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物性研究

Gaussian, exponential and power-law decays and their time ranges : An analysis based on the Friedrichs model(Perspectives of Nonequilibrium Statistical Physics-The Memory of Professor Shuichi Tasaki-)

Hiromichi Nakazato

Published Dec 5, 2011• 0 citations
OpenAlex

Abstract

The time ranges of the three typical decay forms in quantum mechanics, i.e., the Gaussian, exponential and power-law decays, are investigated on the basis of the Friedrichs model. The analysis yields a deeper understanding of the decay dynamics of quantum systems.

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TEMPORAL BEHAVIOR OF QUANTUM MECHANICAL SYSTEMS

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Results of theoretical studies of the quantum unstable systems caused that there are rather widespread belief that a universal feature of the quantum decay process is the presence of three time regimes of the decay process: the early time (initial) leading to the Quantum Zeno (or Anti Zeno) Effects, “exponential” (or “canonical”) described by the decay law of the exponential form, and late time characterized by the decay law having inverse-power law form. Based on the fundamental principles of the quantum theory we give the proof that there is no time interval in which the survival probability (decay law) could be a decreasing function of time of the purely exponential form but even at the “exponential” regime the decay curve is oscillatory modulated with a smaller or a large amplitude of oscillations depending on parameters of the model considered.
Abstract Methods based on the use of Green’s functions or Jost functions and the Fock–Krylov method are apparently very different approaches to understand the time evolution of unstable states. We show that the two former methods are equivalent up to some constants and as an outcome find an analytic expression for the energy density of states in the Fock–Krylov amplitude in terms of the coefficients introduced in the Green’s functions and the Jost functions methods. This model-independent density is further used to obtain an analytical expression for the survival amplitude and study its behaviour at large times. Using these expressions, we investigate the origin of the oscillatory behaviour of the decay law in the region of the transition from the exponential to the non-exponential at large times. With the objective of understanding the failure of nuclear and particle physics experiments in observing the non-exponential decay law predicted by quantum mechanics for large times, we derive analytical formulae for the critical transition time, , from the exponential to the inverse power law behaviour at large times. Evaluating for some particle resonances and narrow nuclear states which have been tested experimentally to verify the exponential decay law, we conclude that the large time power law in particle and nuclear decay is hard to find experimentally.
In quantum mechanics, the properties of an unstable system are closely related to its corresponding energy distribution. One of the predictions of the theory is the emergence of a late-time power law in the survival probability P(t)P(t)P(t) of the unstable state. However, in complex systems, similar effects may emerge due to other phenomena. This is the case for nonextensive statistical models, for some continuous lifetime distribution models, and also for certain energy-migration models applied to fluorescence. In this work, these alternative interpretations are confronted with data from time-resolved fluorescence spectroscopy experiments with erythrosine B and eosine Y as fluorophores. It turns out that some of the features expected within the quantum-mechanical description, such as the sharp transition from the exponential to the power-law regime, cannot be reproduced by the specific statistical and energy-migration parametrizations fitted in the analysis.
The temporal behavior of quantum mechanical systems is reviewed. We mainly focus our attention on the time development of the so-called “survival” probability of those systems that are initially prepared in eigenstates of the unperturbed Hamiltonian, by assuming that the latter has a continuous spectrum. The exponential decay of the survival probability, familiar, for example, in radioactive decay phenomena, is representative of a purely probabilistic character of the system under consideration and is naturally expected to lead to a master equation. This behavior, however, can be found only at intermediate times, for deviations from it exist both at short and long times and can have significant consequences. After a short introduction to the long history of the research on the temporal behavior of such quantum mechanical systems, the short-time behavior and its controversial consequences when it is combined with von Neumann’s projection postulate in quantum measurement theory are critically overviewed from a dynamical point of view. We also discuss the so-called quantum Zeno effect from this standpoint. The behavior of the survival amplitude is then scrutinized by investigating the analytic properties of its Fourier and Laplace transforms. The analytic property that there is no singularity except a branch cut running along the real energy axis in the first Riemannian sheet is an important reflection of the time-reversal invariance of the dynamics governing the whole process. It is shown that the exponential behavior is due to the presence of a simple pole in the second Riemannian sheet, while the contribution of the branch point yields a power behavior for the amplitude. The exponential decay form is cancelled at short times and dominated at very long times by the branch-point contributions, which give a Gaussian behavior for the former and a power behavior for the latter. In order to realize the exponential law in quantum theory, it is essential to take into account a certain kind of macroscopic nature of the total system, since the exponential behavior is regarded as a manifestation of a complete loss of coherence of the quantum subsystem under consideration. In this respect, a few attempts at extracting the exponential decay form on the basis of quantum theory, aiming at the master equation, are briefly reviewed, including van Hove’s pioneering work and his well-known “λ2T” limit. In the attempt to further clarify the mechanism of the appearance of a purely probabilistic behavior without resort to any approximation, a solvable dynamical model is presented and extensively studied. The model describes an ultrarelativistic particle interacting with N two-level systems (called “spins”) and is shown to exhibit an exponential behavior at all times in the weak-coupling, macroscopic limit. Furthermore, it is shown that the model can even reproduce the short-time Gaussian behavior followed by the exponential law when an appropriate initial state is chosen. The analysis is exact and no approximation is involved. An interpretation for the change of the temporal behavior in quantum systems is drawn from the results obtained. Some implications for the quantum measurement problem are also discussed, in particular in connection with dissipation.
The time evolution of quantum states for unstable particles can be conveniently divided into three domains: the very short time where Zeno's paradox is relevant, the intermediate interval where the exponential decay holds more or less, and the very long time where the decay is governed by a power law. In this work, we reexamine several questions relating to the deviations from the simple exponential decay law. On the basis of general considerations, we demonstrate that deviations from exponential decay near t=0t=0t=0 are inevitable. We formulate general resonance models for the decay. From analytic solutions to specific narrow-width models, we estimate the time parameters T1{T}_{1}T1​ and T2{T}_{2}T2​ separating the three domains. The parameter T1{T}_{1}T1​ is found to be much much less than the lifetime ${\ensuremath{\Gamma}}^{\ensuremath{-}1}$, while T2{T}_{2}T2​ is much greater than the lifetime. For instance, for the charged pion decay, ${T}_{1}\ensuremath{\sim}\frac{{10}^{\ensuremath{-}14}}{\ensuremath{\Gamma}}$ and ${T}_{2}\ensuremath{\sim}\frac{190}{\ensuremath{\Gamma}}$. A resolution of Zeno's paradox provided by the present consideration and its limitaions are discussed.
In the paper, a simple model of alpha decay with Dirac delta potential is studied. The model leads to breakdown of the exponential decay and to power law behavior at asymptotic times. Time dependence of the survival probability of the particle in the potential well is analyzed numerically with two methods: integration of Green's function representation and numerical solution of the time-dependent Schrödinger equation. In particular, finite depth potential wells and behavior between the exponential and power law regimes, which are situations that could not be described in detail analytically, are studied. The numerical results confirm power law with exponent n = 3 after the turnover into the non-exponential decay regime. Moreover, the constructive and destructive interference is observed in the intermediate stage of the process. The simple alpha decay model is compared to the results of Rothe- Hintschich-Monkman experiment which was the first experimental proof of violation of the exponential law.