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Quantum and Semiclassical Optics Journal of the European Optical Society Part B

Laser cooling of Rydberg atoms by velocity-selective coherent population trapping

Jingzhong Guo, Eugeny Korsunsky, E. Arimondo

Published Jun 1, 1996• 3 citations
Publisher

Abstract

One-dimensional velocity-selective coherent population trapping (VSCPT) in a cascade atomic configuration, with the second excited level a Rydberg state, is investigated through numerical calculations. The trapping efficiency for the case of travelling wave lasers is derived from the solution of the optical Bloch equations. For excitation by bichromatic standing waves, the energy-band approach is applied. Although the cooling process is limited by the spontaneous emission decay of the Rydberg state, the coexistence of polarization-gradient cooling and VSCPT in the case of standing waves allows the preparation of the majority of the atomic population in a cold Rydberg state.

DOI
10.1088/1355-5111/8/3/018

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ABSTRACT In this work we present an investigation of velocity-selective coherent population trapping (VSCPT) in asym- metric three-level schemes. The light force in such schemes is of an intrinsically transient character and shouldnot be described in a quasiclassical approach. Instead, results of the full quantum-mechanical calculations are presented with emphasis on their meaning to the efficiency of subrecoil laser cooling. 1 INTRODUCTION Laser cooling of neutral atoms has received significant advances by the introduction of velocity-selectivecoherent population trapping ((VSCPT) some years ago.1 Since it leads to atomic temperatures well below therecoil limit, studies of ultracold atoms and atomic interactions may be improved by magnitudes.The effect of VSCPT relies on optical pumping of atoms into a state WNC) which is a trap state for a certaincenter-of-mass velocity vO. This trap state is created by a destructive superposition of atomic states within amultilevel quantum system. Once being in such a state LWNC) the laser light does not interact anymore with theatom which leads to a decoupling with the rest of the system at vo. Atoms located outside this small velocityregion get a chance to be trapped by the momentum diffusion due to spontaneous emission of photons. Aftera sufficient long interaction time nearly all atoms are trapped inside a narrow momentum distribution whichcan be interpreted as cooling. The theoretical and experimental investigation of VSCPT is usually consideredby use of a three-level A-system as shown in Fig.1. Such a system can be found for example in a symmetrical

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Jan 1, 1996•0 citations
One-dimensional velocity-selective coherent population trapping (VSCPT) in a cascade atomic configuration, with the second excited level a Rydberg state, is investigated through numerical calculations. The trapping efficiency for the case of travelling wave lasers is derived from the solution of the optical Bloch equations. For excitation by bichromatic standing waves, the energy-band approach is applied. Although the cooling process is limited by the spontaneous emission decay of the Rydberg state, the coexistence of polarization-gradient cooling and VSCPT in the case of standing waves allows the preparation of the majority of the atomic population in a cold Rydberg state.
We show that an ensemble of atoms in highly excited states with narrow center-of-mass momentum distribution (cold Rydberg atoms) can be obtained with velocity-selective (pi) - pulses and laser cooling by velocity-selective coherent population trapping (VSCPT). Both methods use three-level cascade systems with the uppermost state being the Rydberg one where the atoms are excited and cooled. Very high fraction of atoms can be cooled to subrecoil temperatures by the use of VSCPT in standing light waves.
We present a calculation of cooling of Rydberg atoms in bichromatic standing light waves. The atoms in our model are assumed to have a cascade three-level transition scheme, with the second excited level being the Rydberg state. The cooling fields, which also excite the atoms to the Rydberg state, consist of two standing waves whose frequencies are tuned near the two transition frequencies of the cascade atomic system. It is shown that the mechanisms of Sisyphus cooling and velocity-selective coherent population trapping can co-exist in such a configuration, and under certain conditions the majority of the laser-cooled atoms are in the Rydberg state.
One-dimensional laser cooling based on velocity-selective coherent population trapping (VSCPT) has been investigated numerically through the solution of the optical Bloch equations and through a Monte Carlo analysis. The 1\ensuremath{\rightarrow}1 and 2\ensuremath{\rightarrow}2 transitions have been examined as a function of the atomic recoil frequency, the spontaneous-emission decay rate, and the Rabi frequency of the cooling laser. It has been found that for a large set of those parameters, the VSCPT cooling process may be described through scaling-law relations. The scaling laws are not valid at long atom-laser interaction times or large Rabi frequencies, where the atomic Doppler shift plays a significant role in the atomic motion evolution. Similar results for two atomic transitions suggest the validity of the scaling law for any one-dimensional VSCPT process. \textcopyright{} 1996 The American Physical Society.
One-dimensional laser cooling based on velocity-selective coherent population trapping (VSCPT) on a ${2}_{g}\ensuremath{\rightarrow}{1}_{e}$ transition has been investigated numerically through the solution of the optical Bloch equations. As in the work of G. Morigi et al. [Phys. Rev. A 53, 2616 (1996)], it has been found that for a large set of atomic and laser parameters, the VSCPT cooling process may be described through scaling-law relations. The scaling laws are based on the relations between the loss rates at large atomic momentum and their dependence on the momentum around zero value. The role of the laser detuning on the VSCPT trapping efficiency has been examined and scaling laws including the detuning have been derived.
ABSTRACT In this work we present an investigation of velocity-selective coherent population trapping (VSCPT) in asym- metric three-level schemes. The light force in such schemes is of an intrinsically transient character and shouldnot be described in a quasiclassical approach. Instead, results of the full quantum-mechanical calculations are presented with emphasis on their meaning to the efficiency of subrecoil laser cooling. 1 INTRODUCTION Laser cooling of neutral atoms has received significant advances by the introduction of velocity-selectivecoherent population trapping ((VSCPT) some years ago.1 Since it leads to atomic temperatures well below therecoil limit, studies of ultracold atoms and atomic interactions may be improved by magnitudes.The effect of VSCPT relies on optical pumping of atoms into a state WNC) which is a trap state for a certaincenter-of-mass velocity vO. This trap state is created by a destructive superposition of atomic states within amultilevel quantum system. Once being in such a state LWNC) the laser light does not interact anymore with theatom which leads to a decoupling with the rest of the system at vo. Atoms located outside this small velocityregion get a chance to be trapped by the momentum diffusion due to spontaneous emission of photons. Aftera sufficient long interaction time nearly all atoms are trapped inside a narrow momentum distribution whichcan be interpreted as cooling. The theoretical and experimental investigation of VSCPT is usually consideredby use of a three-level A-system as shown in Fig.1. Such a system can be found for example in a symmetrical