersion result from both inhomogeneous broadening and population pulsations. The lowest instability thresholds occur when both of these mechanisms play a role. The approach can also be used to treat instabilities in optical bistability by substituting the appropriate equation of state for the strong-mode intensity and by changing the sign of the absorption coefficient. In homogeneously broadened, standing-wave lasers, we show that multiwavelength instabilities depend strongly on the position of the medium in the cavity. We illustrate the theory by giving numerical results for the output pulsation frequency and for the instability threshold by using parameters that are appropriate for the He–Xe laser. These results correlate well with experimental observations.
Homogeneously broadened lasers are considered as intrinsically single mode monostable devices [1] where intensity and frequency are defined by the cavity mode that lies nearest to the center of the atomic line. Here we show theoretically and experimentally that this heuristic picture falls when the interaction between different cavity modes becomes relevant. In fact, for sufficiently high detuning between cavity and atomic resonance frequencies (δAC), self pulsing of the laser arise from the simultaneous operation in two modes (phase instability) even if it is operating near threshold (C ⪯ 1) and in the so-called good cavity limit (k ≪ γ⊥, γ‖). Using parameter values which are typical of many solid state and molecular gas lasers (γ‖, k ≪ γ⊥), the theory predicts a bistable behavior in both the output intensity and frequency, as δAC is varied (Fig. 1). These theoretical results have been confirmed by experiments carried out on a CO2 laser where the distance between modes was controlled by changing the losses inside the cavity and the detuning δAC was varied by a fine tuning of the distance between mirrors. The output intensity versus δAC is shown in Fig. 2 for two different values of losses and gas pressure. Direct comparison between Fig. 2b) and Fig. 1 shows a good qualitative agreement. Measurements of the transients during the jump of Fig.2b) confirmed the mode-mode competition interpretation.
The instabilities in homogeneously broadened lasers, which we described in the previous chapter, have a paradigmatic importance because they arise in models which allow one to perform the linear-stability analysis in a simple analytic form. The treatment of the corresponding instabilities in the case of in homogeneously broadened lasers is substantially more complex in general. However, it is very interesting because, as we shall see, the instabilities arise in parametric domains that are much more accessible from the experimental viewpoint. A related issue is that of the possibility of multimodal emission in a laser. It is common knowledge that in order to attain multimode emission it is necessary to have a sort of in homogeneity in the gain medium, because in a completely homogeneous configuration all modes interact with all atoms, and the arising competition among modes implies that only one of them survives. There are basically two main kinds of in homogeneity, the first is of spatial nature and the other is of spectral nature. The first kind is realized in Fabry–Perot lasers, because different cavity modes interact with atoms at different spatial positions in the cavity thanks to the standing-wave configuration of the field and to the consequent phenomenon of spatial hole- burning (see Section 14.2 and Fig. 14.1). This circumstance is capable of weakening the mode–mode competition and allowing multimode operation. In unidirectional ring lasers, on the other hand, there is an “inhomogeneous” configuration in the case of inhomogeneous broadening, because different groups of atoms have different transition frequencies and therefore interact with different modes thanks to the spectral hole-burning (see Section 15.2 and Fig. 15.3). Again, this weakens the mode–mode competition and allows multimode operation. However, these are qualitative considerations, and the only reliable and quantitative method to determine the possibility of multimodal operation is the linear-stability analysis of the single-mode stationary solutions.
Population pulsations are fluctuations in the population difference (of a two level system) due to the presence of two or more coherent waves interfering in the medium. In this work, we show that population pulsations generated by three waves, a central wave and two mode-locked sidebands, are responsible for both the multiwavelength and the single-wavelength instabilities of single-mode lasers containing homogeneously-broadened media. The role of the population pulsations in establishing these instabilities, however, diminish as the central mode is detuned away from the atomic resonance frequency. For homogeneously-broadened lasers, we find two regions of single-wavelength instability. The first is at line center, for which population pulsations are solely responsible, and the second is off line center where the unsaturated medium provides the required gain and anomalous dispersion. For the case of inhomogeneously-broadened lasers, we show that population pulsations significantly increase the instability range over that predicted by Casperson for single-mode bad-cavity lasers. Both the unidirectional ring and the standing-wave cavities are treated. The Fourier expansion technique, used in this work, for treating three-frequency operation in saturation spectroscopy is shown to be equivalent (in appropriate limits) to the linear stability analysis in laser theory and optical bistability. We also show, in single-sideband saturation spectroscopy, that for long interaction lengths propagation effects can significantly influence the absorption and dispersion coefficients of the medium. Finally, we show that under certain conditions the pronounced splittind effects of the population pulsations develop into regions of intense absorption.
The optical spectra corresponding to complex intensity pulsation patterns near line-center tuning of single-mode, standing-wave gas lasers contain some simple indicators of the origins of their complexity. Heterodyne measurements show that on detuning of the laser the power density in each component of the optical spectrum undergoes a Lamb-dip-like reduction as it passes through resonance with the zero-velocity atoms. These observations help to explain the sensitive dependence of the dynamics of standing-wave gas lasers on detuning within the Lamp dip and distortions of the Lamb-dip shapes when the lasers are unstable.
Unstable and bistable behavior has been predicted recently in multimode homogeneously broadened lasers as a function of the detuning between the cavity and the atomic frequencies. As an example of a device for which most required physical conditions for the appearance of this instability are satisfied, we have analyzed the behavior of a low-pressure (10–20 Torr) CO2 laser. The operating parameters (relaxation rates for the population inversion, 104s−1, and for the polarization, 108s−1) restrict the accessible range of theoretically expected phenomena to a stable intensity output without evidence of stable self-pulsing. However, mode–mode competition is responsible for bistability in both the intensity and the operating frequency on varying the detuning parameter. This behavior is confirmed by additional observations of the transient that accompanies the jump between the two stable branches. We have also studied the effect of varying the cavity losses and discovered bistability also in the vicinity of the threshold for laser action. This kind of behavior is not predicted by the plane wave Maxwell-Bloch equations but can be explained in terms of a radial gain profile. Both effects—mode–mode competition and transverse—lead to a variety of bistable behaviors depending on gas pressure and discharge current.