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Journal of the Physical Society of Japan

S-Wave Scattering Parameters for Positronium-Positronium Interaction and Positronium Bose-Einstein Condensates

Kenji Oda, Takahiko Miyakawa, Hiroyuki Yabu, T. Suzuki

Published Jun 15, 2001• 23 citations
Publisher

Abstract

The s-wave scattering parameters for the Positronium–Positronium (Ps–Ps) interaction are estimated semi-phenomenologically with the long-range van der Waals force and the short-range repulsive potential. The obtained values of the scattering length and the effective range are a ∼0.44 nm, and r 0 ∼0.2 nm for the symmetric channel. Stability of them is also checked with two kinds of potential with different parametrizations. Spin coupling schemes for the Ps–Ps system are discussed and the formulae of scattering length for each spin channel are derived. Using this value of the scattering length, the Gross-Pitaevskii equation can be fixed for the Positronium Bose-Einstein condensates (Ps BEC). The static properties of Ps BEC are discussed using the solutions of that equation. The critical temperature shift of the phase-transition due to the Ps–Ps interaction is also evaluated in the mean-field approximation.

DOI
10.1143/jpsj.70.1549

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The s-wave scattering parameters for the Positronium–Positronium (Ps–Ps) interaction are estimated semi-phenomenologically with the long-range van der Waals force and the short-range repulsive potential. The obtained values of the scattering length and the effective range are a ∼0.44 nm, and r 0 ∼0.2 nm for the symmetric channel. Stability of them is also checked with two kinds of potential with different parametrizations. Spin coupling schemes for the Ps–Ps system are discussed and the formulae of scattering length for each spin channel are derived. Using this value of the scattering length, the Gross-Pitaevskii equation can be fixed for the Positronium Bose-Einstein condensates (Ps BEC). The static properties of Ps BEC are discussed using the solutions of that equation. The critical temperature shift of the phase-transition due to the Ps–Ps interaction is also evaluated in the mean-field approximation.
The s-wave scattering length for the Positronium-Positronium interaction is estimated semi-phenomenologically with the long-range van der Waals force and the short-range repulsive potential that represents the hard core between two positronium. The obtained value of the scattering length is a∼0.44nma \sim 0.44{\rm nm}a∼0.44nm, and its stability is also checked for different parametrizations. Using this value, the Gross-Pitaevskii equation can be fixed for the Positronium Bose-Einstein condensates (Ps BEC). The static properties of Ps BEC are studied from the solutions of that equation. The phase-transition temperature shift of the Ps BEC due to the Ps-Ps interaction is also evaluated with the mean-field approximation.
The stochastic variational method is used in conjunction with stabilization ideas to compute the low-energy s-wave phase shifts and scattering lengths for Ps-Ps scattering. The scattering lengths obtained were 8.44a0{8.44a}_{0}8.44a0​ for the singlet-singlet and 3.00a0{3.00a}_{0}3.00a0​ for the triplet-triplet states (the spin state refers to the coupling of the two electrons and the coupling of the two positrons in the system). The positive scattering length in the triplet-triplet channel means a stable Bose-Einstein condensate of triplet Ps atoms is physically possible. The large value of the ${}^{3}{\mathrm{Ps}}^{3}{\stackrel{\ensuremath{\rightarrow}}{\mathrm{Ps}}}^{1}{\mathrm{Ps}}^{1}\mathrm{Ps}$ cross section, $7.41\ensuremath{\pi}{a}_{0}^{2}$ suggests the use of spin-polarized positrons as advanced by Platzmann and Mills [Phys. Rev. B 49 454 (1994)].
Bose-Einstein condensates (BECs) of positronium (Ps) have been of experimental and theoretical interest due to their potential application as the gain medium of a $\ensuremath{\gamma}$-ray laser. Ps BECs are intrinsically spinor due to the presence of ortho-positronium (ooo-Ps) and para-positronium (ppp-Ps), whose annihilation lifetimes differ by three orders of magnitude. In this paper, we study the spinor dynamics and annihilation processes in the ppp-Ps/ooo-Ps system using both solutions of the time-dependent Gross-Pitaevskii equations and a semiclassical rate-equation approach. The spinor interactions have an O(4) symmetry which is broken to SO(3) by an internal energy difference between ooo-Ps and ppp-Ps. For an initially unpolarized condensate, there is a threshold density of $\ensuremath{\approx}{10}^{19}$ cm${}^{\ensuremath{-}3}$ at which spin mixing between ooo-Ps and ppp-Ps occurs. Beyond this threshold, there are unstable spatial modes accompanied by spin mixing. To ensure a high production yield above the critical density, a careful choice of external field must be made to avoid the spin mixing instability.
Projectile-elastic, target-elastic, and full close-coupling approximation models have been employed to investigate scattering of ortho-positronium off Li and Na atoms at low energies. Nine different basis sets for each system have been used to find the relative importance of atomic (target and projectile) states on the elastic scattering parameters and the convergence of the predicted results with added eigen- and pseudostates. The sss-wave elastic phase shifts, scattering lengths and cross sections of both the systems are reported upto the incident energy k=0.5a.u.k=0.5\phantom{\rule{0.3em}{0ex}}\text{a.u.}k=0.5a.u. and compared with the corresponding existing theoretical predictions. It has been found that the van der Waals and higher order long-range interactions play a crucial role in predicting sss-wave elastic parameters for Ps--alkali-metal-atom systems at low energies.
Abstract The production of a Bose–Einstein condensate made of positronium may be feasible in the near future. Below the condensation temperature, the positronium collision process is modified by the presence of the condensate. This makes the theoretical description of the positronium kinetics at low temperature challenging. Based on the quasi-particle Bogoliubov theory, we describe the many-body particle–particle collision in a simple manner. We find that, in a good approximation, the full positronium–positronium interaction can be described by an effective scattering length. Our results are general and apply to different species of bosons. The correction to the bare scattering length is expressed in terms of a single dimensionless parameter that completely characterizes the condensate.
A pseudopotential for positronium-atom interaction, based on electron-atom and positron-atom phase shifts, is constructed, and the phase shifts for Ps-Kr and Ps-Ar scattering are calculated. This approach allows us to extend the Ps-atom cross sections, obtained previously in the impulse approximation [I. I. Fabrikant and G. F. Gribakin, Phys. Rev. Lett. 112, 243201 (2014)], to energies below the Ps ionization threshold. Although experimental data are not available in this low-energy region, our results describe well the tendency of the measured cross sections to drop with decreasing velocity at v<1v<1v<1 a.u. Our results show that the effect of the Ps-atom van der Waals interaction is weak compared to the polarization interaction in electron-atom and positron-atom scattering. As a result, the Ps scattering length for both Ar and Kr is positive, and the Ramsauer-Townsend minimum is not observed for Ps scattering from these targets. This makes Ps scattering quite different from electron scattering in the low-energy region, in contrast to the intermediate energy range from the Ps ionization threshold up to $v\ensuremath{\sim}2$ a.u., where the two are similar.