Resonant two-photon pumping in the Cs 6s2S-7s2S transition has been used for 2.9 μm to 4550 Å image up-conversion. A power conversion efficiency of 20% with 1000 resolvable spots was achieved using a pump power of 8 kW. The pumping laser, Nd : lanthanum berylate, has a natural two-photon coincidence with the Cs 6s2S-7s2S transition.
We present a theoretical and experimental study of IR image upconversion using two-photon resonant optical four-wave mixing in alkali metal vapors. A closed form solution for the upconversion efficiency which includes Doppler broadening of the two-photon transition and a finite bandwidth pump laser is given. Experimental results for two types of image upconverters using Cs are presented. The first upconverts 2.94 μm to 4558 Å with a power efficiency of 32 percent and1.6 \times 10^{4}resolvable spots. The second is IR tunable, but of lower efficiency and resolution. Finally, the optimized characteristics of the Cs upconverter are compared to crystal upconverters and to the requirements of various applications.
Stimulated emission on the ultraviolet and blue transitions in Cs has been achieved by pumping via two-photon absorption and four-wave mixing for the pump transition 62S12→82D32,52. The emission performance of the optically pumped cesium vapor laser operating in ultraviolet and blue has been extended to 650 nJ/pulse for 387 nm, 1 to 3 μJ/pulse for 388 nm, 200 nJ/pulse for 455 nm, and 500 nJ/pulse for 459 nm. Emission performance improves dramatically as the cesium vapor density is increased, and no scaling limitations associated with energy pooling or ionization kinetics have been observed.
Diode-pumped alkali lasers, possessing high efficiency and narrow linewidth, can provide feasible solutions for wavelength ranges difficult to reach by commercial lasers. In this study, we investigate a generation of coherent blue light (CBL) via four-wave mixing (FWM)-based up-conversion processes in cesium (Cs) vapor. A bichromatic pumping scheme with 852- and 917-nm lasers drives the Cs atoms to the 6 D 5/2 excited level, followed by cascaded decay of 6 D 5/2 → 7 P 3/2 → 6 S 1/2 , producing 456-nm CBL under phase matching conditions. The fluorescence in multiple bands from blue to near- and far-infrared in the FWM process is demonstrated under different experimental conditions. To optimize the experimental parameters, we investigate the dependence of 456-nm CBL on the vapor temperature, frequency, and intensity of the two pump lasers. A maximum power of 2.94 mW is achieved with pump powers of 430 mW (for 852 nm) and 470 mW (for 917 nm). The corresponding conversion efficiency is 1.5%/W, three-fold higher than those in previous studies. Our results can contribute to fundamental research on atom—photon interactions and quantum metrology.
A study was made of the dependences of the efficiency of resonant parametric frequency conversion in sodium vapor on the infrared radiation wavelength, vapor density, and detuning from two-photon pump resonance. It was found in this conversion system that for each infrared wave the conversion efficiency had three maxima on tuning the frequency of two-photon pumping over the region of a forbidden transition. The principal maximum was realized for accurate two-photon resonance, and the two other maxima resulted from a rise in the cubic susceptibility close to single-photon sum-frequency resonances. A quantum efficiency of 35% was achieved for a 9.26 μ infrared wave.
We demonstrate highly efficient generation of coherent 420 nm light via up-conversion of near-infrared lasers in a hot rubidium vapor cell. By optimizing pump polarizations and frequencies we achieve a single-pass conversion efficiency of 260% per Watt, significantly higher than in previous experiments. A full exploration of the coherent light generation and fluorescence as a function of both pump frequencies reveals that coherent blue light is generated close to (85)Rb two-photon resonances, as predicted by theory, but at high vapor pressure is suppressed in spectral regions that do not support phase matching or exhibit single-photon Kerr refraction. Favorable scaling of our current 1 mW blue beam power with additional pump power is predicted.