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Il Nuovo Cimento

Shape and behavior of wave pulses

P. Gordon

Published Jun 1, 1964• 2 citations
Publisher
DOI
10.1007/bf02732791

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ACTA PHOTONICA SINICA•Jan 1, 2010•0 citations
We investigate the effects of the input laser beam’s temporal pulse shape on a forward degenerate four-wave mixing (FDFWM) signal, assuming two-level saturable absorbers. Under conditions in which the coherence time is far shorter than the pulse-duration, we can calculate the signal easily in the time and frequency domains. From this result it is shown that, when the pulse duration is longer than ten times the population relaxation time, the calculated signal intensity is almost the same as that obtained by assuming a steady state throughout duration of the laser pulse. With this assumption, we obtain the signal by summing all the steady-state signals at each time-domain grid point during the pulse. The calculation is performed with three input beam temporal pulse shapes: square, Gaussian, and typical Q-switched pulses. After reaching a maximum, the signal intensity decreases. The rates of the signal increase and decrease depend strongly on the temporal shape of the input beam. For the same average power, the square-pulse input saturates the absorber faster than the other pulses. These results indicate that the weak part of the pulse input plays an important role in generating the signal, yielding differences in saturation behavior of the signal intensity and the spectral line shape. We compare the calculations with experiments by fitting the saturation curve of the FDFWM signal of argon atoms in a radio frequency inductively coupled plasma. Also, the spectral line shape of the DFWM signal is fitted with the calculation by use of published experimental data.
Using the numerical solution of the full Maxwell-Bloch equations without the slowly varying envelope approximation and the rotating-wave approximation, propagation behavior of few-cycle laser pulse in a dense ladder-type three-level atomic medium is investigated and it is compared with the case in the corresponding dilute medium. It is found that, in the propagation process, time evolution of the pulse in the dense medium is obviously different from that in the dilute medium, and the difference will become more evident with increasing of the initial pulse area. When the initial pulse area is smaller, in the propagating process, the pulse shape in the dilute medium just have a small change; the pulse shape in the dense medium has considerable variation but the pulse splitting doesn't occur. When the initial pulse area is larger enough, for the dense medium case, the pulse splits into sub-pulses with different numbers and shapes at different propagation distances; while for the dilute medium case, variation of the pulse shape is still smaller in propagation process. The cause producing above difference is from two effects in the dense medium: the effect of the local-field correction (LFC) from the near dipole-dipole interaction and effect of stronger polarization field than that in the dilute medium. In which the effect of stronger polarization field plays a main role, but the role of LFC also cannot be neglected,and the stronger polarization field is due to the atomic density increasing .