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Journal of Physics B Atomic and Molecular Physics

The van der Waals force between positronium and light atoms

D W Martin, P A Fraser

Published Sep 14, 1980• 35 citations
Publisher

Abstract

The long-range interaction energies of H-Ps, Ps-He and Ps-Ps are calculated using the Hylleraas variational method. Implications for low-energy H-Ps and Ps-He scattering theory are discussed.
DOI
10.1088/0022-3700/13/17/017

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Positronium-hydrogen (Ps-H) scattering is of interest, as it is a fundamental four-body Coulomb problem. We have investigated low-energy Ps-H scattering below the Ps(n=2) excitation threshold using the Kohn variational method and variants of the method with a trial wavefunction that includes highly correlated Hylleraas-type short-range terms. We give an elegant formalism that combines all Kohn-type variational methods into a single form. Along with this, we have also developed a general formalism for Kohn-type matrix elements that allows us to evaluate arbitrary partial waves with a single codebase. Computational strategies we have developed and use in this work will also be discussed.With these methods, we have computed phase shifts for the first six partial waves for both the singlet and triplet states. The 1S and 1P phase shifts are highly accurate results and could potentially be viewed as benchmark results. Resonance positions and widths for the 1S-, 1P-, 1D-, and 1F-waves have been calculated.We present elastic integrated, elastic differential, and momentum transfer cross sections using all six partial waves and note interesting features of each. We use multiple effective range theories, including several that explicitly take into account the long-range van der Waals interaction, to investigate scattering lengths for the 1,3S and 1,3P partial waves and effective ranges for the 1,3S-wave.
The s-wave scattering parameters for the Positronium–Positronium (Ps–Ps) interaction are estimated semi-phenomenologically with the long-range van der Waals force and the short-range repulsive potential. The obtained values of the scattering length and the effective range are a ∼0.44 nm, and r 0 ∼0.2 nm for the symmetric channel. Stability of them is also checked with two kinds of potential with different parametrizations. Spin coupling schemes for the Ps–Ps system are discussed and the formulae of scattering length for each spin channel are derived. Using this value of the scattering length, the Gross-Pitaevskii equation can be fixed for the Positronium Bose-Einstein condensates (Ps BEC). The static properties of Ps BEC are discussed using the solutions of that equation. The critical temperature shift of the phase-transition due to the Ps–Ps interaction is also evaluated in the mean-field approximation.
A pseudopotential for positronium-atom interaction, based on electron-atom and positron-atom phase shifts, is constructed, and the phase shifts for Ps-Kr and Ps-Ar scattering are calculated. This approach allows us to extend the Ps-atom cross sections, obtained previously in the impulse approximation [I. I. Fabrikant and G. F. Gribakin, Phys. Rev. Lett. 112, 243201 (2014)], to energies below the Ps ionization threshold. Although experimental data are not available in this low-energy region, our results describe well the tendency of the measured cross sections to drop with decreasing velocity at v<1v<1v<1 a.u. Our results show that the effect of the Ps-atom van der Waals interaction is weak compared to the polarization interaction in electron-atom and positron-atom scattering. As a result, the Ps scattering length for both Ar and Kr is positive, and the Ramsauer-Townsend minimum is not observed for Ps scattering from these targets. This makes Ps scattering quite different from electron scattering in the low-energy region, in contrast to the intermediate energy range from the Ps ionization threshold up to $v\ensuremath{\sim}2$ a.u., where the two are similar.