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Journal of Physics A Mathematical and General

A measurement of optical linewidth by photon-counting statistics

Eric Jakeman, Christopher J. Oliver, Edward R. Pike

Published May 1, 1968• 52 citations
Publisher

Abstract

An optical linewidth of 20 Hz of laser light scattered by spherical particles undergoing Brownian motion has been measured experimentally by photon-counting statistics using the theory of the intensity-fluctuation distribution of Gaussian-Lorentzian light.
DOI
10.1088/0305-4470/1/3/115

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We discuss the quantum-mechanical problem of intensity fluctuations in samples of Gaussian light and its connection with the corresponding classical scalar problem involving fluctuations of random noise power. We obtain an expression for the intensity-fluctuation distribution of light with a Lorentzian spectrum, and investigate analytically its asymptotic behaviour. Numerical techniques are used to evaluate the distribution for various intermediate linewidths, and some examples of the corresponding theoretical photon-counting distributions are also given.
In recent years the utilization of "optical mixing" spectroscopic techniques in laser light scattering experiments has proved to be a successful method for the investigation of the dynamical properties of physical systems. By illuminating a photosensitive detector with the scattered light and measuring the spectrum or autocorrelation function of the resulting photocurrent, one can, in general, obtain the ensemble-average time dependence of specific collective excitations within the scattering medium. We present here a detailed quantitative analysis of the statistical errors inherent in such measurements due to the stochastic nature of both the scattering and photoemission processes. We determine the statistical errors on the optical-intensity correlation function as measured by two photocounting digital correlator models and on the intensity spectrum as measured by a "self-beat" optical mixing spectrometer. From these errors and a generalized least-mean-squares fitting procedure we calculate the uncertainty on the measured correlation time (linewidth) for the case of a Gaussian optical field with an exponential intensity correlation function (a Lorentzian spectrum). Scaling relationships are given which permit our numerical results to be applied to an arbitrary set of experimental parameters.
The authors investigate the statistical errors which arise in digital autocorrelation of photon counting fluctuations due to the finite duration of experiments. An expression for the accuracy with which individual points of the autocorrelation function of intensities can be measured is derived analytically and evaluated for Gaussian- Lorentzian light. The appropriate weighting for a 'least-squares' fitting procedure is determined and the error in spectral linewidth, obtained by this procedure from experiment, is calculated.
The practical treatment of statistics for Gaussian-Lorentzian light is studied theoretically and experimentally by using the time interval distribution of photoelectric pulses, which is derived in two approaches that are based on Markovian processes and the generating function of photon counting statistics, taking the experimental conditions into account. The limits of the validity of the Markovian assumption are made clear. In arbitrary light intensity it is valid experimentally to employ the practical generating function of photon counting distribution expressed as the product of an ideal generating function and a Poissonian one.
Statistical properties of partially polarized Gaussian light were studied experimentally for degrees of polarization PPP from 0.03 to 1 by a standard technique of photon counting. The Gaussian light with an arbitrary degree of polarization was obtained from Rayleigh scattering of orthogonally polarized laser beams. The factorial moments up to sixth order of the photoelectron distribution were measured with an arbitrary temporal and spatial coherence. After corrections were taken for the experimental conditions, the theoretical values of these factorial moments were compared with the experimental results. It is shown that the theoretical predictions were quantitatively well verified by the present measurements. The microscopic process is discussed from the standpoint of the light scattering system used in the present measurements, and it is shown that the orthogonally polarized components of the scattered light observed are statistically independent.