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LASER-INDUCED ADIABATIC POPULATION TRANSFER IN ASYMMETRIC QUANTUM WELLS

Monica Gambhir, Siddhartha Lahon, PRADEEP KUMAR JHA, Man Mohan

Published Oct 1, 2009• 0 citations
Publisher

Abstract

The basic technique of stimulated Raman adiabatic passage for laser-induced adiabatic population transfer between discrete quantum states of an asymmetric double quantum well has been used in our study. The results show that the proper time-delay, overlap, and detuning of two pulses allows the coherent transfer between the states of a double quantum well system, leading to the possibility of implementation of semiconductor–based quantum logic gates and high efficiency optical switches. The impact of phase relaxation on the population transfer efficiency is also studied.

DOI
10.1142/s1793292009001769

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The basic technique of stimulated Raman adiabatic passage for laser-induced adiabatic population transfer between discrete quantum states of an asymmetric double quantum well has been used in our study. The results show that the proper time-delay, overlap, and detuning of two pulses allows the coherent transfer between the states of a double quantum well system, leading to the possibility of implementation of semiconductor–based quantum logic gates and high efficiency optical switches. The impact of phase relaxation on the population transfer efficiency is also studied.
Abstract The population transfer of a NaH molecule from the ground state X 1 Σ + to the target state A 1 Σ + via stimulated Raman adiabatic passage (STIRAP) is investigated. The results show that the intensity, delay time and detuning have a significant effect on population transfer. A large population transfer is observed with increased pump and Stokes intensity, especially when the pump and Stokes intensity match. Population transfer also depends on the delay time between the pump laser pulse and the Stokes laser pulse. The detuning of the two pulses influences the population transfer. Efficient population transfer can be realized under the resonant or two-photon resonant condition.
We investigate the effect of collision-induced coherence on coherent population transfer with the stimulated Raman adiabatic passage technique in a double A-type four-level system with a widely separated excited doublet. It is shown that when the two pulsed lasers with Rabi frequencies nearly comparable to the energy separation of the doublet are tuned to the particular frequency where the condition for quantum interference is satisfied, the very low transfer efficiency due to the nonadiabatic coupling between the two degenerate adiabatic states could be enhanced significantly with the increase of the collisional decay rates in a moderate range. The enhanced transfer efficiency results from the weakening of the nonadiabatic coupling between the two degenerate adiabatic states realized through collision-induced destructive quantum interference.
The authors discuss the technique of stimulated Raman adiabatic passage (STIRAP), a method of using partially overlapping pulses (from pump and Stokes lasers) to produce complete population transfer between two quantum states of an atom or molecule. The procedure relies on the initial creation of a coherence (a population-trapping state) with subsequent adiabatic evolution. The authors present the basic theory, with some extensions, and then describe examples of experimental utilization. They note some applications of the technique not only to preparation of selected states for reaction studies, but also to quantum optics and atom optics.
In atomic and molecular physics, coherent optical techniques allowing for almost complete ultrafast transfer of a population between different molecular eigenstates has been developed and refined for many years. One particularly successful scheme is called stimulated Raman scattering by delayed pulses (STIRAP). Within this scheme, it is possible to transfer a population between two nonoptically coupled states by using a third state (which is optically coupled to both the initial and the final state) without actually occupying it, in the end, at all. As for semiconductors, the question arises whether similar techniques can be used to transfer, for example, holes from the heavy-hole (HH) band to the light-hole (LH) band without creating electrons in the process. We have studied this problem theoretically and have identified parameter regimes where we believe the delayed-pulse scheme can be efficiently applied to the HH-LH population transfer.
Coherent manipulation of quantum states is of crucial importance in accurate control of a quantum system. A fundamental goal is coherently transferring the population of a desired state with near-unit fidelity. For this purpose, we theoretically demonstrate a novel coherent double-stimulated Raman adiabatic passage (STIRAP) in a three-level Λ-type system for realizing the switch of unequal initial preparations on two ground states. This operation uses a single optical pulse sequence accomplishing both bright-STIRAP and dark-STIRAP processes, in which the intermediate-level detuning and the pulse delay must be given an optimal adjustment. Besides, owing to the imperfection of double-STIRAP transition, the sensitivity of the switch fidelity with respect to the spontaneous loss from the intermediate state, to the pulse amplitude and to the population difference, is also discussed. This work suggests a simple and experimentally feasible all-optical approach to switch a superposition quantum state, serving as one-step closer to the goal of coherent manipulation of quantum systems.