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Physical Review A

Subrecoil cooling of Rydberg atoms

Eugeny Korsunsky, Yu. Rozhdestvensky

Published Oct 1, 1995• 7 citations
Publisher

Abstract

Two mechanisms for production of an ensemble of atoms in a highly excited state with very narrow distribution of the atomic center-of-mass momentum (cold Rydberg atoms) are proposed. The mechanisms are based on velocity-selective $\ensuremath{\pi}$ pulses and coherent population trapping in three-level cascade systems with the uppermost state being the Rydberg one. Both methods permit one to reach subrecoil temperatures of the Rydberg atoms.

DOI
10.1103/physreva.52.3027

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Two mechanisms for production of an ensemble of atoms in a highly excited state with very narrow distribution of the atomic center-of-mass momentum (cold Rydberg atoms) are proposed. The mechanisms are based on velocity-selective \ensuremathπ\ensuremath{\pi}\ensuremathπ pulses and coherent population trapping in three-level cascade systems with the uppermost state being the Rydberg one. Both methods permit one to reach subrecoil temperatures of the Rydberg atoms.
We show that an ensemble of atoms in highly excited states with narrow center-of-mass momentum distribution (cold Rydberg atoms) can be obtained with velocity-selective (pi) - pulses and laser cooling by velocity-selective coherent population trapping (VSCPT). Both methods use three-level cascade systems with the uppermost state being the Rydberg one where the atoms are excited and cooled. Very high fraction of atoms can be cooled to subrecoil temperatures by the use of VSCPT in standing light waves.
We demonstrate subrecoil cooling of rubidium atoms by velocity-selective coherent population trapping. By adiabatic transfer of the cooled atoms into a spin polarized single momentum state we show the coherence of the trapped state. Our cooling scheme takes advantage of the rubidium hyperfine structure to integrate subrecoil and sub-Doppler cooling. Starting from an initial velocity distribution of twice the recoil temperature $[{T}_{\mathrm{rec}}\phantom{\rule{0ex}{0ex}}=\phantom{\rule{0ex}{0ex}}(\ensuremath{\Elzxh}k{)}^{2}{/k}_{B}M]$, we cool down to 100 nK $(\ensuremath{\approx}\frac{1}{3}{T}_{\mathrm{rec}})$ within 1 ms, while almost completely suppressing the diffusive heating of velocity-selective coherent population trapping.
We report the first observation of subrecoil laser cooling in two dimensions by velocity selective coherent population trapping. We have compressed the momentum distribution of a cloud of trapped metastable helium atoms along two orthogonal axes to $\ensuremath{\delta}p=\frac{\ensuremath{\hbar}k}{4}$, where $\ensuremath{\hbar}k$ is the photon momentum. The corresponding temperature, 16 times below the single-photon recoil temperature, is 250 nK. Atoms are pumped into a nonabsorbing state exhibiting four well-resolved momentum peaks with subrecoil widths. The momentum space density in the peaks is significantly greater than that in the uncooled distribution.
One-dimensional velocity-selective coherent population trapping (VSCPT) in a cascade atomic configuration, with the second excited level a Rydberg state, is investigated through numerical calculations. The trapping efficiency for the case of travelling wave lasers is derived from the solution of the optical Bloch equations. For excitation by bichromatic standing waves, the energy-band approach is applied. Although the cooling process is limited by the spontaneous emission decay of the Rydberg state, the coexistence of polarization-gradient cooling and VSCPT in the case of standing waves allows the preparation of the majority of the atomic population in a cold Rydberg state.
We present a calculation of cooling of Rydberg atoms in bichromatic standing light waves. The atoms in our model are assumed to have a cascade three-level transition scheme, with the second excited level being the Rydberg state. The cooling fields, which also excite the atoms to the Rydberg state, consist of two standing waves whose frequencies are tuned near the two transition frequencies of the cascade atomic system. It is shown that the mechanisms of Sisyphus cooling and velocity-selective coherent population trapping can co-exist in such a configuration, and under certain conditions the majority of the laser-cooled atoms are in the Rydberg state.
Rydberg-Rydberg collisions in a cold, dense Rydberg gas can lead to the conversion of internal energy into center-of-mass energy of the colliding atoms, resulting in Rydberg-atom velocities much larger than the initial velocities in the gas. We prepare cold Rydberg-atom gases by laser excitation of laser-cooled atom clouds and use time-of-flight measurements to demonstrate the production of fast Rydberg atoms. The velocity distributions of Rydberg atoms emerging from the Rydberg-atom gases are obtained. State-selective field ionization spectra indicate a correlation between the production of fast Rydberg atoms and the presence of Penning ionization signatures. The dependence of the yield of fast Rydberg atoms on Rydberg atom density is measured.